Machine learning techniques to improve the field performance of low-cost air quality sensors

<p>Low-cost air quality sensors offer significant potential for enhancing urban air quality networks by providing higher-spatiotemporal-resolution data needed, for example, for evaluation of air quality interventions. However, these sensors present methodological and deployment challenges whic...

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Main Authors: T. Bush, N. Papaioannou, F. Leach, F. D. Pope, A. Singh, G. N. Thomas, B. Stacey, S. Bartington
Format: Article
Language:English
Published: Copernicus Publications 2022-06-01
Series:Atmospheric Measurement Techniques
Online Access:https://amt.copernicus.org/articles/15/3261/2022/amt-15-3261-2022.pdf
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author T. Bush
T. Bush
N. Papaioannou
F. Leach
F. D. Pope
A. Singh
G. N. Thomas
B. Stacey
S. Bartington
author_facet T. Bush
T. Bush
N. Papaioannou
F. Leach
F. D. Pope
A. Singh
G. N. Thomas
B. Stacey
S. Bartington
author_sort T. Bush
collection DOAJ
description <p>Low-cost air quality sensors offer significant potential for enhancing urban air quality networks by providing higher-spatiotemporal-resolution data needed, for example, for evaluation of air quality interventions. However, these sensors present methodological and deployment challenges which have historically limited operational ability. These include variability in performance characteristics and sensitivity to environmental conditions. In this work, we investigate field “baselining” and interference correction using random forest regression methods for low-cost sensing of NO<span class="inline-formula"><sub>2</sub></span>, PM<span class="inline-formula"><sub>10</sub></span> (particulate matter) and PM<span class="inline-formula"><sub>2.5</sub></span>. Model performance is explored using data obtained over a 7-month period by real-world field sensor deployment alongside reference method instrumentation. Workflows and processes developed are shown to be effective in normalising variable sensor baseline offsets and reducing uncertainty in sensor response arising from environmental interferences. We demonstrate improvements of between 37 % and 94 % in the mean absolute error term of fully corrected sensor datasets; this is equivalent to performance within <span class="inline-formula">±2.6</span> ppb of the reference method for NO<span class="inline-formula"><sub>2</sub></span>, <span class="inline-formula">±4.4</span> <span class="inline-formula">µ</span>g m<span class="inline-formula"><sup>−3</sup></span> for PM<span class="inline-formula"><sub>10</sub></span> and <span class="inline-formula">±2.7</span> <span class="inline-formula">µ</span>g m<span class="inline-formula"><sup>−3</sup></span> for PM<span class="inline-formula"><sub>2.5</sub></span>. Expanded-uncertainty estimates for PM<span class="inline-formula"><sub>10</sub></span> and PM<span class="inline-formula"><sub>2.5</sub></span> correction models are shown to meet performance criteria recommended by European air quality legislation, whilst that of the NO<span class="inline-formula"><sub>2</sub></span> correction model was found to be narrowly (<span class="inline-formula">∼5</span> %) outside of its acceptance envelope. Expanded-uncertainty estimates for corrected sensor datasets not used in model training were 29 %, 21 % and 27 % for NO<span class="inline-formula"><sub>2</sub></span>, PM<span class="inline-formula"><sub>10</sub></span> and PM<span class="inline-formula"><sub>2.5</sub></span> respectively.</p>
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spelling doaj.art-67116e12fa2f428a80fac7f111f0abd82022-12-22T02:22:14ZengCopernicus PublicationsAtmospheric Measurement Techniques1867-13811867-85482022-06-01153261327810.5194/amt-15-3261-2022Machine learning techniques to improve the field performance of low-cost air quality sensorsT. Bush0T. Bush1N. Papaioannou2F. Leach3F. D. Pope4A. Singh5G. N. Thomas6B. Stacey7S. Bartington8Department of Engineering Science, University of Oxford, Parks Road, Oxford, OX1 3PJ, UKApertum Consulting, Harwell, Oxfordshire, UKDepartment of Engineering Science, University of Oxford, Parks Road, Oxford, OX1 3PJ, UKDepartment of Engineering Science, University of Oxford, Parks Road, Oxford, OX1 3PJ, UKSchool of Geography, Earth and Environmental Sciences, University of Birmingham, Edgbaston, Birmingham, B15 2TT, UKSchool of Geography, Earth and Environmental Sciences, University of Birmingham, Edgbaston, Birmingham, B15 2TT, UKInstitute of Applied Health Research, University of Birmingham, Edgbaston, Birmingham, B15 2TT, UKRicardo Energy & Environment, The Gemini Building, Fermi Avenue, Harwell, Didcot, OX11 0QR, UKInstitute of Applied Health Research, University of Birmingham, Edgbaston, Birmingham, B15 2TT, UK<p>Low-cost air quality sensors offer significant potential for enhancing urban air quality networks by providing higher-spatiotemporal-resolution data needed, for example, for evaluation of air quality interventions. However, these sensors present methodological and deployment challenges which have historically limited operational ability. These include variability in performance characteristics and sensitivity to environmental conditions. In this work, we investigate field “baselining” and interference correction using random forest regression methods for low-cost sensing of NO<span class="inline-formula"><sub>2</sub></span>, PM<span class="inline-formula"><sub>10</sub></span> (particulate matter) and PM<span class="inline-formula"><sub>2.5</sub></span>. Model performance is explored using data obtained over a 7-month period by real-world field sensor deployment alongside reference method instrumentation. Workflows and processes developed are shown to be effective in normalising variable sensor baseline offsets and reducing uncertainty in sensor response arising from environmental interferences. We demonstrate improvements of between 37 % and 94 % in the mean absolute error term of fully corrected sensor datasets; this is equivalent to performance within <span class="inline-formula">±2.6</span> ppb of the reference method for NO<span class="inline-formula"><sub>2</sub></span>, <span class="inline-formula">±4.4</span> <span class="inline-formula">µ</span>g m<span class="inline-formula"><sup>−3</sup></span> for PM<span class="inline-formula"><sub>10</sub></span> and <span class="inline-formula">±2.7</span> <span class="inline-formula">µ</span>g m<span class="inline-formula"><sup>−3</sup></span> for PM<span class="inline-formula"><sub>2.5</sub></span>. Expanded-uncertainty estimates for PM<span class="inline-formula"><sub>10</sub></span> and PM<span class="inline-formula"><sub>2.5</sub></span> correction models are shown to meet performance criteria recommended by European air quality legislation, whilst that of the NO<span class="inline-formula"><sub>2</sub></span> correction model was found to be narrowly (<span class="inline-formula">∼5</span> %) outside of its acceptance envelope. Expanded-uncertainty estimates for corrected sensor datasets not used in model training were 29 %, 21 % and 27 % for NO<span class="inline-formula"><sub>2</sub></span>, PM<span class="inline-formula"><sub>10</sub></span> and PM<span class="inline-formula"><sub>2.5</sub></span> respectively.</p>https://amt.copernicus.org/articles/15/3261/2022/amt-15-3261-2022.pdf
spellingShingle T. Bush
T. Bush
N. Papaioannou
F. Leach
F. D. Pope
A. Singh
G. N. Thomas
B. Stacey
S. Bartington
Machine learning techniques to improve the field performance of low-cost air quality sensors
Atmospheric Measurement Techniques
title Machine learning techniques to improve the field performance of low-cost air quality sensors
title_full Machine learning techniques to improve the field performance of low-cost air quality sensors
title_fullStr Machine learning techniques to improve the field performance of low-cost air quality sensors
title_full_unstemmed Machine learning techniques to improve the field performance of low-cost air quality sensors
title_short Machine learning techniques to improve the field performance of low-cost air quality sensors
title_sort machine learning techniques to improve the field performance of low cost air quality sensors
url https://amt.copernicus.org/articles/15/3261/2022/amt-15-3261-2022.pdf
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