Enhancing the Output Performance of a Triboelectric Nanogenerator Based on Modified Polyimide and Sandwich-Structured Nanocomposite Film

Recently, scientists have been facing major obstacles in terms of improving the performances of dielectric materials for triboelectric nanogenerators. The triboelectric nanogenerator (TENG) is one of the first green energy technologies that can convert random mechanical kinetic energy into electrici...

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Main Authors: Jiaheng Zhou, Chunhao Lu, Danquan Lan, Yiyi Zhang, Yiquan Lin, Lingyu Wan, Wenchang Wei, Yuwang Liang, Dongxin Guo, Yansong Liu, Wenyao Yu
Format: Article
Language:English
Published: MDPI AG 2023-03-01
Series:Nanomaterials
Subjects:
Online Access:https://www.mdpi.com/2079-4991/13/6/1056
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author Jiaheng Zhou
Chunhao Lu
Danquan Lan
Yiyi Zhang
Yiquan Lin
Lingyu Wan
Wenchang Wei
Yuwang Liang
Dongxin Guo
Yansong Liu
Wenyao Yu
author_facet Jiaheng Zhou
Chunhao Lu
Danquan Lan
Yiyi Zhang
Yiquan Lin
Lingyu Wan
Wenchang Wei
Yuwang Liang
Dongxin Guo
Yansong Liu
Wenyao Yu
author_sort Jiaheng Zhou
collection DOAJ
description Recently, scientists have been facing major obstacles in terms of improving the performances of dielectric materials for triboelectric nanogenerators. The triboelectric nanogenerator (TENG) is one of the first green energy technologies that can convert random mechanical kinetic energy into electricity. The surface charge density of TENGs is a critical factor speeding up their commercialization, so it is important to explore unique methods to increase the surface charge density. The key to obtaining a high-performance TENG is the preparation of dielectric materials with good mechanical properties, thermal stability and output performance. To solve the problem of the low output performance of PI-based triboelectric nanogenerators, we modified PI films by introducing nanomaterials and designed a new type of sandwich-shaped nanocomposite film. Herein, we used polyimide (PI) with ideal mechanical properties, excellent heat resistance and flexibility as the dielectric material, prepared an A-B-A sandwich structure with PI in the outer layer and modified a copper calcium titanate/polyimide (CCTO/PI) storage layer in the middle to improve the output of a TENG electrode. The doping amount of the CCTO was tailored. The results showed that at 8 wt% CCTO content, the electrical output performance was the highest, and the open-circuit voltage of CCTO/PI was 42 V. In the TENG, the open-circuit voltage, short-circuit current and transfer charge of the prepared sandwich-structured film were increased by 607%, 629% and 672% compared to the TENG with the PI thin film, respectively. This study presents a novel strategy of optimizing dielectric materials for triboelectric nano-generators and has great potential for the future development of high output-performance TENGs.
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spelling doaj.art-67949f1948244299994eb83a19c0f32f2023-11-17T13:00:55ZengMDPI AGNanomaterials2079-49912023-03-01136105610.3390/nano13061056Enhancing the Output Performance of a Triboelectric Nanogenerator Based on Modified Polyimide and Sandwich-Structured Nanocomposite FilmJiaheng Zhou0Chunhao Lu1Danquan Lan2Yiyi Zhang3Yiquan Lin4Lingyu Wan5Wenchang Wei6Yuwang Liang7Dongxin Guo8Yansong Liu9Wenyao Yu10Guangxi Power Transmission and Distribution Network Lightning Protection Engineering Technology Research Center, Guangxi University, Nanning 530004, ChinaGuangxi Power Grid Co., Ltd., Nanning 530023, ChinaGuangxi Power Transmission and Distribution Network Lightning Protection Engineering Technology Research Center, Guangxi University, Nanning 530004, ChinaGuangxi Power Transmission and Distribution Network Lightning Protection Engineering Technology Research Center, Guangxi University, Nanning 530004, ChinaSPIC Guangxi Electric Power Co., Ltd., Nanning 530004, ChinaSchool of Physical Science and Technology, Guangxi University, Nanning 530004, ChinaGuangxi Power Transmission and Distribution Network Lightning Protection Engineering Technology Research Center, Guangxi University, Nanning 530004, ChinaGuangxi Power Transmission and Distribution Network Lightning Protection Engineering Technology Research Center, Guangxi University, Nanning 530004, ChinaSchool of Physical Science and Technology, Guangxi University, Nanning 530004, ChinaGuangxi Power Transmission and Distribution Network Lightning Protection Engineering Technology Research Center, Guangxi University, Nanning 530004, ChinaGuangxi Power Transmission and Distribution Network Lightning Protection Engineering Technology Research Center, Guangxi University, Nanning 530004, ChinaRecently, scientists have been facing major obstacles in terms of improving the performances of dielectric materials for triboelectric nanogenerators. The triboelectric nanogenerator (TENG) is one of the first green energy technologies that can convert random mechanical kinetic energy into electricity. The surface charge density of TENGs is a critical factor speeding up their commercialization, so it is important to explore unique methods to increase the surface charge density. The key to obtaining a high-performance TENG is the preparation of dielectric materials with good mechanical properties, thermal stability and output performance. To solve the problem of the low output performance of PI-based triboelectric nanogenerators, we modified PI films by introducing nanomaterials and designed a new type of sandwich-shaped nanocomposite film. Herein, we used polyimide (PI) with ideal mechanical properties, excellent heat resistance and flexibility as the dielectric material, prepared an A-B-A sandwich structure with PI in the outer layer and modified a copper calcium titanate/polyimide (CCTO/PI) storage layer in the middle to improve the output of a TENG electrode. The doping amount of the CCTO was tailored. The results showed that at 8 wt% CCTO content, the electrical output performance was the highest, and the open-circuit voltage of CCTO/PI was 42 V. In the TENG, the open-circuit voltage, short-circuit current and transfer charge of the prepared sandwich-structured film were increased by 607%, 629% and 672% compared to the TENG with the PI thin film, respectively. This study presents a novel strategy of optimizing dielectric materials for triboelectric nano-generators and has great potential for the future development of high output-performance TENGs.https://www.mdpi.com/2079-4991/13/6/1056sandwich-structured nanocompositespolyimidetriboelectric nanogenerators
spellingShingle Jiaheng Zhou
Chunhao Lu
Danquan Lan
Yiyi Zhang
Yiquan Lin
Lingyu Wan
Wenchang Wei
Yuwang Liang
Dongxin Guo
Yansong Liu
Wenyao Yu
Enhancing the Output Performance of a Triboelectric Nanogenerator Based on Modified Polyimide and Sandwich-Structured Nanocomposite Film
Nanomaterials
sandwich-structured nanocomposites
polyimide
triboelectric nanogenerators
title Enhancing the Output Performance of a Triboelectric Nanogenerator Based on Modified Polyimide and Sandwich-Structured Nanocomposite Film
title_full Enhancing the Output Performance of a Triboelectric Nanogenerator Based on Modified Polyimide and Sandwich-Structured Nanocomposite Film
title_fullStr Enhancing the Output Performance of a Triboelectric Nanogenerator Based on Modified Polyimide and Sandwich-Structured Nanocomposite Film
title_full_unstemmed Enhancing the Output Performance of a Triboelectric Nanogenerator Based on Modified Polyimide and Sandwich-Structured Nanocomposite Film
title_short Enhancing the Output Performance of a Triboelectric Nanogenerator Based on Modified Polyimide and Sandwich-Structured Nanocomposite Film
title_sort enhancing the output performance of a triboelectric nanogenerator based on modified polyimide and sandwich structured nanocomposite film
topic sandwich-structured nanocomposites
polyimide
triboelectric nanogenerators
url https://www.mdpi.com/2079-4991/13/6/1056
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