Study into the dependence of the Co-60 and Lu-177g production efficiency on the energy structure of neutron flux density

At present, the existing approaches to production of artificial isotopes are mostly based on the development experience from previous years. This work aims to develop an algorithm for selecting the most effective irradiation modes for target materials. The study is based on sequential modeling of ir...

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Main Authors: Ruben A. Shaginyan, Valery V. Korobeinikov, Viktor Yu. Stogov
Format: Article
Language:English
Published: National Research Nuclear University (MEPhI) 2023-12-01
Series:Nuclear Energy and Technology
Subjects:
Online Access:https://nucet.pensoft.net/article/116662/download/pdf/
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author Ruben A. Shaginyan
Valery V. Korobeinikov
Viktor Yu. Stogov
author_facet Ruben A. Shaginyan
Valery V. Korobeinikov
Viktor Yu. Stogov
author_sort Ruben A. Shaginyan
collection DOAJ
description At present, the existing approaches to production of artificial isotopes are mostly based on the development experience from previous years. This work aims to develop an algorithm for selecting the most effective irradiation modes for target materials. The study is based on sequential modeling of irradiation of target isotopes by neutrons of different ‘single-group’ fluxes at the same neutron flux density within each energy group (BNAB-93). In this study, a flux density equal to 2×1015 n/(cm2×s) was used for each energy group. This approach will help ‘designing’ and selecting the actual neutron spectrum that has the highest efficiency compared to alternatives. The study modelled Co-60 and Lu-177g production for each energy group. The kinetics was analyzed in the most efficient groups in terms of specific activity. The maximum specific activity for Co-60 is reached in group 17 and is equal to 1 kCi/g. For the scheme of Lu-177g production through Lu-176 the maximum specific activity is reached in group 26 and is equal to 58.5 kCi/g. For the scheme of Lu-177g production through Yb-176, the maximum specific activity is reached in group 17 and is equal to 260 Ci/g, advantageous for production are groups 15–17 and 26.
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spelling doaj.art-68101228443349009d3cafc8b03c11712023-12-22T15:29:51ZengNational Research Nuclear University (MEPhI)Nuclear Energy and Technology2452-30382023-12-019428128710.3897/nucet.9.116662116662Study into the dependence of the Co-60 and Lu-177g production efficiency on the energy structure of neutron flux densityRuben A. Shaginyan0Valery V. Korobeinikov1Viktor Yu. Stogov2IPPE JSCIPPE JSCIPPE JSCAt present, the existing approaches to production of artificial isotopes are mostly based on the development experience from previous years. This work aims to develop an algorithm for selecting the most effective irradiation modes for target materials. The study is based on sequential modeling of irradiation of target isotopes by neutrons of different ‘single-group’ fluxes at the same neutron flux density within each energy group (BNAB-93). In this study, a flux density equal to 2×1015 n/(cm2×s) was used for each energy group. This approach will help ‘designing’ and selecting the actual neutron spectrum that has the highest efficiency compared to alternatives. The study modelled Co-60 and Lu-177g production for each energy group. The kinetics was analyzed in the most efficient groups in terms of specific activity. The maximum specific activity for Co-60 is reached in group 17 and is equal to 1 kCi/g. For the scheme of Lu-177g production through Lu-176 the maximum specific activity is reached in group 26 and is equal to 58.5 kCi/g. For the scheme of Lu-177g production through Yb-176, the maximum specific activity is reached in group 17 and is equal to 260 Ci/g, advantageous for production are groups 15–17 and 26.https://nucet.pensoft.net/article/116662/download/pdf/productionisotopesspecific act
spellingShingle Ruben A. Shaginyan
Valery V. Korobeinikov
Viktor Yu. Stogov
Study into the dependence of the Co-60 and Lu-177g production efficiency on the energy structure of neutron flux density
Nuclear Energy and Technology
production
isotopes
specific act
title Study into the dependence of the Co-60 and Lu-177g production efficiency on the energy structure of neutron flux density
title_full Study into the dependence of the Co-60 and Lu-177g production efficiency on the energy structure of neutron flux density
title_fullStr Study into the dependence of the Co-60 and Lu-177g production efficiency on the energy structure of neutron flux density
title_full_unstemmed Study into the dependence of the Co-60 and Lu-177g production efficiency on the energy structure of neutron flux density
title_short Study into the dependence of the Co-60 and Lu-177g production efficiency on the energy structure of neutron flux density
title_sort study into the dependence of the co 60 and lu 177g production efficiency on the energy structure of neutron flux density
topic production
isotopes
specific act
url https://nucet.pensoft.net/article/116662/download/pdf/
work_keys_str_mv AT rubenashaginyan studyintothedependenceoftheco60andlu177gproductionefficiencyontheenergystructureofneutronfluxdensity
AT valeryvkorobeinikov studyintothedependenceoftheco60andlu177gproductionefficiencyontheenergystructureofneutronfluxdensity
AT viktoryustogov studyintothedependenceoftheco60andlu177gproductionefficiencyontheenergystructureofneutronfluxdensity