Efficient pump-probe sampling with a single-cavity dual-comb laser: Application in ultrafast photoacoustics

Ultrafast pump-probe measurements are used to characterize various samples, such as biological cells, bulk, and thin-film structures. However, typical implementations of the pump-probe apparatus are either slow or complex and costly hindering wide deployment. Here we combine a single-cavity dual-com...

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Main Authors: J. Pupeikis, W. Hu, B. Willenberg, M. Mehendale, G.A. Antonelli, C.R. Phillips, U. Keller
Format: Article
Language:English
Published: Elsevier 2023-02-01
Series:Photoacoustics
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2213597922001045
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author J. Pupeikis
W. Hu
B. Willenberg
M. Mehendale
G.A. Antonelli
C.R. Phillips
U. Keller
author_facet J. Pupeikis
W. Hu
B. Willenberg
M. Mehendale
G.A. Antonelli
C.R. Phillips
U. Keller
author_sort J. Pupeikis
collection DOAJ
description Ultrafast pump-probe measurements are used to characterize various samples, such as biological cells, bulk, and thin-film structures. However, typical implementations of the pump-probe apparatus are either slow or complex and costly hindering wide deployment. Here we combine a single-cavity dual-comb laser with a simple experimental setup to obtain pump-probe measurements with ultra-high sensitivity, fast acquisition, and high timing precision over long optical delay scan ranges of 12.5 ns that would correspond to a mechanical delay of about 3.75 m. We employ digital signal balancing to obtain shot-noise-limited detection compatible with pump-probe microscopy deployment. Here we demonstrate ultrafast photoacoustics for thin-film sample characterization. We measured a tungsten layer thickness of (700 ± 4) Å with shot-noise-limited detection. Such single-cavity dual-comb lasers can be used for any pump-probe measurements and are especially well-suited for ultrafast photoacoustic studies such as involving ultrasonic echoes, Brillouin oscillations, surface acoustic waves and thermal dynamics.
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spelling doaj.art-68f87ff1a3034cb8a92cefcd2ee4118e2023-02-12T04:14:44ZengElsevierPhotoacoustics2213-59792023-02-0129100439Efficient pump-probe sampling with a single-cavity dual-comb laser: Application in ultrafast photoacousticsJ. Pupeikis0W. Hu1B. Willenberg2M. Mehendale3G.A. Antonelli4C.R. Phillips5U. Keller6ETH Zurich, Auguste-Piccard-Hof 1, Zurich 8093, Switzerland; Corresponding author.ETH Zurich, Auguste-Piccard-Hof 1, Zurich 8093, SwitzerlandETH Zurich, Auguste-Piccard-Hof 1, Zurich 8093, SwitzerlandOnto Innovation Inc., 16 Jonspin Road, Wilmington, MA 01887, USAOnto Innovation Inc., 16 Jonspin Road, Wilmington, MA 01887, USAETH Zurich, Auguste-Piccard-Hof 1, Zurich 8093, SwitzerlandETH Zurich, Auguste-Piccard-Hof 1, Zurich 8093, SwitzerlandUltrafast pump-probe measurements are used to characterize various samples, such as biological cells, bulk, and thin-film structures. However, typical implementations of the pump-probe apparatus are either slow or complex and costly hindering wide deployment. Here we combine a single-cavity dual-comb laser with a simple experimental setup to obtain pump-probe measurements with ultra-high sensitivity, fast acquisition, and high timing precision over long optical delay scan ranges of 12.5 ns that would correspond to a mechanical delay of about 3.75 m. We employ digital signal balancing to obtain shot-noise-limited detection compatible with pump-probe microscopy deployment. Here we demonstrate ultrafast photoacoustics for thin-film sample characterization. We measured a tungsten layer thickness of (700 ± 4) Å with shot-noise-limited detection. Such single-cavity dual-comb lasers can be used for any pump-probe measurements and are especially well-suited for ultrafast photoacoustic studies such as involving ultrasonic echoes, Brillouin oscillations, surface acoustic waves and thermal dynamics.http://www.sciencedirect.com/science/article/pii/S2213597922001045Ultrafast pump-probePicosecond ultrasonicsPump-probe microscopyTime domain thermoreflectanceTDTRTime-resolved Brillouin oscillations
spellingShingle J. Pupeikis
W. Hu
B. Willenberg
M. Mehendale
G.A. Antonelli
C.R. Phillips
U. Keller
Efficient pump-probe sampling with a single-cavity dual-comb laser: Application in ultrafast photoacoustics
Photoacoustics
Ultrafast pump-probe
Picosecond ultrasonics
Pump-probe microscopy
Time domain thermoreflectance
TDTR
Time-resolved Brillouin oscillations
title Efficient pump-probe sampling with a single-cavity dual-comb laser: Application in ultrafast photoacoustics
title_full Efficient pump-probe sampling with a single-cavity dual-comb laser: Application in ultrafast photoacoustics
title_fullStr Efficient pump-probe sampling with a single-cavity dual-comb laser: Application in ultrafast photoacoustics
title_full_unstemmed Efficient pump-probe sampling with a single-cavity dual-comb laser: Application in ultrafast photoacoustics
title_short Efficient pump-probe sampling with a single-cavity dual-comb laser: Application in ultrafast photoacoustics
title_sort efficient pump probe sampling with a single cavity dual comb laser application in ultrafast photoacoustics
topic Ultrafast pump-probe
Picosecond ultrasonics
Pump-probe microscopy
Time domain thermoreflectance
TDTR
Time-resolved Brillouin oscillations
url http://www.sciencedirect.com/science/article/pii/S2213597922001045
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