Investigating Influential Parameters for High-Purity Germanium Crystal Growth

This paper focuses on the research and development of high-purity germanium (HPGe) crystals for detector fabrication, specifically targeting applications in rare-event physics searches. The primary objective was to produce large-scale germanium crystals weighing >1 kg with a controlled diameter o...

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Main Authors: Sanjay Bhattarai, Dongming Mei, Narayan Budhathoki, Kunming Dong, Austin Warren
Format: Article
Language:English
Published: MDPI AG 2024-02-01
Series:Crystals
Subjects:
Online Access:https://www.mdpi.com/2073-4352/14/2/177
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author Sanjay Bhattarai
Dongming Mei
Narayan Budhathoki
Kunming Dong
Austin Warren
author_facet Sanjay Bhattarai
Dongming Mei
Narayan Budhathoki
Kunming Dong
Austin Warren
author_sort Sanjay Bhattarai
collection DOAJ
description This paper focuses on the research and development of high-purity germanium (HPGe) crystals for detector fabrication, specifically targeting applications in rare-event physics searches. The primary objective was to produce large-scale germanium crystals weighing >1 kg with a controlled diameter of ∼10 cm and an impurity range of approximately <inline-formula><math xmlns="http://www.w3.org/1998/Math/MathML" display="inline"><semantics><msup><mn>10</mn><mn>10</mn></msup></semantics></math></inline-formula>/cm<inline-formula><math xmlns="http://www.w3.org/1998/Math/MathML" display="inline"><semantics><msup><mo> </mo><mn>3</mn></msup></semantics></math></inline-formula>. Ensuring structural integrity and excellent crystalline quality requires a thorough assessment of dislocation density, a critical aspect of the crystal development process. Dislocation density measurements play a crucial role in maximizing the sensitivity of HPGe detectors, and our findings confirmed that the dislocation density fell within acceptable ranges for detector fabrication. Additionally, this paper examines the segregation coefficient of various contaminants during the crystal development process. Comprehensive analysis of impurity segregation is essential for reducing contaminant quantities in the crystal lattice and customizing purification processes. This, in turn, minimizes undesired background noise, enhancing signal-to-noise ratios for rare-event physics searches and overall detector performance. The investigation included the segregation coefficients of three major acceptors and one donor in crystals grown at the University of South Dakota, providing valuable insights for optimizing crystal purity and detector efficiency.
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spelling doaj.art-69a68f27be9544798b1ead4d229889782024-02-23T15:13:17ZengMDPI AGCrystals2073-43522024-02-0114217710.3390/cryst14020177Investigating Influential Parameters for High-Purity Germanium Crystal GrowthSanjay Bhattarai0Dongming Mei1Narayan Budhathoki2Kunming Dong3Austin Warren4Department of Physics, University of South Dakota, Vermillion, SD 57069, USADepartment of Physics, University of South Dakota, Vermillion, SD 57069, USADepartment of Physics, University of South Dakota, Vermillion, SD 57069, USADepartment of Physics, University of South Dakota, Vermillion, SD 57069, USADepartment of Physics, University of South Dakota, Vermillion, SD 57069, USAThis paper focuses on the research and development of high-purity germanium (HPGe) crystals for detector fabrication, specifically targeting applications in rare-event physics searches. The primary objective was to produce large-scale germanium crystals weighing >1 kg with a controlled diameter of ∼10 cm and an impurity range of approximately <inline-formula><math xmlns="http://www.w3.org/1998/Math/MathML" display="inline"><semantics><msup><mn>10</mn><mn>10</mn></msup></semantics></math></inline-formula>/cm<inline-formula><math xmlns="http://www.w3.org/1998/Math/MathML" display="inline"><semantics><msup><mo> </mo><mn>3</mn></msup></semantics></math></inline-formula>. Ensuring structural integrity and excellent crystalline quality requires a thorough assessment of dislocation density, a critical aspect of the crystal development process. Dislocation density measurements play a crucial role in maximizing the sensitivity of HPGe detectors, and our findings confirmed that the dislocation density fell within acceptable ranges for detector fabrication. Additionally, this paper examines the segregation coefficient of various contaminants during the crystal development process. Comprehensive analysis of impurity segregation is essential for reducing contaminant quantities in the crystal lattice and customizing purification processes. This, in turn, minimizes undesired background noise, enhancing signal-to-noise ratios for rare-event physics searches and overall detector performance. The investigation included the segregation coefficients of three major acceptors and one donor in crystals grown at the University of South Dakota, providing valuable insights for optimizing crystal purity and detector efficiency.https://www.mdpi.com/2073-4352/14/2/177crystal growthimpurity segregationdislocation densitynet impurity concentration
spellingShingle Sanjay Bhattarai
Dongming Mei
Narayan Budhathoki
Kunming Dong
Austin Warren
Investigating Influential Parameters for High-Purity Germanium Crystal Growth
Crystals
crystal growth
impurity segregation
dislocation density
net impurity concentration
title Investigating Influential Parameters for High-Purity Germanium Crystal Growth
title_full Investigating Influential Parameters for High-Purity Germanium Crystal Growth
title_fullStr Investigating Influential Parameters for High-Purity Germanium Crystal Growth
title_full_unstemmed Investigating Influential Parameters for High-Purity Germanium Crystal Growth
title_short Investigating Influential Parameters for High-Purity Germanium Crystal Growth
title_sort investigating influential parameters for high purity germanium crystal growth
topic crystal growth
impurity segregation
dislocation density
net impurity concentration
url https://www.mdpi.com/2073-4352/14/2/177
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AT narayanbudhathoki investigatinginfluentialparametersforhighpuritygermaniumcrystalgrowth
AT kunmingdong investigatinginfluentialparametersforhighpuritygermaniumcrystalgrowth
AT austinwarren investigatinginfluentialparametersforhighpuritygermaniumcrystalgrowth