Chiral nematic liquid crystal microlenses

Abstract Nematic liquid crystals (NLCs) of achiral molecules and racemic mixtures of chiral ones form flat films and show uniform textures between circular polarizers when suspended in sub-millimeter size grids and immersed in water. On addition of chiral dopants to the liquid crystal, the films exh...

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Main Authors: Piotr Popov, Lawrence W. Honaker, Mona Mirheydari, Elizabeth K. Mann, Antal Jákli
Format: Article
Language:English
Published: Nature Portfolio 2017-05-01
Series:Scientific Reports
Online Access:https://doi.org/10.1038/s41598-017-01595-6
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author Piotr Popov
Lawrence W. Honaker
Mona Mirheydari
Elizabeth K. Mann
Antal Jákli
author_facet Piotr Popov
Lawrence W. Honaker
Mona Mirheydari
Elizabeth K. Mann
Antal Jákli
author_sort Piotr Popov
collection DOAJ
description Abstract Nematic liquid crystals (NLCs) of achiral molecules and racemic mixtures of chiral ones form flat films and show uniform textures between circular polarizers when suspended in sub-millimeter size grids and immersed in water. On addition of chiral dopants to the liquid crystal, the films exhibit optical textures with concentric ring patterns and radial variation of the birefringence color. Both are related to a biconvex shape of the chiral liquid crystal film; the rings are due to interference. The curvature radii of the biconvex lens array are in the range of a few millimeters. This curvature leads to a radial variation of the optical axis along the plane of the film. Such a Pancharatnam-type phase lens dominates the imaging and explains the measured focal length of about one millimeter. To our knowledge, these are the first spontaneously formed Pancharatnam devices. The unwinding of the helical structure at the grid walls drives the lens shape. The relation between the lens curvature and material properties such as helical pitch, the twist elastic constant, and the interfacial tensions, is derived. This simple, novel method for spontaneously forming microlens arrays can also be used for various sensors.
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spelling doaj.art-69f6183ed6a945abb4a70d18c10853152022-12-21T21:20:51ZengNature PortfolioScientific Reports2045-23222017-05-01711910.1038/s41598-017-01595-6Chiral nematic liquid crystal microlensesPiotr Popov0Lawrence W. Honaker1Mona Mirheydari2Elizabeth K. Mann3Antal Jákli4Physics Department, Kent State UniversityLiquid Crystal Institute, Kent State UniversityPhysics Department, Kent State UniversityPhysics Department, Kent State UniversityLiquid Crystal Institute, Kent State UniversityAbstract Nematic liquid crystals (NLCs) of achiral molecules and racemic mixtures of chiral ones form flat films and show uniform textures between circular polarizers when suspended in sub-millimeter size grids and immersed in water. On addition of chiral dopants to the liquid crystal, the films exhibit optical textures with concentric ring patterns and radial variation of the birefringence color. Both are related to a biconvex shape of the chiral liquid crystal film; the rings are due to interference. The curvature radii of the biconvex lens array are in the range of a few millimeters. This curvature leads to a radial variation of the optical axis along the plane of the film. Such a Pancharatnam-type phase lens dominates the imaging and explains the measured focal length of about one millimeter. To our knowledge, these are the first spontaneously formed Pancharatnam devices. The unwinding of the helical structure at the grid walls drives the lens shape. The relation between the lens curvature and material properties such as helical pitch, the twist elastic constant, and the interfacial tensions, is derived. This simple, novel method for spontaneously forming microlens arrays can also be used for various sensors.https://doi.org/10.1038/s41598-017-01595-6
spellingShingle Piotr Popov
Lawrence W. Honaker
Mona Mirheydari
Elizabeth K. Mann
Antal Jákli
Chiral nematic liquid crystal microlenses
Scientific Reports
title Chiral nematic liquid crystal microlenses
title_full Chiral nematic liquid crystal microlenses
title_fullStr Chiral nematic liquid crystal microlenses
title_full_unstemmed Chiral nematic liquid crystal microlenses
title_short Chiral nematic liquid crystal microlenses
title_sort chiral nematic liquid crystal microlenses
url https://doi.org/10.1038/s41598-017-01595-6
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AT lawrencewhonaker chiralnematicliquidcrystalmicrolenses
AT monamirheydari chiralnematicliquidcrystalmicrolenses
AT elizabethkmann chiralnematicliquidcrystalmicrolenses
AT antaljakli chiralnematicliquidcrystalmicrolenses