Simply synthesized nitrogen-doped graphene quantum dot (NGQD)-modified electrode for the ultrasensitive photoelectrochemical detection of dopamine

Recently, nitrogen-doped graphene quantum dots (NGQDs), as a new type of quantum semiconductor and photoelectrochemical material, are promising candidates in photoelectric sensing, water splitting, and biological imaging and have various potential application prospects. In this work, NGQDs were prep...

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Main Authors: Wang Jin, Lu Cheng, Chen Tingting, Hu Lanping, Du Yukou, Yao Yong, Goh M. Cynthia
Format: Article
Language:English
Published: De Gruyter 2019-11-01
Series:Nanophotonics
Subjects:
Online Access:https://doi.org/10.1515/nanoph-2019-0418
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author Wang Jin
Lu Cheng
Chen Tingting
Hu Lanping
Du Yukou
Yao Yong
Goh M. Cynthia
author_facet Wang Jin
Lu Cheng
Chen Tingting
Hu Lanping
Du Yukou
Yao Yong
Goh M. Cynthia
author_sort Wang Jin
collection DOAJ
description Recently, nitrogen-doped graphene quantum dots (NGQDs), as a new type of quantum semiconductor and photoelectrochemical material, are promising candidates in photoelectric sensing, water splitting, and biological imaging and have various potential application prospects. In this work, NGQDs were prepared by a simple calcination method, and then a photoelectrochemical sensing platform based on the NGQDs electrode with superior photoelectrochemical activity was designed and fabricated for the detection of dopamine (DA). Benefitting from the quantum effect and size effect, NGQDs displayed an enhanced photocurrent effective within ultra-low detection limit (0.03 μm), wide detection range (0.03–450 and 450–9680 μm), and high sensitivity in detecting DA with the assistance of ultraviolet light irradiation. The NGQDs electrode also showed continuous and stable photocurrent densities after long-term experiment, indicating the excellent durability of NGQDs for DA detection.
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spelling doaj.art-6ad153cbb3554f6bb41e00728268dd4f2022-12-21T23:30:30ZengDe GruyterNanophotonics2192-86062192-86142019-11-019123831383910.1515/nanoph-2019-0418nanoph-2019-0418Simply synthesized nitrogen-doped graphene quantum dot (NGQD)-modified electrode for the ultrasensitive photoelectrochemical detection of dopamineWang Jin0Lu Cheng1Chen Tingting2Hu Lanping3Du Yukou4Yao Yong5Goh M. Cynthia6School of Chemistry and Chemical Engineering, Nantong University, Nantong 226019, ChinaDepartment of Chemistry, Materials Science and Engineering, Institute of Medical Science, University of Toronto, Toronto, Ontario M5S 3H6, CanadaSchool of Chemistry and Chemical Engineering, Nantong University, Nantong 226019, ChinaSchool of Chemistry and Chemical Engineering, Nantong University, Nantong 226019, ChinaCollege of Chemistry, Chemical Engineering and Materials Science, Soochow University, Suzhou 215123, ChinaSchool of Chemistry and Chemical Engineering, Nantong University, Nantong 226019, ChinaDepartment of Chemistry, Materials Science and Engineering, Institute of Medical Science, University of Toronto, Toronto, Ontario M5S 3H6, CanadaRecently, nitrogen-doped graphene quantum dots (NGQDs), as a new type of quantum semiconductor and photoelectrochemical material, are promising candidates in photoelectric sensing, water splitting, and biological imaging and have various potential application prospects. In this work, NGQDs were prepared by a simple calcination method, and then a photoelectrochemical sensing platform based on the NGQDs electrode with superior photoelectrochemical activity was designed and fabricated for the detection of dopamine (DA). Benefitting from the quantum effect and size effect, NGQDs displayed an enhanced photocurrent effective within ultra-low detection limit (0.03 μm), wide detection range (0.03–450 and 450–9680 μm), and high sensitivity in detecting DA with the assistance of ultraviolet light irradiation. The NGQDs electrode also showed continuous and stable photocurrent densities after long-term experiment, indicating the excellent durability of NGQDs for DA detection.https://doi.org/10.1515/nanoph-2019-0418ngqdsphotoelectrochemistrydopamineultrasensitive detection
spellingShingle Wang Jin
Lu Cheng
Chen Tingting
Hu Lanping
Du Yukou
Yao Yong
Goh M. Cynthia
Simply synthesized nitrogen-doped graphene quantum dot (NGQD)-modified electrode for the ultrasensitive photoelectrochemical detection of dopamine
Nanophotonics
ngqds
photoelectrochemistry
dopamine
ultrasensitive detection
title Simply synthesized nitrogen-doped graphene quantum dot (NGQD)-modified electrode for the ultrasensitive photoelectrochemical detection of dopamine
title_full Simply synthesized nitrogen-doped graphene quantum dot (NGQD)-modified electrode for the ultrasensitive photoelectrochemical detection of dopamine
title_fullStr Simply synthesized nitrogen-doped graphene quantum dot (NGQD)-modified electrode for the ultrasensitive photoelectrochemical detection of dopamine
title_full_unstemmed Simply synthesized nitrogen-doped graphene quantum dot (NGQD)-modified electrode for the ultrasensitive photoelectrochemical detection of dopamine
title_short Simply synthesized nitrogen-doped graphene quantum dot (NGQD)-modified electrode for the ultrasensitive photoelectrochemical detection of dopamine
title_sort simply synthesized nitrogen doped graphene quantum dot ngqd modified electrode for the ultrasensitive photoelectrochemical detection of dopamine
topic ngqds
photoelectrochemistry
dopamine
ultrasensitive detection
url https://doi.org/10.1515/nanoph-2019-0418
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