Two-dimensional electronic spectroscopy reveals liquid-like lineshape dynamics in CsPbI3 perovskite nanocrystals
Lead-halide perovskites have promising optoelectronic properties, determined by interplay of electronic and structural properties. Here the authors probe CsPbI3 nanocrystals by two-dimensional electronic spectroscopy, showing liquid-like structural dynamics signature of polaron formation.
Main Authors: | , , , , , , |
---|---|
Format: | Article |
Language: | English |
Published: |
Nature Portfolio
2019-10-01
|
Series: | Nature Communications |
Online Access: | https://doi.org/10.1038/s41467-019-12830-1 |
_version_ | 1818835230952259584 |
---|---|
author | Hélène Seiler Samuel Palato Colin Sonnichsen Harry Baker Etienne Socie Dallas P. Strandell Patanjali Kambhampati |
author_facet | Hélène Seiler Samuel Palato Colin Sonnichsen Harry Baker Etienne Socie Dallas P. Strandell Patanjali Kambhampati |
author_sort | Hélène Seiler |
collection | DOAJ |
description | Lead-halide perovskites have promising optoelectronic properties, determined by interplay of electronic and structural properties. Here the authors probe CsPbI3 nanocrystals by two-dimensional electronic spectroscopy, showing liquid-like structural dynamics signature of polaron formation. |
first_indexed | 2024-12-19T02:47:25Z |
format | Article |
id | doaj.art-6b0dab175ca04375aefa407478f3240a |
institution | Directory Open Access Journal |
issn | 2041-1723 |
language | English |
last_indexed | 2024-12-19T02:47:25Z |
publishDate | 2019-10-01 |
publisher | Nature Portfolio |
record_format | Article |
series | Nature Communications |
spelling | doaj.art-6b0dab175ca04375aefa407478f3240a2022-12-21T20:38:49ZengNature PortfolioNature Communications2041-17232019-10-011011810.1038/s41467-019-12830-1Two-dimensional electronic spectroscopy reveals liquid-like lineshape dynamics in CsPbI3 perovskite nanocrystalsHélène Seiler0Samuel Palato1Colin Sonnichsen2Harry Baker3Etienne Socie4Dallas P. Strandell5Patanjali Kambhampati6Department of Chemistry, McGill UniversityDepartment of Chemistry, McGill UniversityDepartment of Chemistry, McGill UniversityDepartment of Chemistry, McGill UniversityDepartment of Chemistry, McGill UniversityDepartment of Chemistry, McGill UniversityDepartment of Chemistry, McGill UniversityLead-halide perovskites have promising optoelectronic properties, determined by interplay of electronic and structural properties. Here the authors probe CsPbI3 nanocrystals by two-dimensional electronic spectroscopy, showing liquid-like structural dynamics signature of polaron formation.https://doi.org/10.1038/s41467-019-12830-1 |
spellingShingle | Hélène Seiler Samuel Palato Colin Sonnichsen Harry Baker Etienne Socie Dallas P. Strandell Patanjali Kambhampati Two-dimensional electronic spectroscopy reveals liquid-like lineshape dynamics in CsPbI3 perovskite nanocrystals Nature Communications |
title | Two-dimensional electronic spectroscopy reveals liquid-like lineshape dynamics in CsPbI3 perovskite nanocrystals |
title_full | Two-dimensional electronic spectroscopy reveals liquid-like lineshape dynamics in CsPbI3 perovskite nanocrystals |
title_fullStr | Two-dimensional electronic spectroscopy reveals liquid-like lineshape dynamics in CsPbI3 perovskite nanocrystals |
title_full_unstemmed | Two-dimensional electronic spectroscopy reveals liquid-like lineshape dynamics in CsPbI3 perovskite nanocrystals |
title_short | Two-dimensional electronic spectroscopy reveals liquid-like lineshape dynamics in CsPbI3 perovskite nanocrystals |
title_sort | two dimensional electronic spectroscopy reveals liquid like lineshape dynamics in cspbi3 perovskite nanocrystals |
url | https://doi.org/10.1038/s41467-019-12830-1 |
work_keys_str_mv | AT heleneseiler twodimensionalelectronicspectroscopyrevealsliquidlikelineshapedynamicsincspbi3perovskitenanocrystals AT samuelpalato twodimensionalelectronicspectroscopyrevealsliquidlikelineshapedynamicsincspbi3perovskitenanocrystals AT colinsonnichsen twodimensionalelectronicspectroscopyrevealsliquidlikelineshapedynamicsincspbi3perovskitenanocrystals AT harrybaker twodimensionalelectronicspectroscopyrevealsliquidlikelineshapedynamicsincspbi3perovskitenanocrystals AT etiennesocie twodimensionalelectronicspectroscopyrevealsliquidlikelineshapedynamicsincspbi3perovskitenanocrystals AT dallaspstrandell twodimensionalelectronicspectroscopyrevealsliquidlikelineshapedynamicsincspbi3perovskitenanocrystals AT patanjalikambhampati twodimensionalelectronicspectroscopyrevealsliquidlikelineshapedynamicsincspbi3perovskitenanocrystals |