Integrated electrocatalysts derived from metal organic frameworks for gas-involved reactions
Integrated electrocatalysts (IECs) containing well-defined functional materials directly grown on the current collector have sparked increasing interest in the fields of electrocatalysis owing to efficient activity, high stability and the fact that they are easily assembled into devices. Recently, m...
| Main Authors: | , , , |
|---|---|
| Format: | Article |
| Language: | English |
| Published: |
KeAi Communications Co., Ltd.
2023-06-01
|
| Series: | Nano Materials Science |
| Subjects: | |
| Online Access: | http://www.sciencedirect.com/science/article/pii/S2589965122000034 |
| _version_ | 1797783593212182528 |
|---|---|
| author | Yuke Song Wenfu Xie Mingfei Shao Xue Duan |
| author_facet | Yuke Song Wenfu Xie Mingfei Shao Xue Duan |
| author_sort | Yuke Song |
| collection | DOAJ |
| description | Integrated electrocatalysts (IECs) containing well-defined functional materials directly grown on the current collector have sparked increasing interest in the fields of electrocatalysis owing to efficient activity, high stability and the fact that they are easily assembled into devices. Recently, metal organic frameworks (MOFs) provide a promising platform for constructing advanced IECs because of their properties of low cost, large surface area and efficient structural tunability. In this review, the design principles of state-of-the-art IECs based on MOFs are presented, including by hydrothermal/solvothermal, template-directed, electrospinning, electrodeposition and other methods. The high performance of MOF-derived IECs has also been demonstrated in electrocatalytic gas-involved reactions. This is promising for green energy storage and conversion. The structure-activity relationship and performance improvement mechanism of IECs are uncovered by discussing some in situ technologies for IECs. Finally, we provide an outlook on the challenges and prospects in this booming field. |
| first_indexed | 2024-03-13T00:28:05Z |
| format | Article |
| id | doaj.art-6b1050de6f714a7fbcbcdf32b1ba4585 |
| institution | Directory Open Access Journal |
| issn | 2589-9651 |
| language | English |
| last_indexed | 2024-03-13T00:28:05Z |
| publishDate | 2023-06-01 |
| publisher | KeAi Communications Co., Ltd. |
| record_format | Article |
| series | Nano Materials Science |
| spelling | doaj.art-6b1050de6f714a7fbcbcdf32b1ba45852023-07-11T04:06:38ZengKeAi Communications Co., Ltd.Nano Materials Science2589-96512023-06-0152161176Integrated electrocatalysts derived from metal organic frameworks for gas-involved reactionsYuke Song0Wenfu Xie1Mingfei Shao2Xue Duan3State Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical Technology, Beijing, 100029, ChinaCorresponding author. State Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical Technology, Beijing, 100029, China.; State Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical Technology, Beijing, 100029, ChinaCorresponding author. State Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical Technology, Beijing, 100029, China.; State Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical Technology, Beijing, 100029, ChinaState Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical Technology, Beijing, 100029, ChinaIntegrated electrocatalysts (IECs) containing well-defined functional materials directly grown on the current collector have sparked increasing interest in the fields of electrocatalysis owing to efficient activity, high stability and the fact that they are easily assembled into devices. Recently, metal organic frameworks (MOFs) provide a promising platform for constructing advanced IECs because of their properties of low cost, large surface area and efficient structural tunability. In this review, the design principles of state-of-the-art IECs based on MOFs are presented, including by hydrothermal/solvothermal, template-directed, electrospinning, electrodeposition and other methods. The high performance of MOF-derived IECs has also been demonstrated in electrocatalytic gas-involved reactions. This is promising for green energy storage and conversion. The structure-activity relationship and performance improvement mechanism of IECs are uncovered by discussing some in situ technologies for IECs. Finally, we provide an outlook on the challenges and prospects in this booming field.http://www.sciencedirect.com/science/article/pii/S2589965122000034Integrated electrocatalystMetal organic frameworkStructure-activity relationshipGas-involved reaction |
| spellingShingle | Yuke Song Wenfu Xie Mingfei Shao Xue Duan Integrated electrocatalysts derived from metal organic frameworks for gas-involved reactions Nano Materials Science Integrated electrocatalyst Metal organic framework Structure-activity relationship Gas-involved reaction |
| title | Integrated electrocatalysts derived from metal organic frameworks for gas-involved reactions |
| title_full | Integrated electrocatalysts derived from metal organic frameworks for gas-involved reactions |
| title_fullStr | Integrated electrocatalysts derived from metal organic frameworks for gas-involved reactions |
| title_full_unstemmed | Integrated electrocatalysts derived from metal organic frameworks for gas-involved reactions |
| title_short | Integrated electrocatalysts derived from metal organic frameworks for gas-involved reactions |
| title_sort | integrated electrocatalysts derived from metal organic frameworks for gas involved reactions |
| topic | Integrated electrocatalyst Metal organic framework Structure-activity relationship Gas-involved reaction |
| url | http://www.sciencedirect.com/science/article/pii/S2589965122000034 |
| work_keys_str_mv | AT yukesong integratedelectrocatalystsderivedfrommetalorganicframeworksforgasinvolvedreactions AT wenfuxie integratedelectrocatalystsderivedfrommetalorganicframeworksforgasinvolvedreactions AT mingfeishao integratedelectrocatalystsderivedfrommetalorganicframeworksforgasinvolvedreactions AT xueduan integratedelectrocatalystsderivedfrommetalorganicframeworksforgasinvolvedreactions |