Extreme fast charging of commercial Li-ion batteries via combined thermal switching and self-heating approaches

Abstract The mass adoption of electric vehicles is hindered by the inadequate extreme fast charging (XFC) performance (i.e., less than 15 min charging time to reach 80% state of charge) of commercial high-specific-energy (i.e., >200 Wh/kg) lithium-ion batteries (LIBs). Here, to enable the XFC of...

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Main Authors: Yuqiang Zeng, Buyi Zhang, Yanbao Fu, Fengyu Shen, Qiye Zheng, Divya Chalise, Ruijiao Miao, Sumanjeet Kaur, Sean D. Lubner, Michael C. Tucker, Vincent Battaglia, Chris Dames, Ravi S. Prasher
Format: Article
Language:English
Published: Nature Portfolio 2023-06-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-023-38823-9
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author Yuqiang Zeng
Buyi Zhang
Yanbao Fu
Fengyu Shen
Qiye Zheng
Divya Chalise
Ruijiao Miao
Sumanjeet Kaur
Sean D. Lubner
Michael C. Tucker
Vincent Battaglia
Chris Dames
Ravi S. Prasher
author_facet Yuqiang Zeng
Buyi Zhang
Yanbao Fu
Fengyu Shen
Qiye Zheng
Divya Chalise
Ruijiao Miao
Sumanjeet Kaur
Sean D. Lubner
Michael C. Tucker
Vincent Battaglia
Chris Dames
Ravi S. Prasher
author_sort Yuqiang Zeng
collection DOAJ
description Abstract The mass adoption of electric vehicles is hindered by the inadequate extreme fast charging (XFC) performance (i.e., less than 15 min charging time to reach 80% state of charge) of commercial high-specific-energy (i.e., >200 Wh/kg) lithium-ion batteries (LIBs). Here, to enable the XFC of commercial LIBs, we propose the regulation of the battery’s self-generated heat via active thermal switching. We demonstrate that retaining the heat during XFC with the switch OFF boosts the cell’s kinetics while dissipating the heat after XFC with the switch ON reduces detrimental reactions in the battery. Without modifying cell materials or structures, the proposed XFC approach enables reliable battery operation by applying <15 min of charge and 1 h of discharge. These results are almost identical regarding operativity for the same battery type tested applying a 1 h of charge and 1 h of discharge, thus, meeting the XFC targets set by the United States Department of Energy. Finally, we also demonstrate the feasibility of integrating the XFC approach in a commercial battery thermal management system.
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spelling doaj.art-6c51fffee77745ddae55816c631f32602023-06-04T11:32:41ZengNature PortfolioNature Communications2041-17232023-06-011411910.1038/s41467-023-38823-9Extreme fast charging of commercial Li-ion batteries via combined thermal switching and self-heating approachesYuqiang Zeng0Buyi Zhang1Yanbao Fu2Fengyu Shen3Qiye Zheng4Divya Chalise5Ruijiao Miao6Sumanjeet Kaur7Sean D. Lubner8Michael C. Tucker9Vincent Battaglia10Chris Dames11Ravi S. Prasher12Energy Storage and Distributed Resources Division, Lawrence Berkeley National LaboratoryEnergy Storage and Distributed Resources Division, Lawrence Berkeley National LaboratoryEnergy Storage and Distributed Resources Division, Lawrence Berkeley National LaboratoryEnergy Storage and Distributed Resources Division, Lawrence Berkeley National LaboratoryEnergy Storage and Distributed Resources Division, Lawrence Berkeley National LaboratoryEnergy Storage and Distributed Resources Division, Lawrence Berkeley National LaboratoryEnergy Storage and Distributed Resources Division, Lawrence Berkeley National LaboratoryEnergy Storage and Distributed Resources Division, Lawrence Berkeley National LaboratoryEnergy Storage and Distributed Resources Division, Lawrence Berkeley National LaboratoryEnergy Storage and Distributed Resources Division, Lawrence Berkeley National LaboratoryEnergy Storage and Distributed Resources Division, Lawrence Berkeley National LaboratoryEnergy Storage and Distributed Resources Division, Lawrence Berkeley National LaboratoryEnergy Storage and Distributed Resources Division, Lawrence Berkeley National LaboratoryAbstract The mass adoption of electric vehicles is hindered by the inadequate extreme fast charging (XFC) performance (i.e., less than 15 min charging time to reach 80% state of charge) of commercial high-specific-energy (i.e., >200 Wh/kg) lithium-ion batteries (LIBs). Here, to enable the XFC of commercial LIBs, we propose the regulation of the battery’s self-generated heat via active thermal switching. We demonstrate that retaining the heat during XFC with the switch OFF boosts the cell’s kinetics while dissipating the heat after XFC with the switch ON reduces detrimental reactions in the battery. Without modifying cell materials or structures, the proposed XFC approach enables reliable battery operation by applying <15 min of charge and 1 h of discharge. These results are almost identical regarding operativity for the same battery type tested applying a 1 h of charge and 1 h of discharge, thus, meeting the XFC targets set by the United States Department of Energy. Finally, we also demonstrate the feasibility of integrating the XFC approach in a commercial battery thermal management system.https://doi.org/10.1038/s41467-023-38823-9
spellingShingle Yuqiang Zeng
Buyi Zhang
Yanbao Fu
Fengyu Shen
Qiye Zheng
Divya Chalise
Ruijiao Miao
Sumanjeet Kaur
Sean D. Lubner
Michael C. Tucker
Vincent Battaglia
Chris Dames
Ravi S. Prasher
Extreme fast charging of commercial Li-ion batteries via combined thermal switching and self-heating approaches
Nature Communications
title Extreme fast charging of commercial Li-ion batteries via combined thermal switching and self-heating approaches
title_full Extreme fast charging of commercial Li-ion batteries via combined thermal switching and self-heating approaches
title_fullStr Extreme fast charging of commercial Li-ion batteries via combined thermal switching and self-heating approaches
title_full_unstemmed Extreme fast charging of commercial Li-ion batteries via combined thermal switching and self-heating approaches
title_short Extreme fast charging of commercial Li-ion batteries via combined thermal switching and self-heating approaches
title_sort extreme fast charging of commercial li ion batteries via combined thermal switching and self heating approaches
url https://doi.org/10.1038/s41467-023-38823-9
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