An Evaluation of Radon in Drinking Water Supplies in Major Cities of the Province of Chimborazo, Central Andes of Ecuador

The activity concentrations of <sup>222</sup>Rn were measured in 53 public water supplies of underground (50) and surface (3) origin, and the relation of such with five geological units where these supplies are located, in the central Ecuadorian Andes, was also explored. These units supp...

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Main Authors: Jheny Orbe, José Luis Herrera-Robalino, Gabriela Ureña-Callay, Jonatan Telenchano-Ilbay, Shirley Samaniego-León, Augusto Fienco-Bacusoy, Andrea Cando-Veintimilla, Theofilos Toulkeridis
Format: Article
Language:English
Published: MDPI AG 2023-06-01
Series:Water
Subjects:
Online Access:https://www.mdpi.com/2073-4441/15/12/2255
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author Jheny Orbe
José Luis Herrera-Robalino
Gabriela Ureña-Callay
Jonatan Telenchano-Ilbay
Shirley Samaniego-León
Augusto Fienco-Bacusoy
Andrea Cando-Veintimilla
Theofilos Toulkeridis
author_facet Jheny Orbe
José Luis Herrera-Robalino
Gabriela Ureña-Callay
Jonatan Telenchano-Ilbay
Shirley Samaniego-León
Augusto Fienco-Bacusoy
Andrea Cando-Veintimilla
Theofilos Toulkeridis
author_sort Jheny Orbe
collection DOAJ
description The activity concentrations of <sup>222</sup>Rn were measured in 53 public water supplies of underground (50) and surface (3) origin, and the relation of such with five geological units where these supplies are located, in the central Ecuadorian Andes, was also explored. These units supply drinking water to 10 cities, located between the 1500 and 3120 m.a.s.l. The experimental setup consisted of the RAD7 radon detector and the RAD H<sub>2</sub>O degassing system. The <sup>222</sup>Rn levels measured in groundwater ranged from 0.53 to 14.78 Bq/L while surface waters did not indicate detectable radon levels. The radon concentrations were below the parametric value of 100 Bq/L for water intended for human consumption, recommended by the European Atomic Energy Community (EURATOM) in its Directive 2013/51, and the alternative maximum contamination level (AMCL) of 150 Bq/L, proposed by the Environmental Protection Agency (EPA). The Pisayambo Volcanic unit, mapped as intermediate volcaniclastic to felsic deposits, presented a mean radon concentration higher than the other geological units and lithologies (9.58 ± 3.04 Bq/L). The Cunupogyo well (11.36 ± 0.48 Bq/L) presented a radon concentration more than 70% higher than the neighboring springs, which may be explained by its proximity to the Pallatanga geological fault. The maximum annual effective doses, by cities, due to the ingestion and inhalation of radon, ranged from 0.010 to 0.108 mSv and from 0.008 to 0.091 mSv, respectively; therefore, these waters do not represent a risk to the health of the population. In addition, a correlation was observed between the activity concentration of <sup>222</sup>Rn and the activity concentration of the parent <sup>226</sup>Ra in samples collected from some springs.
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spelling doaj.art-6d7b0acee35b43fdb2f4dad643e7dba92023-11-18T13:05:28ZengMDPI AGWater2073-44412023-06-011512225510.3390/w15122255An Evaluation of Radon in Drinking Water Supplies in Major Cities of the Province of Chimborazo, Central Andes of EcuadorJheny Orbe0José Luis Herrera-Robalino1Gabriela Ureña-Callay2Jonatan Telenchano-Ilbay3Shirley Samaniego-León4Augusto Fienco-Bacusoy5Andrea Cando-Veintimilla6Theofilos Toulkeridis7Escuela Superior Politécnica de Chimborazo (ESPOCH), Riobamba 060101, EcuadorEscuela Superior Politécnica de Chimborazo (ESPOCH), Riobamba 060101, EcuadorEscuela Superior Politécnica de Chimborazo (ESPOCH), Riobamba 060101, EcuadorCentro de Imagen Castro Sanchez Cindy Mireya, Riobamba 060110, EcuadorColegio de Bachillerato Bernardo Dávalos León, Riobamba 060104, EcuadorUnidad Educativa República del Ecuador, Jipijapa 130301, EcuadorUniversidad de Alicante, 03690 Alicante, SpainUniversidad de las Fuerzas Armadas ESPE, Av. General Rumiñahui S/N, Sangolquí 171103, EcuadorThe activity concentrations of <sup>222</sup>Rn were measured in 53 public water supplies of underground (50) and surface (3) origin, and the relation of such with five geological units where these supplies are located, in the central Ecuadorian Andes, was also explored. These units supply drinking water to 10 cities, located between the 1500 and 3120 m.a.s.l. The experimental setup consisted of the RAD7 radon detector and the RAD H<sub>2</sub>O degassing system. The <sup>222</sup>Rn levels measured in groundwater ranged from 0.53 to 14.78 Bq/L while surface waters did not indicate detectable radon levels. The radon concentrations were below the parametric value of 100 Bq/L for water intended for human consumption, recommended by the European Atomic Energy Community (EURATOM) in its Directive 2013/51, and the alternative maximum contamination level (AMCL) of 150 Bq/L, proposed by the Environmental Protection Agency (EPA). The Pisayambo Volcanic unit, mapped as intermediate volcaniclastic to felsic deposits, presented a mean radon concentration higher than the other geological units and lithologies (9.58 ± 3.04 Bq/L). The Cunupogyo well (11.36 ± 0.48 Bq/L) presented a radon concentration more than 70% higher than the neighboring springs, which may be explained by its proximity to the Pallatanga geological fault. The maximum annual effective doses, by cities, due to the ingestion and inhalation of radon, ranged from 0.010 to 0.108 mSv and from 0.008 to 0.091 mSv, respectively; therefore, these waters do not represent a risk to the health of the population. In addition, a correlation was observed between the activity concentration of <sup>222</sup>Rn and the activity concentration of the parent <sup>226</sup>Ra in samples collected from some springs.https://www.mdpi.com/2073-4441/15/12/2255<sup>222</sup>Ra<sup>226</sup>Raspring waterannual effective dosesdrinking waterEcuador
spellingShingle Jheny Orbe
José Luis Herrera-Robalino
Gabriela Ureña-Callay
Jonatan Telenchano-Ilbay
Shirley Samaniego-León
Augusto Fienco-Bacusoy
Andrea Cando-Veintimilla
Theofilos Toulkeridis
An Evaluation of Radon in Drinking Water Supplies in Major Cities of the Province of Chimborazo, Central Andes of Ecuador
Water
<sup>222</sup>Ra
<sup>226</sup>Ra
spring water
annual effective doses
drinking water
Ecuador
title An Evaluation of Radon in Drinking Water Supplies in Major Cities of the Province of Chimborazo, Central Andes of Ecuador
title_full An Evaluation of Radon in Drinking Water Supplies in Major Cities of the Province of Chimborazo, Central Andes of Ecuador
title_fullStr An Evaluation of Radon in Drinking Water Supplies in Major Cities of the Province of Chimborazo, Central Andes of Ecuador
title_full_unstemmed An Evaluation of Radon in Drinking Water Supplies in Major Cities of the Province of Chimborazo, Central Andes of Ecuador
title_short An Evaluation of Radon in Drinking Water Supplies in Major Cities of the Province of Chimborazo, Central Andes of Ecuador
title_sort evaluation of radon in drinking water supplies in major cities of the province of chimborazo central andes of ecuador
topic <sup>222</sup>Ra
<sup>226</sup>Ra
spring water
annual effective doses
drinking water
Ecuador
url https://www.mdpi.com/2073-4441/15/12/2255
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