Spin excitations and correlations in scanning tunneling spectroscopy

In recent years inelastic spin-flip spectroscopy using a low-temperature scanning tunneling microscope has been a very successful tool for studying not only individual spins but also complex coupled systems. When these systems interact with the electrons of the supporting substrate correlated many-p...

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Main Author: Markus Ternes
Format: Article
Language:English
Published: IOP Publishing 2015-01-01
Series:New Journal of Physics
Subjects:
Online Access:https://doi.org/10.1088/1367-2630/17/6/063016
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author Markus Ternes
author_facet Markus Ternes
author_sort Markus Ternes
collection DOAJ
description In recent years inelastic spin-flip spectroscopy using a low-temperature scanning tunneling microscope has been a very successful tool for studying not only individual spins but also complex coupled systems. When these systems interact with the electrons of the supporting substrate correlated many-particle states can emerge, making them ideal prototypical quantum systems. The spin systems, which can be constructed by arranging individual atoms on appropriate surfaces or embedded in synthesized molecular structures, can reveal very rich spectral features. Up to now the spectral complexity has only been partly described. This manuscript shows that perturbation theory enables one to describe the tunneling transport, reproducing the differential conductance with surprisingly high accuracy. Well established scattering models, which include Kondo-like spin–spin and potential interactions, are expanded to enable calculation of arbitrary complex spin systems in reasonable time scale and the extraction of important physical properties. The emergence of correlations between spins and, in particular, between the localized spins and the supporting bath electrons are discussed and related to experimentally tunable parameters. These results might stimulate new experiments by providing experimentalists with an easily applicable modeling tool.
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spelling doaj.art-6e08623473244d2c951b17e1913363f22023-08-08T14:18:26ZengIOP PublishingNew Journal of Physics1367-26302015-01-0117606301610.1088/1367-2630/17/6/063016Spin excitations and correlations in scanning tunneling spectroscopyMarkus Ternes0Max-Planck Institute for Solid State Research, Heisenbergstr. 1, D-70569 Stuttgart, GermanyIn recent years inelastic spin-flip spectroscopy using a low-temperature scanning tunneling microscope has been a very successful tool for studying not only individual spins but also complex coupled systems. When these systems interact with the electrons of the supporting substrate correlated many-particle states can emerge, making them ideal prototypical quantum systems. The spin systems, which can be constructed by arranging individual atoms on appropriate surfaces or embedded in synthesized molecular structures, can reveal very rich spectral features. Up to now the spectral complexity has only been partly described. This manuscript shows that perturbation theory enables one to describe the tunneling transport, reproducing the differential conductance with surprisingly high accuracy. Well established scattering models, which include Kondo-like spin–spin and potential interactions, are expanded to enable calculation of arbitrary complex spin systems in reasonable time scale and the extraction of important physical properties. The emergence of correlations between spins and, in particular, between the localized spins and the supporting bath electrons are discussed and related to experimentally tunable parameters. These results might stimulate new experiments by providing experimentalists with an easily applicable modeling tool.https://doi.org/10.1088/1367-2630/17/6/063016spin excitationsspin-flip spectroscopyKondo effectcorrelations68.37.Ef72.15.Qm
spellingShingle Markus Ternes
Spin excitations and correlations in scanning tunneling spectroscopy
New Journal of Physics
spin excitations
spin-flip spectroscopy
Kondo effect
correlations
68.37.Ef
72.15.Qm
title Spin excitations and correlations in scanning tunneling spectroscopy
title_full Spin excitations and correlations in scanning tunneling spectroscopy
title_fullStr Spin excitations and correlations in scanning tunneling spectroscopy
title_full_unstemmed Spin excitations and correlations in scanning tunneling spectroscopy
title_short Spin excitations and correlations in scanning tunneling spectroscopy
title_sort spin excitations and correlations in scanning tunneling spectroscopy
topic spin excitations
spin-flip spectroscopy
Kondo effect
correlations
68.37.Ef
72.15.Qm
url https://doi.org/10.1088/1367-2630/17/6/063016
work_keys_str_mv AT markusternes spinexcitationsandcorrelationsinscanningtunnelingspectroscopy