Analysis of the Process of Mineral Sequestration of CO<sub>2</sub> with the Use of Fluidised Bed Combustion (FBC) Fly Ashes

There is a current focus on replacing the generally accepted conventional power generation technologies with more advanced ones that will better protect the natural environment. The need to limit CO<sub>2</sub> emissions from power generation plants presents a problem that must be solved...

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Main Authors: Alicja Uliasz-Bocheńczyk, Eugeniusz Mokrzycki
Format: Article
Language:English
Published: MDPI AG 2021-06-01
Series:Minerals
Subjects:
Online Access:https://www.mdpi.com/2075-163X/11/7/676
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author Alicja Uliasz-Bocheńczyk
Eugeniusz Mokrzycki
author_facet Alicja Uliasz-Bocheńczyk
Eugeniusz Mokrzycki
author_sort Alicja Uliasz-Bocheńczyk
collection DOAJ
description There is a current focus on replacing the generally accepted conventional power generation technologies with more advanced ones that will better protect the natural environment. The need to limit CO<sub>2</sub> emissions from power generation plants presents a problem that must be solved in many countries that use coal or lignite as basic fuels. One potential option is mineral sequestration performed using side products of fossil fuel combustion, such as fluidised bed combustion (FBC) fly ashes. Fluidised bed combustion (FBC) lignite fly ashes are characterised by a high storage capacity of 15.7%. Research conducted with the most commonly used method of direct mineral sequestration—CO<sub>2</sub> trapping with fluidised bed combustion (FBC) ash in water suspension—has indicated a very high level of carbonation of CO<sub>2</sub>, reaching 11%. Calcite was the basic product of carbonation. The calcite content increased from 2% to 12% in the suspension subjected to treatment with CO<sub>2</sub>. Furthermore, CO<sub>2</sub> reduced the pH and limited the leaching of impurities, such as Zn, Cu, Pb, Ni, As, Hg, Cd, Cr, Cl, and SO<sub>4</sub>. The fly ash suspensions subjected to CO<sub>2</sub> treatment can be used in industry in the final stage of carbon capture and utilisation (CCU) technology, which will further contribute to the implementation of the circular economy.
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spelling doaj.art-6f2284fa406a46678b9057dba57feb922023-12-03T13:07:32ZengMDPI AGMinerals2075-163X2021-06-0111767610.3390/min11070676Analysis of the Process of Mineral Sequestration of CO<sub>2</sub> with the Use of Fluidised Bed Combustion (FBC) Fly AshesAlicja Uliasz-Bocheńczyk0Eugeniusz Mokrzycki1Faculty of Civil Engineering and Resource Management, AGH University of Science and Technology, Mickiewicza 30, 30-059 Krakow, PolandMineral and Energy Economy Research Institute of the Polish Academy of Sciences, Wybickiego 7A, 31-261 Krakow, PolandThere is a current focus on replacing the generally accepted conventional power generation technologies with more advanced ones that will better protect the natural environment. The need to limit CO<sub>2</sub> emissions from power generation plants presents a problem that must be solved in many countries that use coal or lignite as basic fuels. One potential option is mineral sequestration performed using side products of fossil fuel combustion, such as fluidised bed combustion (FBC) fly ashes. Fluidised bed combustion (FBC) lignite fly ashes are characterised by a high storage capacity of 15.7%. Research conducted with the most commonly used method of direct mineral sequestration—CO<sub>2</sub> trapping with fluidised bed combustion (FBC) ash in water suspension—has indicated a very high level of carbonation of CO<sub>2</sub>, reaching 11%. Calcite was the basic product of carbonation. The calcite content increased from 2% to 12% in the suspension subjected to treatment with CO<sub>2</sub>. Furthermore, CO<sub>2</sub> reduced the pH and limited the leaching of impurities, such as Zn, Cu, Pb, Ni, As, Hg, Cd, Cr, Cl, and SO<sub>4</sub>. The fly ash suspensions subjected to CO<sub>2</sub> treatment can be used in industry in the final stage of carbon capture and utilisation (CCU) technology, which will further contribute to the implementation of the circular economy.https://www.mdpi.com/2075-163X/11/7/676fluidised bed combustion (FBC) fly ashmineral sequestrationCO<sub>2</sub>direct processlignite combustion
spellingShingle Alicja Uliasz-Bocheńczyk
Eugeniusz Mokrzycki
Analysis of the Process of Mineral Sequestration of CO<sub>2</sub> with the Use of Fluidised Bed Combustion (FBC) Fly Ashes
Minerals
fluidised bed combustion (FBC) fly ash
mineral sequestration
CO<sub>2</sub>
direct process
lignite combustion
title Analysis of the Process of Mineral Sequestration of CO<sub>2</sub> with the Use of Fluidised Bed Combustion (FBC) Fly Ashes
title_full Analysis of the Process of Mineral Sequestration of CO<sub>2</sub> with the Use of Fluidised Bed Combustion (FBC) Fly Ashes
title_fullStr Analysis of the Process of Mineral Sequestration of CO<sub>2</sub> with the Use of Fluidised Bed Combustion (FBC) Fly Ashes
title_full_unstemmed Analysis of the Process of Mineral Sequestration of CO<sub>2</sub> with the Use of Fluidised Bed Combustion (FBC) Fly Ashes
title_short Analysis of the Process of Mineral Sequestration of CO<sub>2</sub> with the Use of Fluidised Bed Combustion (FBC) Fly Ashes
title_sort analysis of the process of mineral sequestration of co sub 2 sub with the use of fluidised bed combustion fbc fly ashes
topic fluidised bed combustion (FBC) fly ash
mineral sequestration
CO<sub>2</sub>
direct process
lignite combustion
url https://www.mdpi.com/2075-163X/11/7/676
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