Analysis of the Process of Mineral Sequestration of CO<sub>2</sub> with the Use of Fluidised Bed Combustion (FBC) Fly Ashes
There is a current focus on replacing the generally accepted conventional power generation technologies with more advanced ones that will better protect the natural environment. The need to limit CO<sub>2</sub> emissions from power generation plants presents a problem that must be solved...
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MDPI AG
2021-06-01
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Series: | Minerals |
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Online Access: | https://www.mdpi.com/2075-163X/11/7/676 |
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author | Alicja Uliasz-Bocheńczyk Eugeniusz Mokrzycki |
author_facet | Alicja Uliasz-Bocheńczyk Eugeniusz Mokrzycki |
author_sort | Alicja Uliasz-Bocheńczyk |
collection | DOAJ |
description | There is a current focus on replacing the generally accepted conventional power generation technologies with more advanced ones that will better protect the natural environment. The need to limit CO<sub>2</sub> emissions from power generation plants presents a problem that must be solved in many countries that use coal or lignite as basic fuels. One potential option is mineral sequestration performed using side products of fossil fuel combustion, such as fluidised bed combustion (FBC) fly ashes. Fluidised bed combustion (FBC) lignite fly ashes are characterised by a high storage capacity of 15.7%. Research conducted with the most commonly used method of direct mineral sequestration—CO<sub>2</sub> trapping with fluidised bed combustion (FBC) ash in water suspension—has indicated a very high level of carbonation of CO<sub>2</sub>, reaching 11%. Calcite was the basic product of carbonation. The calcite content increased from 2% to 12% in the suspension subjected to treatment with CO<sub>2</sub>. Furthermore, CO<sub>2</sub> reduced the pH and limited the leaching of impurities, such as Zn, Cu, Pb, Ni, As, Hg, Cd, Cr, Cl, and SO<sub>4</sub>. The fly ash suspensions subjected to CO<sub>2</sub> treatment can be used in industry in the final stage of carbon capture and utilisation (CCU) technology, which will further contribute to the implementation of the circular economy. |
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format | Article |
id | doaj.art-6f2284fa406a46678b9057dba57feb92 |
institution | Directory Open Access Journal |
issn | 2075-163X |
language | English |
last_indexed | 2024-03-09T04:54:03Z |
publishDate | 2021-06-01 |
publisher | MDPI AG |
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series | Minerals |
spelling | doaj.art-6f2284fa406a46678b9057dba57feb922023-12-03T13:07:32ZengMDPI AGMinerals2075-163X2021-06-0111767610.3390/min11070676Analysis of the Process of Mineral Sequestration of CO<sub>2</sub> with the Use of Fluidised Bed Combustion (FBC) Fly AshesAlicja Uliasz-Bocheńczyk0Eugeniusz Mokrzycki1Faculty of Civil Engineering and Resource Management, AGH University of Science and Technology, Mickiewicza 30, 30-059 Krakow, PolandMineral and Energy Economy Research Institute of the Polish Academy of Sciences, Wybickiego 7A, 31-261 Krakow, PolandThere is a current focus on replacing the generally accepted conventional power generation technologies with more advanced ones that will better protect the natural environment. The need to limit CO<sub>2</sub> emissions from power generation plants presents a problem that must be solved in many countries that use coal or lignite as basic fuels. One potential option is mineral sequestration performed using side products of fossil fuel combustion, such as fluidised bed combustion (FBC) fly ashes. Fluidised bed combustion (FBC) lignite fly ashes are characterised by a high storage capacity of 15.7%. Research conducted with the most commonly used method of direct mineral sequestration—CO<sub>2</sub> trapping with fluidised bed combustion (FBC) ash in water suspension—has indicated a very high level of carbonation of CO<sub>2</sub>, reaching 11%. Calcite was the basic product of carbonation. The calcite content increased from 2% to 12% in the suspension subjected to treatment with CO<sub>2</sub>. Furthermore, CO<sub>2</sub> reduced the pH and limited the leaching of impurities, such as Zn, Cu, Pb, Ni, As, Hg, Cd, Cr, Cl, and SO<sub>4</sub>. The fly ash suspensions subjected to CO<sub>2</sub> treatment can be used in industry in the final stage of carbon capture and utilisation (CCU) technology, which will further contribute to the implementation of the circular economy.https://www.mdpi.com/2075-163X/11/7/676fluidised bed combustion (FBC) fly ashmineral sequestrationCO<sub>2</sub>direct processlignite combustion |
spellingShingle | Alicja Uliasz-Bocheńczyk Eugeniusz Mokrzycki Analysis of the Process of Mineral Sequestration of CO<sub>2</sub> with the Use of Fluidised Bed Combustion (FBC) Fly Ashes Minerals fluidised bed combustion (FBC) fly ash mineral sequestration CO<sub>2</sub> direct process lignite combustion |
title | Analysis of the Process of Mineral Sequestration of CO<sub>2</sub> with the Use of Fluidised Bed Combustion (FBC) Fly Ashes |
title_full | Analysis of the Process of Mineral Sequestration of CO<sub>2</sub> with the Use of Fluidised Bed Combustion (FBC) Fly Ashes |
title_fullStr | Analysis of the Process of Mineral Sequestration of CO<sub>2</sub> with the Use of Fluidised Bed Combustion (FBC) Fly Ashes |
title_full_unstemmed | Analysis of the Process of Mineral Sequestration of CO<sub>2</sub> with the Use of Fluidised Bed Combustion (FBC) Fly Ashes |
title_short | Analysis of the Process of Mineral Sequestration of CO<sub>2</sub> with the Use of Fluidised Bed Combustion (FBC) Fly Ashes |
title_sort | analysis of the process of mineral sequestration of co sub 2 sub with the use of fluidised bed combustion fbc fly ashes |
topic | fluidised bed combustion (FBC) fly ash mineral sequestration CO<sub>2</sub> direct process lignite combustion |
url | https://www.mdpi.com/2075-163X/11/7/676 |
work_keys_str_mv | AT alicjauliaszbochenczyk analysisoftheprocessofmineralsequestrationofcosub2subwiththeuseoffluidisedbedcombustionfbcflyashes AT eugeniuszmokrzycki analysisoftheprocessofmineralsequestrationofcosub2subwiththeuseoffluidisedbedcombustionfbcflyashes |