Dynamic Modelling of CO<sub>2</sub> Capture by Calcium-Looping Cycle

Carbon capture and storage (CCS) technologies are mitigation measures aimed to reduce CO2 emissions from energy and other energy-intensive sectors. Among various CCS technologies, chemical looping systems are considered as potential promising solutions to reduce CO2 capture energy penalty. The paper...

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Main Authors: A.M. Cormos, A. Simon
Format: Article
Language:English
Published: AIDIC Servizi S.r.l. 2013-09-01
Series:Chemical Engineering Transactions
Online Access:https://www.cetjournal.it/index.php/cet/article/view/6019
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author A.M. Cormos
A. Simon
author_facet A.M. Cormos
A. Simon
author_sort A.M. Cormos
collection DOAJ
description Carbon capture and storage (CCS) technologies are mitigation measures aimed to reduce CO2 emissions from energy and other energy-intensive sectors. Among various CCS technologies, chemical looping systems are considered as potential promising solutions to reduce CO2 capture energy penalty. The paper presents a dynamic mathematical model of carbonation and calcination reactors of calcium-looping process to be used for carbon capture in fossil fuel-based power plants. The model described the particle distribution in carbonator / calciner according a 1D model for fast fluidization presented by Kunii and Levenspiel. The CO2 adsorption efficiency in the carbonator is divided in two terms taking into account the dense and lean regions of the bed. The dynamic model evaluates the solid distribution gas velocity and particle diameter and predicts the overall CO2 capture efficiency, taking into account that in every carbonation-calcination cycle the sorbent capacity decreases with the number of cycles.
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spelling doaj.art-7077a0dad0e04e449dd903f3fafa27772022-12-21T23:06:10ZengAIDIC Servizi S.r.l.Chemical Engineering Transactions2283-92162013-09-013510.3303/CET1335070Dynamic Modelling of CO<sub>2</sub> Capture by Calcium-Looping CycleA.M. CormosA. SimonCarbon capture and storage (CCS) technologies are mitigation measures aimed to reduce CO2 emissions from energy and other energy-intensive sectors. Among various CCS technologies, chemical looping systems are considered as potential promising solutions to reduce CO2 capture energy penalty. The paper presents a dynamic mathematical model of carbonation and calcination reactors of calcium-looping process to be used for carbon capture in fossil fuel-based power plants. The model described the particle distribution in carbonator / calciner according a 1D model for fast fluidization presented by Kunii and Levenspiel. The CO2 adsorption efficiency in the carbonator is divided in two terms taking into account the dense and lean regions of the bed. The dynamic model evaluates the solid distribution gas velocity and particle diameter and predicts the overall CO2 capture efficiency, taking into account that in every carbonation-calcination cycle the sorbent capacity decreases with the number of cycles.https://www.cetjournal.it/index.php/cet/article/view/6019
spellingShingle A.M. Cormos
A. Simon
Dynamic Modelling of CO<sub>2</sub> Capture by Calcium-Looping Cycle
Chemical Engineering Transactions
title Dynamic Modelling of CO<sub>2</sub> Capture by Calcium-Looping Cycle
title_full Dynamic Modelling of CO<sub>2</sub> Capture by Calcium-Looping Cycle
title_fullStr Dynamic Modelling of CO<sub>2</sub> Capture by Calcium-Looping Cycle
title_full_unstemmed Dynamic Modelling of CO<sub>2</sub> Capture by Calcium-Looping Cycle
title_short Dynamic Modelling of CO<sub>2</sub> Capture by Calcium-Looping Cycle
title_sort dynamic modelling of co sub 2 sub capture by calcium looping cycle
url https://www.cetjournal.it/index.php/cet/article/view/6019
work_keys_str_mv AT amcormos dynamicmodellingofcosub2subcapturebycalciumloopingcycle
AT asimon dynamicmodellingofcosub2subcapturebycalciumloopingcycle