Control of coherent extreme-ultraviolet emission around atomic potential through laser chirp

Substantial neutral atoms can tunnel to excited states in an intense laser field and subsequently generate coherent emission through free induction decay. We experimentally observe an enhanced coherent emission in the harmonic slightly below the threshold, which is consistent with the free induction...

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Main Authors: Chun Yang, Zhiyuan Lou, Fan Yang, Xiaochun Ge, Yinghui Zheng, Zhinan Zeng, Ruxin Li
Format: Article
Language:English
Published: Frontiers Media S.A. 2022-10-01
Series:Frontiers in Physics
Subjects:
Online Access:https://www.frontiersin.org/articles/10.3389/fphy.2022.990002/full
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author Chun Yang
Chun Yang
Zhiyuan Lou
Fan Yang
Xiaochun Ge
Yinghui Zheng
Zhinan Zeng
Ruxin Li
author_facet Chun Yang
Chun Yang
Zhiyuan Lou
Fan Yang
Xiaochun Ge
Yinghui Zheng
Zhinan Zeng
Ruxin Li
author_sort Chun Yang
collection DOAJ
description Substantial neutral atoms can tunnel to excited states in an intense laser field and subsequently generate coherent emission through free induction decay. We experimentally observe an enhanced coherent emission in the harmonic slightly below the threshold, which is consistent with the free induction decay of Rydberg states produced by the frustrated tunnelling ionization (FTI) process. We further find that the intensity of the coherent emission significantly depends on the chirp of laser pulses. The simulations based on the strong field approximation model show that laser chirp affects the probability that the returned electrons recombine to the Rydberg states. Our result shows that coherent emission can be controlled by laser chirp, which facilitates understanding the dynamics of the Rydberg atom and coupling mechanism between the below-threshold harmonics and atomic energy level. In addition, the coherent below-threshold FTI emission we observed has small divergence which is good for EUV light source applications.
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spelling doaj.art-707b4fe56e2746198173edddf95e61df2022-12-22T04:34:39ZengFrontiers Media S.A.Frontiers in Physics2296-424X2022-10-011010.3389/fphy.2022.990002990002Control of coherent extreme-ultraviolet emission around atomic potential through laser chirpChun Yang0Chun Yang1Zhiyuan Lou2Fan Yang3Xiaochun Ge4Yinghui Zheng5Zhinan Zeng6Ruxin Li7State Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai, ChinaCenter of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing, ChinaState Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai, ChinaState Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai, ChinaState Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai, ChinaState Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai, ChinaState Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai, ChinaState Key Laboratory of High Field Laser Physics, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai, ChinaSubstantial neutral atoms can tunnel to excited states in an intense laser field and subsequently generate coherent emission through free induction decay. We experimentally observe an enhanced coherent emission in the harmonic slightly below the threshold, which is consistent with the free induction decay of Rydberg states produced by the frustrated tunnelling ionization (FTI) process. We further find that the intensity of the coherent emission significantly depends on the chirp of laser pulses. The simulations based on the strong field approximation model show that laser chirp affects the probability that the returned electrons recombine to the Rydberg states. Our result shows that coherent emission can be controlled by laser chirp, which facilitates understanding the dynamics of the Rydberg atom and coupling mechanism between the below-threshold harmonics and atomic energy level. In addition, the coherent below-threshold FTI emission we observed has small divergence which is good for EUV light source applications.https://www.frontiersin.org/articles/10.3389/fphy.2022.990002/fullfrustrated tunnelling ionizationchirphigh-order harmonic generationRydberg statesionization potentialtime dependent Schrödinger equation
spellingShingle Chun Yang
Chun Yang
Zhiyuan Lou
Fan Yang
Xiaochun Ge
Yinghui Zheng
Zhinan Zeng
Ruxin Li
Control of coherent extreme-ultraviolet emission around atomic potential through laser chirp
Frontiers in Physics
frustrated tunnelling ionization
chirp
high-order harmonic generation
Rydberg states
ionization potential
time dependent Schrödinger equation
title Control of coherent extreme-ultraviolet emission around atomic potential through laser chirp
title_full Control of coherent extreme-ultraviolet emission around atomic potential through laser chirp
title_fullStr Control of coherent extreme-ultraviolet emission around atomic potential through laser chirp
title_full_unstemmed Control of coherent extreme-ultraviolet emission around atomic potential through laser chirp
title_short Control of coherent extreme-ultraviolet emission around atomic potential through laser chirp
title_sort control of coherent extreme ultraviolet emission around atomic potential through laser chirp
topic frustrated tunnelling ionization
chirp
high-order harmonic generation
Rydberg states
ionization potential
time dependent Schrödinger equation
url https://www.frontiersin.org/articles/10.3389/fphy.2022.990002/full
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