Environmental transmission electron microscopy study of hydrogen charging effect on a Cu-Zr metallic glass

Hydrogen induced plasticity has been found in metallic glasses; however, the underlying mechanism remains unclear. Herein, we studied a Cu-Zr metallic glass charged in a hydrogen atmosphere inside an environmental transmission electron microscope. Compression tests of hydrogen charged nanopillars sh...

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Main Authors: Lin Tian, Yue-Qing Yang, Tobias Meyer, Dominik Tönnies, Vladimir Roddatis, Hendrik Voigt, Xin-Ai Zhao, Zhang-Jie Wang, De-Gang Xie, Michael Seibt, Cynthia A. Volkert, Zhi-Wei Shan
Format: Article
Language:English
Published: Taylor & Francis Group 2020-12-01
Series:Materials Research Letters
Subjects:
Online Access:http://dx.doi.org/10.1080/21663831.2020.1791273
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author Lin Tian
Yue-Qing Yang
Tobias Meyer
Dominik Tönnies
Vladimir Roddatis
Hendrik Voigt
Xin-Ai Zhao
Zhang-Jie Wang
De-Gang Xie
Michael Seibt
Cynthia A. Volkert
Zhi-Wei Shan
author_facet Lin Tian
Yue-Qing Yang
Tobias Meyer
Dominik Tönnies
Vladimir Roddatis
Hendrik Voigt
Xin-Ai Zhao
Zhang-Jie Wang
De-Gang Xie
Michael Seibt
Cynthia A. Volkert
Zhi-Wei Shan
author_sort Lin Tian
collection DOAJ
description Hydrogen induced plasticity has been found in metallic glasses; however, the underlying mechanism remains unclear. Herein, we studied a Cu-Zr metallic glass charged in a hydrogen atmosphere inside an environmental transmission electron microscope. Compression tests of hydrogen charged nanopillars show more controllable deformation compared to uncharged ones. A variable resolution fluctuation electron microscopy study of the hydrogen charged samples reveals an increase in the correlation length of the medium-range order. Our results provide experimental evidence for hydrogen-induced heterogeneity and support the idea that increasing the degree of heterogeneity leads to multiple local shear events and suppresses catastrophic shear banding. IMPACT STATEMENT Direct evidence of an increase in the spatial correlation length of the medium-range order is found during hydrogen charging of a Cu-Zr metallic glass and leads to enhanced plastic deformation.
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spelling doaj.art-729c130a902048b1834634cb0e41e48b2022-12-21T20:20:50ZengTaylor & Francis GroupMaterials Research Letters2166-38312020-12-0181243944510.1080/21663831.2020.17912731791273Environmental transmission electron microscopy study of hydrogen charging effect on a Cu-Zr metallic glassLin Tian0Yue-Qing Yang1Tobias Meyer2Dominik Tönnies3Vladimir Roddatis4Hendrik Voigt5Xin-Ai Zhao6Zhang-Jie Wang7De-Gang Xie8Michael Seibt9Cynthia A. Volkert10Zhi-Wei Shan11Center for Advancing Materials Performance from the Nanoscale (CAMP-NANO) and Hysitron Applied Research Center in China (HARCC), State Key Laboratory for Mechanical Behavior of Materials, Xi’an Jiaotong UniversityCenter for Advancing Materials Performance from the Nanoscale (CAMP-NANO) and Hysitron Applied Research Center in China (HARCC), State Key Laboratory for Mechanical Behavior of Materials, Xi’an Jiaotong University4th Physical Institute – Solids and Nanostructures, University of GöttingenInstitute of Materials Physics, University of GöttingenInstitute of Materials Physics, University of Göttingen4th Physical Institute – Solids and Nanostructures, University of GöttingenCenter for Advancing Materials Performance from the Nanoscale (CAMP-NANO) and Hysitron Applied Research Center in China (HARCC), State Key Laboratory for Mechanical Behavior of Materials, Xi’an Jiaotong UniversityCenter for Advancing Materials Performance from the Nanoscale (CAMP-NANO) and Hysitron Applied Research Center in China (HARCC), State Key Laboratory for Mechanical Behavior of Materials, Xi’an Jiaotong UniversityCenter for Advancing Materials Performance from the Nanoscale (CAMP-NANO) and Hysitron Applied Research Center in China (HARCC), State Key Laboratory for Mechanical Behavior of Materials, Xi’an Jiaotong University4th Physical Institute – Solids and Nanostructures, University of GöttingenInstitute of Materials Physics, University of GöttingenCenter for Advancing Materials Performance from the Nanoscale (CAMP-NANO) and Hysitron Applied Research Center in China (HARCC), State Key Laboratory for Mechanical Behavior of Materials, Xi’an Jiaotong UniversityHydrogen induced plasticity has been found in metallic glasses; however, the underlying mechanism remains unclear. Herein, we studied a Cu-Zr metallic glass charged in a hydrogen atmosphere inside an environmental transmission electron microscope. Compression tests of hydrogen charged nanopillars show more controllable deformation compared to uncharged ones. A variable resolution fluctuation electron microscopy study of the hydrogen charged samples reveals an increase in the correlation length of the medium-range order. Our results provide experimental evidence for hydrogen-induced heterogeneity and support the idea that increasing the degree of heterogeneity leads to multiple local shear events and suppresses catastrophic shear banding. IMPACT STATEMENT Direct evidence of an increase in the spatial correlation length of the medium-range order is found during hydrogen charging of a Cu-Zr metallic glass and leads to enhanced plastic deformation.http://dx.doi.org/10.1080/21663831.2020.1791273correlation lengthhydrogenmetallic glassplasticityvariable resolution fluctuation electron microscopy
spellingShingle Lin Tian
Yue-Qing Yang
Tobias Meyer
Dominik Tönnies
Vladimir Roddatis
Hendrik Voigt
Xin-Ai Zhao
Zhang-Jie Wang
De-Gang Xie
Michael Seibt
Cynthia A. Volkert
Zhi-Wei Shan
Environmental transmission electron microscopy study of hydrogen charging effect on a Cu-Zr metallic glass
Materials Research Letters
correlation length
hydrogen
metallic glass
plasticity
variable resolution fluctuation electron microscopy
title Environmental transmission electron microscopy study of hydrogen charging effect on a Cu-Zr metallic glass
title_full Environmental transmission electron microscopy study of hydrogen charging effect on a Cu-Zr metallic glass
title_fullStr Environmental transmission electron microscopy study of hydrogen charging effect on a Cu-Zr metallic glass
title_full_unstemmed Environmental transmission electron microscopy study of hydrogen charging effect on a Cu-Zr metallic glass
title_short Environmental transmission electron microscopy study of hydrogen charging effect on a Cu-Zr metallic glass
title_sort environmental transmission electron microscopy study of hydrogen charging effect on a cu zr metallic glass
topic correlation length
hydrogen
metallic glass
plasticity
variable resolution fluctuation electron microscopy
url http://dx.doi.org/10.1080/21663831.2020.1791273
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