Inversion of the Complex Refractive Index of Au-Ag Alloy Nanospheres Based on the Contour Intersection Method

The contour intersection method is a new method used to invert the complex refractive index of small particles. Research has yet to be reported on using this method to invert the complex refractive index of nanoparticles. This paper reports the feasibility and reliability of the contour intersection...

Full description

Bibliographic Details
Main Authors: Long Cheng, Paerhatijiang Tuersun, Dengpan Ma, Dilishati Wumaier, Yixuan Li
Format: Article
Language:English
Published: MDPI AG 2023-04-01
Series:Materials
Subjects:
Online Access:https://www.mdpi.com/1996-1944/16/9/3291
_version_ 1797602308412932096
author Long Cheng
Paerhatijiang Tuersun
Dengpan Ma
Dilishati Wumaier
Yixuan Li
author_facet Long Cheng
Paerhatijiang Tuersun
Dengpan Ma
Dilishati Wumaier
Yixuan Li
author_sort Long Cheng
collection DOAJ
description The contour intersection method is a new method used to invert the complex refractive index of small particles. Research has yet to be reported on using this method to invert the complex refractive index of nanoparticles. This paper reports the feasibility and reliability of the contour intersection method in the inversion of the complex refractive index of nanoparticles using Au-Ag alloy nanospheres. The Mie theory and the size-dependent dielectric function are used to calculate the light scattering and absorption efficiency of Au-Ag alloy nanospheres corresponding to the complex refractive index. The complex refractive index of the particles is obtained by inversion with the contour intersection method. The backscattering efficiency constraint method is used to determine the unique solution when multiple valid solutions from the contour intersection method appear. The effects of the Au component percentage, particle size, and measurement errors on the inversion results are quantitatively analyzed. Finally, the inversion accuracy is compared and analyzed with the traditional iterative method. The results show that as long as the light scattering efficiency, light absorption efficiency, and backscattering efficiency of Au nanospheres can be measured, the accurate complex refractive index can also be calculated by inversion using the contour intersection method. The accuracy of the inversion results can be ensured when the measurement error is less than 5%. The results of inversion using the contour intersection method are better than those of the iterative methods under the same conditions. This study provides a simple and reliable inversion method for measuring the complex refractive index of Au-Ag alloy nanospheres.
first_indexed 2024-03-11T04:14:12Z
format Article
id doaj.art-7328d9bbf8eb4e63893380131776842b
institution Directory Open Access Journal
issn 1996-1944
language English
last_indexed 2024-03-11T04:14:12Z
publishDate 2023-04-01
publisher MDPI AG
record_format Article
series Materials
spelling doaj.art-7328d9bbf8eb4e63893380131776842b2023-11-17T23:14:07ZengMDPI AGMaterials1996-19442023-04-01169329110.3390/ma16093291Inversion of the Complex Refractive Index of Au-Ag Alloy Nanospheres Based on the Contour Intersection MethodLong Cheng0Paerhatijiang Tuersun1Dengpan Ma2Dilishati Wumaier3Yixuan Li4Xinjiang Key Laboratory for Luminescence Minerals and Optical Functional Materials, School of Physics and Electronic Engineering, Xinjiang Normal University, Urumqi 830054, ChinaXinjiang Key Laboratory for Luminescence Minerals and Optical Functional Materials, School of Physics and Electronic Engineering, Xinjiang Normal University, Urumqi 830054, ChinaXinjiang Key Laboratory for Luminescence Minerals and Optical Functional Materials, School of Physics and Electronic Engineering, Xinjiang Normal University, Urumqi 830054, ChinaXinjiang Key Laboratory for Luminescence Minerals and Optical Functional Materials, School of Physics and Electronic Engineering, Xinjiang Normal University, Urumqi 830054, ChinaXinjiang Key Laboratory for Luminescence Minerals and Optical Functional Materials, School of Physics and Electronic Engineering, Xinjiang Normal University, Urumqi 830054, ChinaThe contour intersection method is a new method used to invert the complex refractive index of small particles. Research has yet to be reported on using this method to invert the complex refractive index of nanoparticles. This paper reports the feasibility and reliability of the contour intersection method in the inversion of the complex refractive index of nanoparticles using Au-Ag alloy nanospheres. The Mie theory and the size-dependent dielectric function are used to calculate the light scattering and absorption efficiency of Au-Ag alloy nanospheres corresponding to the complex refractive index. The complex refractive index of the particles is obtained by inversion with the contour intersection method. The backscattering efficiency constraint method is used to determine the unique solution when multiple valid solutions from the contour intersection method appear. The effects of the Au component percentage, particle size, and measurement errors on the inversion results are quantitatively analyzed. Finally, the inversion accuracy is compared and analyzed with the traditional iterative method. The results show that as long as the light scattering efficiency, light absorption efficiency, and backscattering efficiency of Au nanospheres can be measured, the accurate complex refractive index can also be calculated by inversion using the contour intersection method. The accuracy of the inversion results can be ensured when the measurement error is less than 5%. The results of inversion using the contour intersection method are better than those of the iterative methods under the same conditions. This study provides a simple and reliable inversion method for measuring the complex refractive index of Au-Ag alloy nanospheres.https://www.mdpi.com/1996-1944/16/9/3291Mie theorycontour intersection methodAu-Ag alloy nanospherescomplex refractive index
spellingShingle Long Cheng
Paerhatijiang Tuersun
Dengpan Ma
Dilishati Wumaier
Yixuan Li
Inversion of the Complex Refractive Index of Au-Ag Alloy Nanospheres Based on the Contour Intersection Method
Materials
Mie theory
contour intersection method
Au-Ag alloy nanospheres
complex refractive index
title Inversion of the Complex Refractive Index of Au-Ag Alloy Nanospheres Based on the Contour Intersection Method
title_full Inversion of the Complex Refractive Index of Au-Ag Alloy Nanospheres Based on the Contour Intersection Method
title_fullStr Inversion of the Complex Refractive Index of Au-Ag Alloy Nanospheres Based on the Contour Intersection Method
title_full_unstemmed Inversion of the Complex Refractive Index of Au-Ag Alloy Nanospheres Based on the Contour Intersection Method
title_short Inversion of the Complex Refractive Index of Au-Ag Alloy Nanospheres Based on the Contour Intersection Method
title_sort inversion of the complex refractive index of au ag alloy nanospheres based on the contour intersection method
topic Mie theory
contour intersection method
Au-Ag alloy nanospheres
complex refractive index
url https://www.mdpi.com/1996-1944/16/9/3291
work_keys_str_mv AT longcheng inversionofthecomplexrefractiveindexofauagalloynanospheresbasedonthecontourintersectionmethod
AT paerhatijiangtuersun inversionofthecomplexrefractiveindexofauagalloynanospheresbasedonthecontourintersectionmethod
AT dengpanma inversionofthecomplexrefractiveindexofauagalloynanospheresbasedonthecontourintersectionmethod
AT dilishatiwumaier inversionofthecomplexrefractiveindexofauagalloynanospheresbasedonthecontourintersectionmethod
AT yixuanli inversionofthecomplexrefractiveindexofauagalloynanospheresbasedonthecontourintersectionmethod