The four-wavelength Photoacoustic Aerosol Absorption Spectrometer (PAAS-4<i>λ</i>)

<p>In this paper, the Photoacoustic Aerosol Absorption Spectrometer (PAAS-4<span class="inline-formula"><i>λ</i></span>) is introduced. PAAS-4<span class="inline-formula"><i>λ</i></span> was specifically developed for long-ter...

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Main Authors: F. M. Schnaiter, C. Linke, E. Asmi, H. Servomaa, A.-P. Hyvärinen, S. Ohata, Y. Kondo, E. Järvinen
Format: Article
Language:English
Published: Copernicus Publications 2023-06-01
Series:Atmospheric Measurement Techniques
Online Access:https://amt.copernicus.org/articles/16/2753/2023/amt-16-2753-2023.pdf
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author F. M. Schnaiter
F. M. Schnaiter
C. Linke
E. Asmi
H. Servomaa
A.-P. Hyvärinen
S. Ohata
S. Ohata
Y. Kondo
E. Järvinen
author_facet F. M. Schnaiter
F. M. Schnaiter
C. Linke
E. Asmi
H. Servomaa
A.-P. Hyvärinen
S. Ohata
S. Ohata
Y. Kondo
E. Järvinen
author_sort F. M. Schnaiter
collection DOAJ
description <p>In this paper, the Photoacoustic Aerosol Absorption Spectrometer (PAAS-4<span class="inline-formula"><i>λ</i></span>) is introduced. PAAS-4<span class="inline-formula"><i>λ</i></span> was specifically developed for long-term monitoring tasks in (unattended) air quality stations. It uses four wavelengths coupled to a single acoustic resonator in a compact and robust set-up. The instrument has been thoroughly characterized and carefully calibrated in the laboratory using NO<span class="inline-formula"><sub>2</sub></span>/air mixtures and Nigrosin aerosol. It has an ultimate <span class="inline-formula">1<i>σ</i></span> detection limit below 0.1 Mm<span class="inline-formula"><sup>−1</sup></span>, at a measurement precision and accuracy of 3 % and 10 %, respectively. In order to demonstrate the PAAS-4<span class="inline-formula"><i>λ</i></span> suitability for long-term monitoring tasks, the instrument is currently validated at the air quality monitoring station Pallas in Finland, about 140 km north of the Arctic circle. A total of 11 months of PAAS-4<span class="inline-formula"><i>λ</i></span> data from this deployment are presented and discussed in terms of instrument performance. Intercomparisons with the filter-based photometers of a continuous soot monitoring system (COSMOS), the Multi-Angle Absorption Photometer (MAAP), and Aethalometer (AE33) demonstrate the capabilities and value of PAAS-4<span class="inline-formula"><i>λ</i></span>, as well as for the validation of the widely used filter-based instruments.</p>
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spelling doaj.art-7399f90d6d3e4744b5464369678a09772023-06-02T09:22:14ZengCopernicus PublicationsAtmospheric Measurement Techniques1867-13811867-85482023-06-01162753276910.5194/amt-16-2753-2023The four-wavelength Photoacoustic Aerosol Absorption Spectrometer (PAAS-4<i>λ</i>)F. M. Schnaiter0F. M. Schnaiter1C. Linke2E. Asmi3H. Servomaa4A.-P. Hyvärinen5S. Ohata6S. Ohata7Y. Kondo8E. Järvinen9Institute of Meteorology and Climate Research, Karlsruhe Institute of Technology, Kaiserstraße 12, 76021 Karlsruhe, Germany​​​​​​​schnaiTEC GmbH, Werner-von-Siemens-Str. 2–6, 76646 Bruchsal, GermanyInstitute of Meteorology and Climate Research, Karlsruhe Institute of Technology, Kaiserstraße 12, 76021 Karlsruhe, Germany​​​​​​​Finnish Meteorological Institute, P.O. Box 503, 00101 Helsinki, FinlandFinnish Meteorological Institute, P.O. Box 503, 00101 Helsinki, FinlandFinnish Meteorological Institute, P.O. Box 503, 00101 Helsinki, FinlandInstitute for Space–Earth Environmental Research, Nagoya University, Nagoya, Aichi, JapanInstitute for Advanced Research, Nagoya University, Nagoya, Aichi, JapanNational Institute of Polar Research, Tokyo, JapanInstitute of Meteorology and Climate Research, Karlsruhe Institute of Technology, Kaiserstraße 12, 76021 Karlsruhe, Germany​​​​​​​<p>In this paper, the Photoacoustic Aerosol Absorption Spectrometer (PAAS-4<span class="inline-formula"><i>λ</i></span>) is introduced. PAAS-4<span class="inline-formula"><i>λ</i></span> was specifically developed for long-term monitoring tasks in (unattended) air quality stations. It uses four wavelengths coupled to a single acoustic resonator in a compact and robust set-up. The instrument has been thoroughly characterized and carefully calibrated in the laboratory using NO<span class="inline-formula"><sub>2</sub></span>/air mixtures and Nigrosin aerosol. It has an ultimate <span class="inline-formula">1<i>σ</i></span> detection limit below 0.1 Mm<span class="inline-formula"><sup>−1</sup></span>, at a measurement precision and accuracy of 3 % and 10 %, respectively. In order to demonstrate the PAAS-4<span class="inline-formula"><i>λ</i></span> suitability for long-term monitoring tasks, the instrument is currently validated at the air quality monitoring station Pallas in Finland, about 140 km north of the Arctic circle. A total of 11 months of PAAS-4<span class="inline-formula"><i>λ</i></span> data from this deployment are presented and discussed in terms of instrument performance. Intercomparisons with the filter-based photometers of a continuous soot monitoring system (COSMOS), the Multi-Angle Absorption Photometer (MAAP), and Aethalometer (AE33) demonstrate the capabilities and value of PAAS-4<span class="inline-formula"><i>λ</i></span>, as well as for the validation of the widely used filter-based instruments.</p>https://amt.copernicus.org/articles/16/2753/2023/amt-16-2753-2023.pdf
spellingShingle F. M. Schnaiter
F. M. Schnaiter
C. Linke
E. Asmi
H. Servomaa
A.-P. Hyvärinen
S. Ohata
S. Ohata
Y. Kondo
E. Järvinen
The four-wavelength Photoacoustic Aerosol Absorption Spectrometer (PAAS-4<i>λ</i>)
Atmospheric Measurement Techniques
title The four-wavelength Photoacoustic Aerosol Absorption Spectrometer (PAAS-4<i>λ</i>)
title_full The four-wavelength Photoacoustic Aerosol Absorption Spectrometer (PAAS-4<i>λ</i>)
title_fullStr The four-wavelength Photoacoustic Aerosol Absorption Spectrometer (PAAS-4<i>λ</i>)
title_full_unstemmed The four-wavelength Photoacoustic Aerosol Absorption Spectrometer (PAAS-4<i>λ</i>)
title_short The four-wavelength Photoacoustic Aerosol Absorption Spectrometer (PAAS-4<i>λ</i>)
title_sort four wavelength photoacoustic aerosol absorption spectrometer paas 4 i λ i
url https://amt.copernicus.org/articles/16/2753/2023/amt-16-2753-2023.pdf
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