The effect of pressure variation on droplet size distribution of dispersed oil under simulated deep-water conditions
Droplet size distribution of dispersed oil in deep-water is critical to the transport and biodegradation of spilled oil in deep-sea. Few studies have focused on the effects of pressure on chemically dispersed oil through experiments. This study thus simulated how the crude oil homogenously pre-dispe...
Main Authors: | , , , , , , , , |
---|---|
Format: | Article |
Language: | English |
Published: |
Elsevier
2021-03-01
|
Series: | Heliyon |
Subjects: | |
Online Access: | http://www.sciencedirect.com/science/article/pii/S2405844021003960 |
_version_ | 1819142261432123392 |
---|---|
author | Xing Song Liang Jing Bing Chen Zhiwen Zhu Qinhong Cai Xudong Ye Xiao Zheng Stephen J. Hill Baiyu Zhang |
author_facet | Xing Song Liang Jing Bing Chen Zhiwen Zhu Qinhong Cai Xudong Ye Xiao Zheng Stephen J. Hill Baiyu Zhang |
author_sort | Xing Song |
collection | DOAJ |
description | Droplet size distribution of dispersed oil in deep-water is critical to the transport and biodegradation of spilled oil in deep-sea. Few studies have focused on the effects of pressure on chemically dispersed oil through experiments. This study thus simulated how the crude oil homogenously pre-dispersed by Corexit 9500A using baffled flasks would behave after being exposed to deep-water conditions. Key factors included dispersant-to-oil ratio (DOR), mixing energy (energy dissipation rate and Kolmogorov microscale), and pressure (up to 150 bar). The variations of pressure were demonstrated to have insignificant effects on the size distribution of pre-dispersed oil. Both the average and medium droplet sizes were correlated negatively with DOR and mixing energy in an established model with a p-value ≤ 0.0011. The log-normal and log-logistic distributions provided a reasonable fit to simulate the droplet size distribution. The two parameters of log-logistic distribution were dependent on DOR and mixing energy with a p-value < 0.005. The results would be valuable to advance the understanding of the behaviours and trajectories of chemically dispersed oil under deep-water conditions. The research helped provide more scientific evidence to improve the understanding of dispersed oil behaviours under high pressure and support deep-sea oil spill research and potential extension of the existing results from shallow water to deep water conditions. |
first_indexed | 2024-12-22T12:07:32Z |
format | Article |
id | doaj.art-74e1e79a4fcb4f4cb957f1edeaecff01 |
institution | Directory Open Access Journal |
issn | 2405-8440 |
language | English |
last_indexed | 2024-12-22T12:07:32Z |
publishDate | 2021-03-01 |
publisher | Elsevier |
record_format | Article |
series | Heliyon |
spelling | doaj.art-74e1e79a4fcb4f4cb957f1edeaecff012022-12-21T18:26:23ZengElsevierHeliyon2405-84402021-03-0173e06291The effect of pressure variation on droplet size distribution of dispersed oil under simulated deep-water conditionsXing Song0Liang Jing1Bing Chen2Zhiwen Zhu3Qinhong Cai4Xudong Ye5Xiao Zheng6Stephen J. Hill7Baiyu Zhang8Northern Region Persistent Organic Pollution Control (NRPOP) Laboratory, Faculty of Engineering and Applied Science, Memorial University of Newfoundland, St. John's, NL A1B 3X5, CanadaNorthern Region Persistent Organic Pollution Control (NRPOP) Laboratory, Faculty of Engineering and Applied Science, Memorial University of Newfoundland, St. John's, NL A1B 3X5, Canada; Department of Chemical and Petroleum Engineering, Schulich School of Engineering, University of Calgary, Calgary, AB T2N 1N4, CanadaNorthern Region Persistent Organic Pollution Control (NRPOP) Laboratory, Faculty of Engineering and Applied Science, Memorial University of Newfoundland, St. John's, NL A1B 3X5, Canada; Corresponding author.Northern Region Persistent Organic Pollution Control (NRPOP) Laboratory, Faculty of Engineering and Applied Science, Memorial University of Newfoundland, St. John's, NL A1B 3X5, CanadaNorthern Region Persistent Organic Pollution Control (NRPOP) Laboratory, Faculty of Engineering and Applied Science, Memorial University of Newfoundland, St. John's, NL A1B 3X5, Canada; Department of Natural Resource Sciences, McGill University, Anne de Bellevue, QC H9X 3V9, CanadaNorthern Region Persistent Organic Pollution Control (NRPOP) Laboratory, Faculty of Engineering and Applied Science, Memorial University of Newfoundland, St. John's, NL A1B 3X5, CanadaNorthern Region Persistent Organic Pollution Control (NRPOP) Laboratory, Faculty of Engineering and Applied Science, Memorial University of Newfoundland, St. John's, NL A1B 3X5, CanadaDepartment of Ocean Sciences, Memorial University of Newfoundland, St. John's, NL A1B 5S7, CanadaNorthern Region Persistent Organic Pollution Control (NRPOP) Laboratory, Faculty of Engineering and Applied Science, Memorial University of Newfoundland, St. John's, NL A1B 3X5, CanadaDroplet size distribution of dispersed oil in deep-water is critical to the transport and biodegradation of spilled oil in deep-sea. Few studies have focused on the effects of pressure on chemically dispersed oil through experiments. This study thus simulated how the crude oil homogenously pre-dispersed by Corexit 9500A using baffled flasks would behave after being exposed to deep-water conditions. Key factors included dispersant-to-oil ratio (DOR), mixing energy (energy dissipation rate and Kolmogorov microscale), and pressure (up to 150 bar). The variations of pressure were demonstrated to have insignificant effects on the size distribution of pre-dispersed oil. Both the average and medium droplet sizes were correlated negatively with DOR and mixing energy in an established model with a p-value ≤ 0.0011. The log-normal and log-logistic distributions provided a reasonable fit to simulate the droplet size distribution. The two parameters of log-logistic distribution were dependent on DOR and mixing energy with a p-value < 0.005. The results would be valuable to advance the understanding of the behaviours and trajectories of chemically dispersed oil under deep-water conditions. The research helped provide more scientific evidence to improve the understanding of dispersed oil behaviours under high pressure and support deep-sea oil spill research and potential extension of the existing results from shallow water to deep water conditions.http://www.sciencedirect.com/science/article/pii/S2405844021003960Marine oil spillChemically dispersed oilDroplet size distributionDeep-waterHigh pressureMixing energy |
spellingShingle | Xing Song Liang Jing Bing Chen Zhiwen Zhu Qinhong Cai Xudong Ye Xiao Zheng Stephen J. Hill Baiyu Zhang The effect of pressure variation on droplet size distribution of dispersed oil under simulated deep-water conditions Heliyon Marine oil spill Chemically dispersed oil Droplet size distribution Deep-water High pressure Mixing energy |
title | The effect of pressure variation on droplet size distribution of dispersed oil under simulated deep-water conditions |
title_full | The effect of pressure variation on droplet size distribution of dispersed oil under simulated deep-water conditions |
title_fullStr | The effect of pressure variation on droplet size distribution of dispersed oil under simulated deep-water conditions |
title_full_unstemmed | The effect of pressure variation on droplet size distribution of dispersed oil under simulated deep-water conditions |
title_short | The effect of pressure variation on droplet size distribution of dispersed oil under simulated deep-water conditions |
title_sort | effect of pressure variation on droplet size distribution of dispersed oil under simulated deep water conditions |
topic | Marine oil spill Chemically dispersed oil Droplet size distribution Deep-water High pressure Mixing energy |
url | http://www.sciencedirect.com/science/article/pii/S2405844021003960 |
work_keys_str_mv | AT xingsong theeffectofpressurevariationondropletsizedistributionofdispersedoilundersimulateddeepwaterconditions AT liangjing theeffectofpressurevariationondropletsizedistributionofdispersedoilundersimulateddeepwaterconditions AT bingchen theeffectofpressurevariationondropletsizedistributionofdispersedoilundersimulateddeepwaterconditions AT zhiwenzhu theeffectofpressurevariationondropletsizedistributionofdispersedoilundersimulateddeepwaterconditions AT qinhongcai theeffectofpressurevariationondropletsizedistributionofdispersedoilundersimulateddeepwaterconditions AT xudongye theeffectofpressurevariationondropletsizedistributionofdispersedoilundersimulateddeepwaterconditions AT xiaozheng theeffectofpressurevariationondropletsizedistributionofdispersedoilundersimulateddeepwaterconditions AT stephenjhill theeffectofpressurevariationondropletsizedistributionofdispersedoilundersimulateddeepwaterconditions AT baiyuzhang theeffectofpressurevariationondropletsizedistributionofdispersedoilundersimulateddeepwaterconditions AT xingsong effectofpressurevariationondropletsizedistributionofdispersedoilundersimulateddeepwaterconditions AT liangjing effectofpressurevariationondropletsizedistributionofdispersedoilundersimulateddeepwaterconditions AT bingchen effectofpressurevariationondropletsizedistributionofdispersedoilundersimulateddeepwaterconditions AT zhiwenzhu effectofpressurevariationondropletsizedistributionofdispersedoilundersimulateddeepwaterconditions AT qinhongcai effectofpressurevariationondropletsizedistributionofdispersedoilundersimulateddeepwaterconditions AT xudongye effectofpressurevariationondropletsizedistributionofdispersedoilundersimulateddeepwaterconditions AT xiaozheng effectofpressurevariationondropletsizedistributionofdispersedoilundersimulateddeepwaterconditions AT stephenjhill effectofpressurevariationondropletsizedistributionofdispersedoilundersimulateddeepwaterconditions AT baiyuzhang effectofpressurevariationondropletsizedistributionofdispersedoilundersimulateddeepwaterconditions |