The effect of pressure variation on droplet size distribution of dispersed oil under simulated deep-water conditions

Droplet size distribution of dispersed oil in deep-water is critical to the transport and biodegradation of spilled oil in deep-sea. Few studies have focused on the effects of pressure on chemically dispersed oil through experiments. This study thus simulated how the crude oil homogenously pre-dispe...

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Main Authors: Xing Song, Liang Jing, Bing Chen, Zhiwen Zhu, Qinhong Cai, Xudong Ye, Xiao Zheng, Stephen J. Hill, Baiyu Zhang
Format: Article
Language:English
Published: Elsevier 2021-03-01
Series:Heliyon
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2405844021003960
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author Xing Song
Liang Jing
Bing Chen
Zhiwen Zhu
Qinhong Cai
Xudong Ye
Xiao Zheng
Stephen J. Hill
Baiyu Zhang
author_facet Xing Song
Liang Jing
Bing Chen
Zhiwen Zhu
Qinhong Cai
Xudong Ye
Xiao Zheng
Stephen J. Hill
Baiyu Zhang
author_sort Xing Song
collection DOAJ
description Droplet size distribution of dispersed oil in deep-water is critical to the transport and biodegradation of spilled oil in deep-sea. Few studies have focused on the effects of pressure on chemically dispersed oil through experiments. This study thus simulated how the crude oil homogenously pre-dispersed by Corexit 9500A using baffled flasks would behave after being exposed to deep-water conditions. Key factors included dispersant-to-oil ratio (DOR), mixing energy (energy dissipation rate and Kolmogorov microscale), and pressure (up to 150 bar). The variations of pressure were demonstrated to have insignificant effects on the size distribution of pre-dispersed oil. Both the average and medium droplet sizes were correlated negatively with DOR and mixing energy in an established model with a p-value ≤ 0.0011. The log-normal and log-logistic distributions provided a reasonable fit to simulate the droplet size distribution. The two parameters of log-logistic distribution were dependent on DOR and mixing energy with a p-value < 0.005. The results would be valuable to advance the understanding of the behaviours and trajectories of chemically dispersed oil under deep-water conditions. The research helped provide more scientific evidence to improve the understanding of dispersed oil behaviours under high pressure and support deep-sea oil spill research and potential extension of the existing results from shallow water to deep water conditions.
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spelling doaj.art-74e1e79a4fcb4f4cb957f1edeaecff012022-12-21T18:26:23ZengElsevierHeliyon2405-84402021-03-0173e06291The effect of pressure variation on droplet size distribution of dispersed oil under simulated deep-water conditionsXing Song0Liang Jing1Bing Chen2Zhiwen Zhu3Qinhong Cai4Xudong Ye5Xiao Zheng6Stephen J. Hill7Baiyu Zhang8Northern Region Persistent Organic Pollution Control (NRPOP) Laboratory, Faculty of Engineering and Applied Science, Memorial University of Newfoundland, St. John's, NL A1B 3X5, CanadaNorthern Region Persistent Organic Pollution Control (NRPOP) Laboratory, Faculty of Engineering and Applied Science, Memorial University of Newfoundland, St. John's, NL A1B 3X5, Canada; Department of Chemical and Petroleum Engineering, Schulich School of Engineering, University of Calgary, Calgary, AB T2N 1N4, CanadaNorthern Region Persistent Organic Pollution Control (NRPOP) Laboratory, Faculty of Engineering and Applied Science, Memorial University of Newfoundland, St. John's, NL A1B 3X5, Canada; Corresponding author.Northern Region Persistent Organic Pollution Control (NRPOP) Laboratory, Faculty of Engineering and Applied Science, Memorial University of Newfoundland, St. John's, NL A1B 3X5, CanadaNorthern Region Persistent Organic Pollution Control (NRPOP) Laboratory, Faculty of Engineering and Applied Science, Memorial University of Newfoundland, St. John's, NL A1B 3X5, Canada; Department of Natural Resource Sciences, McGill University, Anne de Bellevue, QC H9X 3V9, CanadaNorthern Region Persistent Organic Pollution Control (NRPOP) Laboratory, Faculty of Engineering and Applied Science, Memorial University of Newfoundland, St. John's, NL A1B 3X5, CanadaNorthern Region Persistent Organic Pollution Control (NRPOP) Laboratory, Faculty of Engineering and Applied Science, Memorial University of Newfoundland, St. John's, NL A1B 3X5, CanadaDepartment of Ocean Sciences, Memorial University of Newfoundland, St. John's, NL A1B 5S7, CanadaNorthern Region Persistent Organic Pollution Control (NRPOP) Laboratory, Faculty of Engineering and Applied Science, Memorial University of Newfoundland, St. John's, NL A1B 3X5, CanadaDroplet size distribution of dispersed oil in deep-water is critical to the transport and biodegradation of spilled oil in deep-sea. Few studies have focused on the effects of pressure on chemically dispersed oil through experiments. This study thus simulated how the crude oil homogenously pre-dispersed by Corexit 9500A using baffled flasks would behave after being exposed to deep-water conditions. Key factors included dispersant-to-oil ratio (DOR), mixing energy (energy dissipation rate and Kolmogorov microscale), and pressure (up to 150 bar). The variations of pressure were demonstrated to have insignificant effects on the size distribution of pre-dispersed oil. Both the average and medium droplet sizes were correlated negatively with DOR and mixing energy in an established model with a p-value ≤ 0.0011. The log-normal and log-logistic distributions provided a reasonable fit to simulate the droplet size distribution. The two parameters of log-logistic distribution were dependent on DOR and mixing energy with a p-value < 0.005. The results would be valuable to advance the understanding of the behaviours and trajectories of chemically dispersed oil under deep-water conditions. The research helped provide more scientific evidence to improve the understanding of dispersed oil behaviours under high pressure and support deep-sea oil spill research and potential extension of the existing results from shallow water to deep water conditions.http://www.sciencedirect.com/science/article/pii/S2405844021003960Marine oil spillChemically dispersed oilDroplet size distributionDeep-waterHigh pressureMixing energy
spellingShingle Xing Song
Liang Jing
Bing Chen
Zhiwen Zhu
Qinhong Cai
Xudong Ye
Xiao Zheng
Stephen J. Hill
Baiyu Zhang
The effect of pressure variation on droplet size distribution of dispersed oil under simulated deep-water conditions
Heliyon
Marine oil spill
Chemically dispersed oil
Droplet size distribution
Deep-water
High pressure
Mixing energy
title The effect of pressure variation on droplet size distribution of dispersed oil under simulated deep-water conditions
title_full The effect of pressure variation on droplet size distribution of dispersed oil under simulated deep-water conditions
title_fullStr The effect of pressure variation on droplet size distribution of dispersed oil under simulated deep-water conditions
title_full_unstemmed The effect of pressure variation on droplet size distribution of dispersed oil under simulated deep-water conditions
title_short The effect of pressure variation on droplet size distribution of dispersed oil under simulated deep-water conditions
title_sort effect of pressure variation on droplet size distribution of dispersed oil under simulated deep water conditions
topic Marine oil spill
Chemically dispersed oil
Droplet size distribution
Deep-water
High pressure
Mixing energy
url http://www.sciencedirect.com/science/article/pii/S2405844021003960
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