New Composite Materials Prepared by Solution Combustion Synthesis for Catalytic Reforming of Methane

Processing of natural gas into motor fuel has become one of the major problems of chemistry. Partial oxidation and CO2 reforming of CH4 attract a great attention in recent years. Resistant to temperature extremes and thermal shocks is one of the most important requirements for catalysts. Works on re...

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Main Authors: S.A. Tungatarova, G. Xanthopoulou, K. Karanasios, T.S. Baizhumanova, M. Zhumabek, G. Kaumenova
Format: Article
Language:English
Published: AIDIC Servizi S.r.l. 2017-10-01
Series:Chemical Engineering Transactions
Online Access:https://www.cetjournal.it/index.php/cet/article/view/371
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author S.A. Tungatarova
G. Xanthopoulou
K. Karanasios
T.S. Baizhumanova
M. Zhumabek
G. Kaumenova
author_facet S.A. Tungatarova
G. Xanthopoulou
K. Karanasios
T.S. Baizhumanova
M. Zhumabek
G. Kaumenova
author_sort S.A. Tungatarova
collection DOAJ
description Processing of natural gas into motor fuel has become one of the major problems of chemistry. Partial oxidation and CO2 reforming of CH4 attract a great attention in recent years. Resistant to temperature extremes and thermal shocks is one of the most important requirements for catalysts. Works on research of intermetallic compounds as a contact mass for conversion of methane were carried out. Method of self- propagating high temperature synthesis was used for synthesis of catalysts. Investigation of the activity of catalysts based on the initial mixture of metal oxides produced in the solution combustion synthesis process was carried out in the reaction of carbon dioxide conversion and partial oxidation of methane. 100 % methane conversion at 750 °C was carried out on the catalyst, whereas the conversion of CO2 reached 81.7 % at 900 oC. H2 yield reached 99.2 %, yield of CO - 99.1 % in the ratio of H2/CO = 1.2. Effective catalysts for the production of synthesis gas from methane have been developed.
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spelling doaj.art-75e02cceb96e457195f0d26eb629ba002022-12-21T20:14:27ZengAIDIC Servizi S.r.l.Chemical Engineering Transactions2283-92162017-10-016110.3303/CET1761318New Composite Materials Prepared by Solution Combustion Synthesis for Catalytic Reforming of MethaneS.A. TungatarovaG. XanthopoulouK. KaranasiosT.S. BaizhumanovaM. ZhumabekG. KaumenovaProcessing of natural gas into motor fuel has become one of the major problems of chemistry. Partial oxidation and CO2 reforming of CH4 attract a great attention in recent years. Resistant to temperature extremes and thermal shocks is one of the most important requirements for catalysts. Works on research of intermetallic compounds as a contact mass for conversion of methane were carried out. Method of self- propagating high temperature synthesis was used for synthesis of catalysts. Investigation of the activity of catalysts based on the initial mixture of metal oxides produced in the solution combustion synthesis process was carried out in the reaction of carbon dioxide conversion and partial oxidation of methane. 100 % methane conversion at 750 °C was carried out on the catalyst, whereas the conversion of CO2 reached 81.7 % at 900 oC. H2 yield reached 99.2 %, yield of CO - 99.1 % in the ratio of H2/CO = 1.2. Effective catalysts for the production of synthesis gas from methane have been developed.https://www.cetjournal.it/index.php/cet/article/view/371
spellingShingle S.A. Tungatarova
G. Xanthopoulou
K. Karanasios
T.S. Baizhumanova
M. Zhumabek
G. Kaumenova
New Composite Materials Prepared by Solution Combustion Synthesis for Catalytic Reforming of Methane
Chemical Engineering Transactions
title New Composite Materials Prepared by Solution Combustion Synthesis for Catalytic Reforming of Methane
title_full New Composite Materials Prepared by Solution Combustion Synthesis for Catalytic Reforming of Methane
title_fullStr New Composite Materials Prepared by Solution Combustion Synthesis for Catalytic Reforming of Methane
title_full_unstemmed New Composite Materials Prepared by Solution Combustion Synthesis for Catalytic Reforming of Methane
title_short New Composite Materials Prepared by Solution Combustion Synthesis for Catalytic Reforming of Methane
title_sort new composite materials prepared by solution combustion synthesis for catalytic reforming of methane
url https://www.cetjournal.it/index.php/cet/article/view/371
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AT gxanthopoulou newcompositematerialspreparedbysolutioncombustionsynthesisforcatalyticreformingofmethane
AT kkaranasios newcompositematerialspreparedbysolutioncombustionsynthesisforcatalyticreformingofmethane
AT tsbaizhumanova newcompositematerialspreparedbysolutioncombustionsynthesisforcatalyticreformingofmethane
AT mzhumabek newcompositematerialspreparedbysolutioncombustionsynthesisforcatalyticreformingofmethane
AT gkaumenova newcompositematerialspreparedbysolutioncombustionsynthesisforcatalyticreformingofmethane