Repetitive non-thermal melting as a timing monitor for femtosecond pump/probe X-ray experiments

Time-resolved optical pump/X-ray probe experiments are often used to study structural dynamics. To ensure high temporal resolution, it is necessary to monitor the timing between the X-ray pulses and the laser pulses. The transition from a crystalline solid material to a disordered state in a non-the...

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Main Authors: Å. U. J. Bengtsson, J. C. Ekström, Xiaocui Wang, A. Jurgilaitis, Van-Thai Pham, D. Kroon, J. Larsson
Format: Article
Language:English
Published: AIP Publishing LLC and ACA 2020-09-01
Series:Structural Dynamics
Online Access:http://dx.doi.org/10.1063/4.0000020
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author Å. U. J. Bengtsson
J. C. Ekström
Xiaocui Wang
A. Jurgilaitis
Van-Thai Pham
D. Kroon
J. Larsson
author_facet Å. U. J. Bengtsson
J. C. Ekström
Xiaocui Wang
A. Jurgilaitis
Van-Thai Pham
D. Kroon
J. Larsson
author_sort Å. U. J. Bengtsson
collection DOAJ
description Time-resolved optical pump/X-ray probe experiments are often used to study structural dynamics. To ensure high temporal resolution, it is necessary to monitor the timing between the X-ray pulses and the laser pulses. The transition from a crystalline solid material to a disordered state in a non-thermal melting process can be used as a reliable timing monitor. We have performed a study of the non-thermal melting of InSb in single-shot mode, where we varied the sample temperature in order to determine the conditions required for repetitive melting. We show how experimental conditions affect the feasibility of such a timing tool.
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spelling doaj.art-762153257bbd49049069ad9547c65fdf2022-12-22T01:07:08ZengAIP Publishing LLC and ACAStructural Dynamics2329-77782020-09-0175054303054303-610.1063/4.0000020Repetitive non-thermal melting as a timing monitor for femtosecond pump/probe X-ray experimentsÅ. U. J. Bengtsson0J. C. Ekström1Xiaocui Wang2A. Jurgilaitis3Van-Thai Pham4D. Kroon5J. Larsson6 Department of Physics, Lund University, P.O. Box 118, SE-221 00 Lund, Sweden Department of Physics, Lund University, P.O. Box 118, SE-221 00 Lund, Sweden Department of Physics, Lund University, P.O. Box 118, SE-221 00 Lund, Sweden MAX IV Laboratory, Lund University, P.O. Box 118, SE-221 00 Lund, Sweden MAX IV Laboratory, Lund University, P.O. Box 118, SE-221 00 Lund, Sweden MAX IV Laboratory, Lund University, P.O. Box 118, SE-221 00 Lund, Sweden Department of Physics, Lund University, P.O. Box 118, SE-221 00 Lund, SwedenTime-resolved optical pump/X-ray probe experiments are often used to study structural dynamics. To ensure high temporal resolution, it is necessary to monitor the timing between the X-ray pulses and the laser pulses. The transition from a crystalline solid material to a disordered state in a non-thermal melting process can be used as a reliable timing monitor. We have performed a study of the non-thermal melting of InSb in single-shot mode, where we varied the sample temperature in order to determine the conditions required for repetitive melting. We show how experimental conditions affect the feasibility of such a timing tool.http://dx.doi.org/10.1063/4.0000020
spellingShingle Å. U. J. Bengtsson
J. C. Ekström
Xiaocui Wang
A. Jurgilaitis
Van-Thai Pham
D. Kroon
J. Larsson
Repetitive non-thermal melting as a timing monitor for femtosecond pump/probe X-ray experiments
Structural Dynamics
title Repetitive non-thermal melting as a timing monitor for femtosecond pump/probe X-ray experiments
title_full Repetitive non-thermal melting as a timing monitor for femtosecond pump/probe X-ray experiments
title_fullStr Repetitive non-thermal melting as a timing monitor for femtosecond pump/probe X-ray experiments
title_full_unstemmed Repetitive non-thermal melting as a timing monitor for femtosecond pump/probe X-ray experiments
title_short Repetitive non-thermal melting as a timing monitor for femtosecond pump/probe X-ray experiments
title_sort repetitive non thermal melting as a timing monitor for femtosecond pump probe x ray experiments
url http://dx.doi.org/10.1063/4.0000020
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