Repetitive non-thermal melting as a timing monitor for femtosecond pump/probe X-ray experiments
Time-resolved optical pump/X-ray probe experiments are often used to study structural dynamics. To ensure high temporal resolution, it is necessary to monitor the timing between the X-ray pulses and the laser pulses. The transition from a crystalline solid material to a disordered state in a non-the...
Main Authors: | , , , , , , |
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Format: | Article |
Language: | English |
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AIP Publishing LLC and ACA
2020-09-01
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Series: | Structural Dynamics |
Online Access: | http://dx.doi.org/10.1063/4.0000020 |
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author | Å. U. J. Bengtsson J. C. Ekström Xiaocui Wang A. Jurgilaitis Van-Thai Pham D. Kroon J. Larsson |
author_facet | Å. U. J. Bengtsson J. C. Ekström Xiaocui Wang A. Jurgilaitis Van-Thai Pham D. Kroon J. Larsson |
author_sort | Å. U. J. Bengtsson |
collection | DOAJ |
description | Time-resolved optical pump/X-ray probe experiments are often used to study structural dynamics. To ensure high temporal resolution, it is necessary to monitor the timing between the X-ray pulses and the laser pulses. The transition from a crystalline solid material to a disordered state in a non-thermal melting process can be used as a reliable timing monitor. We have performed a study of the non-thermal melting of InSb in single-shot mode, where we varied the sample temperature in order to determine the conditions required for repetitive melting. We show how experimental conditions affect the feasibility of such a timing tool. |
first_indexed | 2024-12-11T12:36:04Z |
format | Article |
id | doaj.art-762153257bbd49049069ad9547c65fdf |
institution | Directory Open Access Journal |
issn | 2329-7778 |
language | English |
last_indexed | 2024-12-11T12:36:04Z |
publishDate | 2020-09-01 |
publisher | AIP Publishing LLC and ACA |
record_format | Article |
series | Structural Dynamics |
spelling | doaj.art-762153257bbd49049069ad9547c65fdf2022-12-22T01:07:08ZengAIP Publishing LLC and ACAStructural Dynamics2329-77782020-09-0175054303054303-610.1063/4.0000020Repetitive non-thermal melting as a timing monitor for femtosecond pump/probe X-ray experimentsÅ. U. J. Bengtsson0J. C. Ekström1Xiaocui Wang2A. Jurgilaitis3Van-Thai Pham4D. Kroon5J. Larsson6 Department of Physics, Lund University, P.O. Box 118, SE-221 00 Lund, Sweden Department of Physics, Lund University, P.O. Box 118, SE-221 00 Lund, Sweden Department of Physics, Lund University, P.O. Box 118, SE-221 00 Lund, Sweden MAX IV Laboratory, Lund University, P.O. Box 118, SE-221 00 Lund, Sweden MAX IV Laboratory, Lund University, P.O. Box 118, SE-221 00 Lund, Sweden MAX IV Laboratory, Lund University, P.O. Box 118, SE-221 00 Lund, Sweden Department of Physics, Lund University, P.O. Box 118, SE-221 00 Lund, SwedenTime-resolved optical pump/X-ray probe experiments are often used to study structural dynamics. To ensure high temporal resolution, it is necessary to monitor the timing between the X-ray pulses and the laser pulses. The transition from a crystalline solid material to a disordered state in a non-thermal melting process can be used as a reliable timing monitor. We have performed a study of the non-thermal melting of InSb in single-shot mode, where we varied the sample temperature in order to determine the conditions required for repetitive melting. We show how experimental conditions affect the feasibility of such a timing tool.http://dx.doi.org/10.1063/4.0000020 |
spellingShingle | Å. U. J. Bengtsson J. C. Ekström Xiaocui Wang A. Jurgilaitis Van-Thai Pham D. Kroon J. Larsson Repetitive non-thermal melting as a timing monitor for femtosecond pump/probe X-ray experiments Structural Dynamics |
title | Repetitive non-thermal melting as a timing monitor for femtosecond pump/probe X-ray experiments |
title_full | Repetitive non-thermal melting as a timing monitor for femtosecond pump/probe X-ray experiments |
title_fullStr | Repetitive non-thermal melting as a timing monitor for femtosecond pump/probe X-ray experiments |
title_full_unstemmed | Repetitive non-thermal melting as a timing monitor for femtosecond pump/probe X-ray experiments |
title_short | Repetitive non-thermal melting as a timing monitor for femtosecond pump/probe X-ray experiments |
title_sort | repetitive non thermal melting as a timing monitor for femtosecond pump probe x ray experiments |
url | http://dx.doi.org/10.1063/4.0000020 |
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