Enhancement of electrocatalytic oxygen evolution by chiral molecular functionalization of hybrid 2D electrodes
While solar-to-fuel catalysis requires the careful transfer of electrons, there are still challenges understanding how electron spin contributes to reactivity. Here, authors employ chiral fused thiadiazole-helicenes to control spin polarization in oxygen evolution electrocatalysts.
| Main Authors: | , , , , , , , , , , |
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| Format: | Article |
| Language: | English |
| Published: |
Nature Portfolio
2022-06-01
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| Series: | Nature Communications |
| Online Access: | https://doi.org/10.1038/s41467-022-31096-8 |
| _version_ | 1818211654467321856 |
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| author | Yunchang Liang Karla Banjac Kévin Martin Nicolas Zigon Seunghwa Lee Nicolas Vanthuyne Felipe Andrés Garcés-Pineda José R. Galán-Mascarós Xile Hu Narcis Avarvari Magalí Lingenfelder |
| author_facet | Yunchang Liang Karla Banjac Kévin Martin Nicolas Zigon Seunghwa Lee Nicolas Vanthuyne Felipe Andrés Garcés-Pineda José R. Galán-Mascarós Xile Hu Narcis Avarvari Magalí Lingenfelder |
| author_sort | Yunchang Liang |
| collection | DOAJ |
| description | While solar-to-fuel catalysis requires the careful transfer of electrons, there are still challenges understanding how electron spin contributes to reactivity. Here, authors employ chiral fused thiadiazole-helicenes to control spin polarization in oxygen evolution electrocatalysts. |
| first_indexed | 2024-12-12T05:35:56Z |
| format | Article |
| id | doaj.art-76e8032fc6e944cb914da5db0d4e563c |
| institution | Directory Open Access Journal |
| issn | 2041-1723 |
| language | English |
| last_indexed | 2024-12-12T05:35:56Z |
| publishDate | 2022-06-01 |
| publisher | Nature Portfolio |
| record_format | Article |
| series | Nature Communications |
| spelling | doaj.art-76e8032fc6e944cb914da5db0d4e563c2022-12-22T00:36:08ZengNature PortfolioNature Communications2041-17232022-06-011311910.1038/s41467-022-31096-8Enhancement of electrocatalytic oxygen evolution by chiral molecular functionalization of hybrid 2D electrodesYunchang Liang0Karla Banjac1Kévin Martin2Nicolas Zigon3Seunghwa Lee4Nicolas Vanthuyne5Felipe Andrés Garcés-Pineda6José R. Galán-Mascarós7Xile Hu8Narcis Avarvari9Magalí Lingenfelder10Max Planck-EPFL Laboratory for Molecular Nanoscience and Technology, École Polytechnique Fédérale de Lausanne (EPFL)Max Planck-EPFL Laboratory for Molecular Nanoscience and Technology, École Polytechnique Fédérale de Lausanne (EPFL)Univ Angers, CNRS, MOLTECH-Anjou, SFR MATRIXUniv Angers, CNRS, MOLTECH-Anjou, SFR MATRIXLaboratory of Inorganic Synthesis and Catalysis, Institute of Chemical Sciences and Engineering, École Polytechnique Fédérale de Lausanne (EPFL)Aix Marseille Université, CNRS, Centrale Marseille, iSm2Institute of Chemical Research of Catalonia (ICIQ), The Barcelona Institute of Science and Technology (BIST)Institute of Chemical Research of Catalonia (ICIQ), The Barcelona Institute of Science and Technology (BIST)Laboratory of Inorganic Synthesis and Catalysis, Institute of Chemical Sciences and Engineering, École Polytechnique Fédérale de Lausanne (EPFL)Univ Angers, CNRS, MOLTECH-Anjou, SFR MATRIXMax Planck-EPFL Laboratory for Molecular Nanoscience and Technology, École Polytechnique Fédérale de Lausanne (EPFL)While solar-to-fuel catalysis requires the careful transfer of electrons, there are still challenges understanding how electron spin contributes to reactivity. Here, authors employ chiral fused thiadiazole-helicenes to control spin polarization in oxygen evolution electrocatalysts.https://doi.org/10.1038/s41467-022-31096-8 |
| spellingShingle | Yunchang Liang Karla Banjac Kévin Martin Nicolas Zigon Seunghwa Lee Nicolas Vanthuyne Felipe Andrés Garcés-Pineda José R. Galán-Mascarós Xile Hu Narcis Avarvari Magalí Lingenfelder Enhancement of electrocatalytic oxygen evolution by chiral molecular functionalization of hybrid 2D electrodes Nature Communications |
| title | Enhancement of electrocatalytic oxygen evolution by chiral molecular functionalization of hybrid 2D electrodes |
| title_full | Enhancement of electrocatalytic oxygen evolution by chiral molecular functionalization of hybrid 2D electrodes |
| title_fullStr | Enhancement of electrocatalytic oxygen evolution by chiral molecular functionalization of hybrid 2D electrodes |
| title_full_unstemmed | Enhancement of electrocatalytic oxygen evolution by chiral molecular functionalization of hybrid 2D electrodes |
| title_short | Enhancement of electrocatalytic oxygen evolution by chiral molecular functionalization of hybrid 2D electrodes |
| title_sort | enhancement of electrocatalytic oxygen evolution by chiral molecular functionalization of hybrid 2d electrodes |
| url | https://doi.org/10.1038/s41467-022-31096-8 |
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