Properties-Adjustable Alumina-Zirconia Nanolaminate Dielectric Fabricated by Spin-Coating
In this paper, an alumina-zirconia (Al2O3-ZrO2) nanolaminate dielectric was fabricated by spin-coating and the performance was investigated. It was found that the properties of the dielectric can be adjusted by changing the content of Al2O3/ZrO2 in nanolaminates: when the content of Al2O3 was higher...
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MDPI AG
2017-11-01
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author | Junbiao Peng Jinglin Wei Zhennan Zhu Honglong Ning Wei Cai Kuankuan Lu Rihui Yao Hong Tao Yanqiong Zheng Xubing Lu |
author_facet | Junbiao Peng Jinglin Wei Zhennan Zhu Honglong Ning Wei Cai Kuankuan Lu Rihui Yao Hong Tao Yanqiong Zheng Xubing Lu |
author_sort | Junbiao Peng |
collection | DOAJ |
description | In this paper, an alumina-zirconia (Al2O3-ZrO2) nanolaminate dielectric was fabricated by spin-coating and the performance was investigated. It was found that the properties of the dielectric can be adjusted by changing the content of Al2O3/ZrO2 in nanolaminates: when the content of Al2O3 was higher than 50%, the properties of nanolaminates, such as the optical energy gap, dielectric strength (Vds), capacitance density, and relative permittivity were relatively stable, while the change of these properties became larger when the content of Al2O3 was less than 50%. With the content of ZrO2 varying from 50% to 100%, the variation of these properties was up to 0.482 eV, 2.12 MV/cm, 135.35 nF/cm2, and 11.64, respectively. Furthermore, it was demonstrated that the dielectric strength of nanolaminates were influenced significantly by the number (n) of bilayers. Every increment of one Al2O3-ZrO2 bilayer will enhance the dielectric strength by around 0.39 MV/cm (Vds ≈ 0.86 + 0.39n). This could be contributed to the amorphous alumina which interrupted the grain boundaries of zirconia. |
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spelling | doaj.art-77111ce55d5c42b4827c80597b69ffdb2022-12-22T02:42:25ZengMDPI AGNanomaterials2079-49912017-11-0171241910.3390/nano7120419nano7120419Properties-Adjustable Alumina-Zirconia Nanolaminate Dielectric Fabricated by Spin-CoatingJunbiao Peng0Jinglin Wei1Zhennan Zhu2Honglong Ning3Wei Cai4Kuankuan Lu5Rihui Yao6Hong Tao7Yanqiong Zheng8Xubing Lu9School of Electronic and Information Engineering, South China University of Technology, Guangzhou 510640, ChinaSchool of Electronic and Information Engineering, South China University of Technology, Guangzhou 510640, ChinaInstitute of Polymer Optoelectronic Materials and Devices, State Key Laboratory of Luminescent Materials and Devices, South China University of Technology, Guangzhou 510640, ChinaInstitute of Polymer Optoelectronic Materials and Devices, State Key Laboratory of Luminescent Materials and Devices, South China University of Technology, Guangzhou 510640, ChinaInstitute of Polymer Optoelectronic Materials and Devices, State Key Laboratory of Luminescent Materials and Devices, South China University of Technology, Guangzhou 510640, ChinaInstitute of Polymer Optoelectronic Materials and Devices, State Key Laboratory of Luminescent Materials and Devices, South China University of Technology, Guangzhou 510640, ChinaInstitute of Polymer Optoelectronic Materials and Devices, State Key Laboratory of Luminescent Materials and Devices, South China University of Technology, Guangzhou 510640, ChinaInstitute of Polymer Optoelectronic Materials and Devices, State Key Laboratory of Luminescent Materials and Devices, South China University of Technology, Guangzhou 510640, ChinaKey Laboratory of Advanced Display and System Applications of Ministry of Education, Shanghai University, Shanghai 200072, ChinaInstitute for Advanced Materials and Guangdong Provincial Key Laboratory of Quantum Engineering and Quantum Materials, South China Normal University, Guangzhou 510006, ChinaIn this paper, an alumina-zirconia (Al2O3-ZrO2) nanolaminate dielectric was fabricated by spin-coating and the performance was investigated. It was found that the properties of the dielectric can be adjusted by changing the content of Al2O3/ZrO2 in nanolaminates: when the content of Al2O3 was higher than 50%, the properties of nanolaminates, such as the optical energy gap, dielectric strength (Vds), capacitance density, and relative permittivity were relatively stable, while the change of these properties became larger when the content of Al2O3 was less than 50%. With the content of ZrO2 varying from 50% to 100%, the variation of these properties was up to 0.482 eV, 2.12 MV/cm, 135.35 nF/cm2, and 11.64, respectively. Furthermore, it was demonstrated that the dielectric strength of nanolaminates were influenced significantly by the number (n) of bilayers. Every increment of one Al2O3-ZrO2 bilayer will enhance the dielectric strength by around 0.39 MV/cm (Vds ≈ 0.86 + 0.39n). This could be contributed to the amorphous alumina which interrupted the grain boundaries of zirconia.https://www.mdpi.com/2079-4991/7/12/419properties-adjustableAl2O3-ZrO2 nanolaminate dielectricspin-coating |
spellingShingle | Junbiao Peng Jinglin Wei Zhennan Zhu Honglong Ning Wei Cai Kuankuan Lu Rihui Yao Hong Tao Yanqiong Zheng Xubing Lu Properties-Adjustable Alumina-Zirconia Nanolaminate Dielectric Fabricated by Spin-Coating Nanomaterials properties-adjustable Al2O3-ZrO2 nanolaminate dielectric spin-coating |
title | Properties-Adjustable Alumina-Zirconia Nanolaminate Dielectric Fabricated by Spin-Coating |
title_full | Properties-Adjustable Alumina-Zirconia Nanolaminate Dielectric Fabricated by Spin-Coating |
title_fullStr | Properties-Adjustable Alumina-Zirconia Nanolaminate Dielectric Fabricated by Spin-Coating |
title_full_unstemmed | Properties-Adjustable Alumina-Zirconia Nanolaminate Dielectric Fabricated by Spin-Coating |
title_short | Properties-Adjustable Alumina-Zirconia Nanolaminate Dielectric Fabricated by Spin-Coating |
title_sort | properties adjustable alumina zirconia nanolaminate dielectric fabricated by spin coating |
topic | properties-adjustable Al2O3-ZrO2 nanolaminate dielectric spin-coating |
url | https://www.mdpi.com/2079-4991/7/12/419 |
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