Short-term dispersal of Fukushima-derived radionuclides off Japan: modeling efforts and model-data intercomparison

The Great East Japan Earthquake and tsunami that caused a loss of power at the Fukushima nuclear power plants (FNPP) resulted in emission of radioactive isotopes into the atmosphere and the ocean. In June of 2011, an international survey measuring a variety of radionuclide isotopes, including <su...

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Main Authors: I. I. Rypina, S. R. Jayne, S. Yoshida, A. M. Macdonald, E. Douglass, K. Buesseler
Format: Article
Language:English
Published: Copernicus Publications 2013-07-01
Series:Biogeosciences
Online Access:http://www.biogeosciences.net/10/4973/2013/bg-10-4973-2013.pdf
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author I. I. Rypina
S. R. Jayne
S. Yoshida
A. M. Macdonald
E. Douglass
K. Buesseler
author_facet I. I. Rypina
S. R. Jayne
S. Yoshida
A. M. Macdonald
E. Douglass
K. Buesseler
author_sort I. I. Rypina
collection DOAJ
description The Great East Japan Earthquake and tsunami that caused a loss of power at the Fukushima nuclear power plants (FNPP) resulted in emission of radioactive isotopes into the atmosphere and the ocean. In June of 2011, an international survey measuring a variety of radionuclide isotopes, including <sup>137</sup>Cs, was conducted in surface and subsurface waters off Japan. This paper presents the results of numerical simulations specifically aimed at interpreting these observations and investigating the spread of Fukushima-derived radionuclides off the coast of Japan and into the greater Pacific Ocean. Together, the simulations and observations allow us to study the dominant mechanisms governing this process, and to estimate the total amount of radionuclides in discharged coolant waters and atmospheric airborne radionuclide fallout. The numerical simulations are based on two different ocean circulation models, one inferred from AVISO altimetry and NCEP/NCAR reanalysis wind stress, and the second generated numerically by the NCOM model. Our simulations determine that > 95% of <sup>137</sup>Cs remaining in the water within ~600 km of Fukushima, Japan in mid-June 2011 was due to the direct oceanic discharge. The estimated strength of the oceanic source is 16.2 ± 1.6 PBq, based on minimizing the model-data mismatch. We cannot make an accurate estimate for the atmospheric source strength since most of the fallout cesium had left the survey area by mid-June. The model explained several key features of the observed <sup>137</sup>Cs distribution. First, the absence of <sup>137</sup>Cs at the southernmost stations is attributed to the Kuroshio Current acting as a transport barrier against the southward progression of <sup>137</sup>Cs. Second, the largest <sup>137</sup>Cs concentrations were associated with a semi-permanent eddy that entrained <sup>137</sup>Cs-rich waters, collecting and stirring them around the eddy perimeter. Finally, the intermediate <sup>137</sup>Cs concentrations at the westernmost stations are attributed to younger, and therefore less Cs-rich, coolant waters that continued to leak from the reactor in June of that year.
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spelling doaj.art-7783c07c75ff4cefbee74f9940fb78392022-12-21T23:58:32ZengCopernicus PublicationsBiogeosciences1726-41701726-41892013-07-011074973499010.5194/bg-10-4973-2013Short-term dispersal of Fukushima-derived radionuclides off Japan: modeling efforts and model-data intercomparisonI. I. RypinaS. R. JayneS. YoshidaA. M. MacdonaldE. DouglassK. BuesselerThe Great East Japan Earthquake and tsunami that caused a loss of power at the Fukushima nuclear power plants (FNPP) resulted in emission of radioactive isotopes into the atmosphere and the ocean. In June of 2011, an international survey measuring a variety of radionuclide isotopes, including <sup>137</sup>Cs, was conducted in surface and subsurface waters off Japan. This paper presents the results of numerical simulations specifically aimed at interpreting these observations and investigating the spread of Fukushima-derived radionuclides off the coast of Japan and into the greater Pacific Ocean. Together, the simulations and observations allow us to study the dominant mechanisms governing this process, and to estimate the total amount of radionuclides in discharged coolant waters and atmospheric airborne radionuclide fallout. The numerical simulations are based on two different ocean circulation models, one inferred from AVISO altimetry and NCEP/NCAR reanalysis wind stress, and the second generated numerically by the NCOM model. Our simulations determine that > 95% of <sup>137</sup>Cs remaining in the water within ~600 km of Fukushima, Japan in mid-June 2011 was due to the direct oceanic discharge. The estimated strength of the oceanic source is 16.2 ± 1.6 PBq, based on minimizing the model-data mismatch. We cannot make an accurate estimate for the atmospheric source strength since most of the fallout cesium had left the survey area by mid-June. The model explained several key features of the observed <sup>137</sup>Cs distribution. First, the absence of <sup>137</sup>Cs at the southernmost stations is attributed to the Kuroshio Current acting as a transport barrier against the southward progression of <sup>137</sup>Cs. Second, the largest <sup>137</sup>Cs concentrations were associated with a semi-permanent eddy that entrained <sup>137</sup>Cs-rich waters, collecting and stirring them around the eddy perimeter. Finally, the intermediate <sup>137</sup>Cs concentrations at the westernmost stations are attributed to younger, and therefore less Cs-rich, coolant waters that continued to leak from the reactor in June of that year.http://www.biogeosciences.net/10/4973/2013/bg-10-4973-2013.pdf
spellingShingle I. I. Rypina
S. R. Jayne
S. Yoshida
A. M. Macdonald
E. Douglass
K. Buesseler
Short-term dispersal of Fukushima-derived radionuclides off Japan: modeling efforts and model-data intercomparison
Biogeosciences
title Short-term dispersal of Fukushima-derived radionuclides off Japan: modeling efforts and model-data intercomparison
title_full Short-term dispersal of Fukushima-derived radionuclides off Japan: modeling efforts and model-data intercomparison
title_fullStr Short-term dispersal of Fukushima-derived radionuclides off Japan: modeling efforts and model-data intercomparison
title_full_unstemmed Short-term dispersal of Fukushima-derived radionuclides off Japan: modeling efforts and model-data intercomparison
title_short Short-term dispersal of Fukushima-derived radionuclides off Japan: modeling efforts and model-data intercomparison
title_sort short term dispersal of fukushima derived radionuclides off japan modeling efforts and model data intercomparison
url http://www.biogeosciences.net/10/4973/2013/bg-10-4973-2013.pdf
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