Spin-orbit coupling-enhanced valley ordering of malleable bands in twisted bilayer graphene on WSe2

Abstract Recent experiments in magic-angle twisted bilayer graphene have revealed a wealth of novel electronic phases as a result of interaction-driven spin-valley flavour polarisation. In this work, we investigate correlated phases due to the combined effect of spin-orbit coupling-enhanced valley p...

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Main Authors: Saisab Bhowmik, Bhaskar Ghawri, Youngju Park, Dongkyu Lee, Suvronil Datta, Radhika Soni, K. Watanabe, T. Taniguchi, Arindam Ghosh, Jeil Jung, U. Chandni
Format: Article
Language:English
Published: Nature Portfolio 2023-07-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-023-39855-x
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author Saisab Bhowmik
Bhaskar Ghawri
Youngju Park
Dongkyu Lee
Suvronil Datta
Radhika Soni
K. Watanabe
T. Taniguchi
Arindam Ghosh
Jeil Jung
U. Chandni
author_facet Saisab Bhowmik
Bhaskar Ghawri
Youngju Park
Dongkyu Lee
Suvronil Datta
Radhika Soni
K. Watanabe
T. Taniguchi
Arindam Ghosh
Jeil Jung
U. Chandni
author_sort Saisab Bhowmik
collection DOAJ
description Abstract Recent experiments in magic-angle twisted bilayer graphene have revealed a wealth of novel electronic phases as a result of interaction-driven spin-valley flavour polarisation. In this work, we investigate correlated phases due to the combined effect of spin-orbit coupling-enhanced valley polarisation and the large density of states below half filling of the moiré band in twisted bilayer graphene coupled to tungsten diselenide. We observe an anomalous Hall effect, accompanied by a series of Lifshitz transitions that are highly tunable with carrier density and magnetic field. The magnetisation shows an abrupt change of sign near half-filling, confirming its orbital nature. While the Hall resistance is not quantised at zero magnetic fields—indicating a ground state with partial valley polarisation—perfect quantisation and complete valley polarisation are observed at finite fields. Our results illustrate that singularities in the flat bands in the presence of spin-orbit coupling can stabilise ordered phases even at non-integer moiré band fillings.
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spelling doaj.art-789672dcee27490b8d97ce15521650ef2023-07-09T11:18:41ZengNature PortfolioNature Communications2041-17232023-07-011411810.1038/s41467-023-39855-xSpin-orbit coupling-enhanced valley ordering of malleable bands in twisted bilayer graphene on WSe2Saisab Bhowmik0Bhaskar Ghawri1Youngju Park2Dongkyu Lee3Suvronil Datta4Radhika Soni5K. Watanabe6T. Taniguchi7Arindam Ghosh8Jeil Jung9U. Chandni10Department of Instrumentation and Applied Physics, Indian Institute of ScienceDepartment of Physics, Indian Institute of ScienceDepartment of Physics, University of SeoulDepartment of Physics, University of SeoulDepartment of Instrumentation and Applied Physics, Indian Institute of ScienceDepartment of Instrumentation and Applied Physics, Indian Institute of ScienceResearch Center for Functional Materials, National Institute for Materials ScienceInternational Center for Materials Nanoarchitectonics, National Institute for Materials ScienceDepartment of Physics, Indian Institute of ScienceDepartment of Physics, University of SeoulDepartment of Instrumentation and Applied Physics, Indian Institute of ScienceAbstract Recent experiments in magic-angle twisted bilayer graphene have revealed a wealth of novel electronic phases as a result of interaction-driven spin-valley flavour polarisation. In this work, we investigate correlated phases due to the combined effect of spin-orbit coupling-enhanced valley polarisation and the large density of states below half filling of the moiré band in twisted bilayer graphene coupled to tungsten diselenide. We observe an anomalous Hall effect, accompanied by a series of Lifshitz transitions that are highly tunable with carrier density and magnetic field. The magnetisation shows an abrupt change of sign near half-filling, confirming its orbital nature. While the Hall resistance is not quantised at zero magnetic fields—indicating a ground state with partial valley polarisation—perfect quantisation and complete valley polarisation are observed at finite fields. Our results illustrate that singularities in the flat bands in the presence of spin-orbit coupling can stabilise ordered phases even at non-integer moiré band fillings.https://doi.org/10.1038/s41467-023-39855-x
spellingShingle Saisab Bhowmik
Bhaskar Ghawri
Youngju Park
Dongkyu Lee
Suvronil Datta
Radhika Soni
K. Watanabe
T. Taniguchi
Arindam Ghosh
Jeil Jung
U. Chandni
Spin-orbit coupling-enhanced valley ordering of malleable bands in twisted bilayer graphene on WSe2
Nature Communications
title Spin-orbit coupling-enhanced valley ordering of malleable bands in twisted bilayer graphene on WSe2
title_full Spin-orbit coupling-enhanced valley ordering of malleable bands in twisted bilayer graphene on WSe2
title_fullStr Spin-orbit coupling-enhanced valley ordering of malleable bands in twisted bilayer graphene on WSe2
title_full_unstemmed Spin-orbit coupling-enhanced valley ordering of malleable bands in twisted bilayer graphene on WSe2
title_short Spin-orbit coupling-enhanced valley ordering of malleable bands in twisted bilayer graphene on WSe2
title_sort spin orbit coupling enhanced valley ordering of malleable bands in twisted bilayer graphene on wse2
url https://doi.org/10.1038/s41467-023-39855-x
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