Improve Dentin Bonding Performance Using a Hydrolytically Stable, Ether-Based Primer
The objective of this study is to replace a traditional methacrylate-based primer (glycine, N-(2-hydroxy-3-(2-methyl-1-oxo-2-propenyl)propyl)-N-(4-methylphenyl) monosodium salt, NTG-GMA) with a hydrolytically stable ether-based primer (glycine, N-2-hydroxy-3-(4-vinylbenzyloxy)-propyl-N-(4-methylphen...
| Main Authors: | , , |
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| Format: | Article |
| Language: | English |
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MDPI AG
2022-08-01
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| Series: | Journal of Functional Biomaterials |
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| Online Access: | https://www.mdpi.com/2079-4983/13/3/128 |
| _version_ | 1827660083094355968 |
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| author | Xiaohong Wang Shinobu Yamauchi Jirun Sun |
| author_facet | Xiaohong Wang Shinobu Yamauchi Jirun Sun |
| author_sort | Xiaohong Wang |
| collection | DOAJ |
| description | The objective of this study is to replace a traditional methacrylate-based primer (glycine, N-(2-hydroxy-3-(2-methyl-1-oxo-2-propenyl)propyl)-N-(4-methylphenyl) monosodium salt, NTG-GMA) with a hydrolytically stable ether-based primer (glycine, N-2-hydroxy-3-(4-vinylbenzyloxy)-propyl-N-(4-methylphenyl), monosodium salt, NTG-VBGE). The performance and durability of bonding composites to detin of two primers combined with methacrylate-based or ether-based adhesives were evaluated using shear bond strength (SBS) and micro-tensile bond strength (μTBS) combined with thermal cycling. The hydrolysis resistance of NTG-VBGE against hydrolysis was tested by challenging primed hydroxyapatite crystals with an esterase. The hydrophilicity of the primers and the resin spreading kinetics of adhesives on primed dentin were characterized by water contact angle measurements. The new primer NTG-VBGE was found to be compatible with both methacrylate-based adhesives and ether-based adhesives. The highest μTBS values were found in the test group of NTG-VBGE and ether-based adhesive, which was consistent with the resin spreading kinetics results. The more hydrophobic and hydrolytically stable primer/adhesive achieved improved dentin infiltration and bonding strength, suggesting significant potential for further developing dental restorative materials with extended service life. |
| first_indexed | 2024-03-09T23:34:11Z |
| format | Article |
| id | doaj.art-78d7a05112264ec5aad1167ca6c4dfa0 |
| institution | Directory Open Access Journal |
| issn | 2079-4983 |
| language | English |
| last_indexed | 2024-03-09T23:34:11Z |
| publishDate | 2022-08-01 |
| publisher | MDPI AG |
| record_format | Article |
| series | Journal of Functional Biomaterials |
| spelling | doaj.art-78d7a05112264ec5aad1167ca6c4dfa02023-11-23T17:03:32ZengMDPI AGJournal of Functional Biomaterials2079-49832022-08-0113312810.3390/jfb13030128Improve Dentin Bonding Performance Using a Hydrolytically Stable, Ether-Based PrimerXiaohong Wang0Shinobu Yamauchi1Jirun Sun2American Dental Association Science & Research Institute, Gaithersburg, MD 20899, USAAmerican Dental Association Science & Research Institute, Gaithersburg, MD 20899, USAThe Forsyth Institute, Cambridge, MA 02142, USAThe objective of this study is to replace a traditional methacrylate-based primer (glycine, N-(2-hydroxy-3-(2-methyl-1-oxo-2-propenyl)propyl)-N-(4-methylphenyl) monosodium salt, NTG-GMA) with a hydrolytically stable ether-based primer (glycine, N-2-hydroxy-3-(4-vinylbenzyloxy)-propyl-N-(4-methylphenyl), monosodium salt, NTG-VBGE). The performance and durability of bonding composites to detin of two primers combined with methacrylate-based or ether-based adhesives were evaluated using shear bond strength (SBS) and micro-tensile bond strength (μTBS) combined with thermal cycling. The hydrolysis resistance of NTG-VBGE against hydrolysis was tested by challenging primed hydroxyapatite crystals with an esterase. The hydrophilicity of the primers and the resin spreading kinetics of adhesives on primed dentin were characterized by water contact angle measurements. The new primer NTG-VBGE was found to be compatible with both methacrylate-based adhesives and ether-based adhesives. The highest μTBS values were found in the test group of NTG-VBGE and ether-based adhesive, which was consistent with the resin spreading kinetics results. The more hydrophobic and hydrolytically stable primer/adhesive achieved improved dentin infiltration and bonding strength, suggesting significant potential for further developing dental restorative materials with extended service life.https://www.mdpi.com/2079-4983/13/3/128dental adhesivebonding primerhydrolytically stableshear bond strengthmicro-tensile bond strength |
| spellingShingle | Xiaohong Wang Shinobu Yamauchi Jirun Sun Improve Dentin Bonding Performance Using a Hydrolytically Stable, Ether-Based Primer Journal of Functional Biomaterials dental adhesive bonding primer hydrolytically stable shear bond strength micro-tensile bond strength |
| title | Improve Dentin Bonding Performance Using a Hydrolytically Stable, Ether-Based Primer |
| title_full | Improve Dentin Bonding Performance Using a Hydrolytically Stable, Ether-Based Primer |
| title_fullStr | Improve Dentin Bonding Performance Using a Hydrolytically Stable, Ether-Based Primer |
| title_full_unstemmed | Improve Dentin Bonding Performance Using a Hydrolytically Stable, Ether-Based Primer |
| title_short | Improve Dentin Bonding Performance Using a Hydrolytically Stable, Ether-Based Primer |
| title_sort | improve dentin bonding performance using a hydrolytically stable ether based primer |
| topic | dental adhesive bonding primer hydrolytically stable shear bond strength micro-tensile bond strength |
| url | https://www.mdpi.com/2079-4983/13/3/128 |
| work_keys_str_mv | AT xiaohongwang improvedentinbondingperformanceusingahydrolyticallystableetherbasedprimer AT shinobuyamauchi improvedentinbondingperformanceusingahydrolyticallystableetherbasedprimer AT jirunsun improvedentinbondingperformanceusingahydrolyticallystableetherbasedprimer |