Characterisation of the Manchester Aerosol Chamber facility
<p>This study describes the design of the Manchester Aerosol Chamber (MAC), initially developed in 2005 and presents for the first time its comprehensive characterisation. The MAC is designed to investigate multi-phase chemistry and the evolution of aerosol physico-chemical properties from the...
Main Authors: | , , , , , , , |
---|---|
Format: | Article |
Language: | English |
Published: |
Copernicus Publications
2022-01-01
|
Series: | Atmospheric Measurement Techniques |
Online Access: | https://amt.copernicus.org/articles/15/539/2022/amt-15-539-2022.pdf |
_version_ | 1818319754963714048 |
---|---|
author | Y. Shao Y. Wang M. Du A. Voliotis M. R. Alfarra M. R. Alfarra M. R. Alfarra S. P. O'Meara S. P. O'Meara S. F. Turner S. F. Turner G. McFiggans |
author_facet | Y. Shao Y. Wang M. Du A. Voliotis M. R. Alfarra M. R. Alfarra M. R. Alfarra S. P. O'Meara S. P. O'Meara S. F. Turner S. F. Turner G. McFiggans |
author_sort | Y. Shao |
collection | DOAJ |
description | <p>This study describes the design of the Manchester Aerosol Chamber (MAC), initially developed in 2005 and presents for the first time its comprehensive characterisation. The MAC is designed to investigate multi-phase chemistry and the evolution of aerosol physico-chemical properties from the real-world emissions (e.g. diesel engine, plants) or of secondary organic aerosol (SOA) produced from pure volatile organic compounds (VOCs). Additionally, the generated aerosol particles in the MAC can be transferred to the Manchester Ice Cloud Chamber (MICC), which enables investigation of cloud formation in warm, mixed-phase, and fully glaciated conditions (with temperature, <span class="inline-formula"><i>T</i></span>, as low as <span class="inline-formula">−55</span> <span class="inline-formula"><sup>∘</sup>C</span>). The MAC is an 18 <span class="inline-formula">m<sup>3</sup></span> fluorinated ethylene propylene (FEP) Teflon chamber with the potential to conduct experiments at controlled temperature (15–35 <span class="inline-formula"><sup>∘</sup>C</span>) and relative humidity (RH; 25 %–80 %) under simulated solar radiation or dark conditions. Detailed characterisations were conducted at common experimental conditions (25 <span class="inline-formula"><sup>∘</sup>C</span>, 50 % RH) for actinometry and determination of background contamination, wall losses of gases (<span class="inline-formula">NO<sub>2</sub></span>, <span class="inline-formula">O<sub>3</sub></span>, and selected VOCs), aerosol particles at different sizes, chamber wall reactivity, and aerosol formation. In addition, the influences of chamber contamination on the wall loss rate of gases and particles and the photolysis of <span class="inline-formula">NO<sub>2</sub></span> were estimated.</p> |
first_indexed | 2024-12-13T10:14:09Z |
format | Article |
id | doaj.art-79fbc4a8d83a4e11ad865fdfef2aa510 |
institution | Directory Open Access Journal |
issn | 1867-1381 1867-8548 |
language | English |
last_indexed | 2024-12-13T10:14:09Z |
publishDate | 2022-01-01 |
publisher | Copernicus Publications |
record_format | Article |
series | Atmospheric Measurement Techniques |
spelling | doaj.art-79fbc4a8d83a4e11ad865fdfef2aa5102022-12-21T23:51:20ZengCopernicus PublicationsAtmospheric Measurement Techniques1867-13811867-85482022-01-011553955910.5194/amt-15-539-2022Characterisation of the Manchester Aerosol Chamber facilityY. Shao0Y. Wang1M. Du2A. Voliotis3M. R. Alfarra4M. R. Alfarra5M. R. Alfarra6S. P. O'Meara7S. P. O'Meara8S. F. Turner9S. F. Turner10G. McFiggans11Centre for Atmospheric Science, Department of Earth and Environmental Sciences, School of Natural Sciences, University of Manchester, Manchester, M13 9PL, UKCentre for Atmospheric Science, Department of Earth and Environmental Sciences, School of Natural Sciences, University of Manchester, Manchester, M13 9PL, UKCentre for Atmospheric Science, Department of Earth and Environmental Sciences, School of Natural Sciences, University of Manchester, Manchester, M13 9PL, UKCentre for Atmospheric Science, Department of Earth and Environmental Sciences, School of Natural Sciences, University of Manchester, Manchester, M13 9PL, UKCentre for Atmospheric Science, Department of Earth and Environmental Sciences, School of Natural Sciences, University of Manchester, Manchester, M13 9PL, UKNational Centre for Atmospheric Science (NCAS), University of Manchester, Manchester, M13 9PL, UKnow at: Environment & Sustainability Center, Qatar Environment & Energy Research Institute, 34110, Doha, QatarCentre for Atmospheric Science, Department of Earth and Environmental Sciences, School of Natural Sciences, University of Manchester, Manchester, M13 9PL, UKNational Centre for Atmospheric Science (NCAS), University of Manchester, Manchester, M13 9PL, UKCentre for Atmospheric Science, Department of Earth and Environmental Sciences, School of Natural Sciences, University of Manchester, Manchester, M13 9PL, UKnow at: AMETEK Land, Dronfield, Derbyshire, S18 1DJ, UKCentre for Atmospheric Science, Department of Earth and Environmental Sciences, School of Natural Sciences, University of Manchester, Manchester, M13 9PL, UK<p>This study describes the design of the Manchester Aerosol Chamber (MAC), initially developed in 2005 and presents for the first time its comprehensive characterisation. The MAC is designed to investigate multi-phase chemistry and the evolution of aerosol physico-chemical properties from the real-world emissions (e.g. diesel engine, plants) or of secondary organic aerosol (SOA) produced from pure volatile organic compounds (VOCs). Additionally, the generated aerosol particles in the MAC can be transferred to the Manchester Ice Cloud Chamber (MICC), which enables investigation of cloud formation in warm, mixed-phase, and fully glaciated conditions (with temperature, <span class="inline-formula"><i>T</i></span>, as low as <span class="inline-formula">−55</span> <span class="inline-formula"><sup>∘</sup>C</span>). The MAC is an 18 <span class="inline-formula">m<sup>3</sup></span> fluorinated ethylene propylene (FEP) Teflon chamber with the potential to conduct experiments at controlled temperature (15–35 <span class="inline-formula"><sup>∘</sup>C</span>) and relative humidity (RH; 25 %–80 %) under simulated solar radiation or dark conditions. Detailed characterisations were conducted at common experimental conditions (25 <span class="inline-formula"><sup>∘</sup>C</span>, 50 % RH) for actinometry and determination of background contamination, wall losses of gases (<span class="inline-formula">NO<sub>2</sub></span>, <span class="inline-formula">O<sub>3</sub></span>, and selected VOCs), aerosol particles at different sizes, chamber wall reactivity, and aerosol formation. In addition, the influences of chamber contamination on the wall loss rate of gases and particles and the photolysis of <span class="inline-formula">NO<sub>2</sub></span> were estimated.</p>https://amt.copernicus.org/articles/15/539/2022/amt-15-539-2022.pdf |
spellingShingle | Y. Shao Y. Wang M. Du A. Voliotis M. R. Alfarra M. R. Alfarra M. R. Alfarra S. P. O'Meara S. P. O'Meara S. F. Turner S. F. Turner G. McFiggans Characterisation of the Manchester Aerosol Chamber facility Atmospheric Measurement Techniques |
title | Characterisation of the Manchester Aerosol Chamber facility |
title_full | Characterisation of the Manchester Aerosol Chamber facility |
title_fullStr | Characterisation of the Manchester Aerosol Chamber facility |
title_full_unstemmed | Characterisation of the Manchester Aerosol Chamber facility |
title_short | Characterisation of the Manchester Aerosol Chamber facility |
title_sort | characterisation of the manchester aerosol chamber facility |
url | https://amt.copernicus.org/articles/15/539/2022/amt-15-539-2022.pdf |
work_keys_str_mv | AT yshao characterisationofthemanchesteraerosolchamberfacility AT ywang characterisationofthemanchesteraerosolchamberfacility AT mdu characterisationofthemanchesteraerosolchamberfacility AT avoliotis characterisationofthemanchesteraerosolchamberfacility AT mralfarra characterisationofthemanchesteraerosolchamberfacility AT mralfarra characterisationofthemanchesteraerosolchamberfacility AT mralfarra characterisationofthemanchesteraerosolchamberfacility AT spomeara characterisationofthemanchesteraerosolchamberfacility AT spomeara characterisationofthemanchesteraerosolchamberfacility AT sfturner characterisationofthemanchesteraerosolchamberfacility AT sfturner characterisationofthemanchesteraerosolchamberfacility AT gmcfiggans characterisationofthemanchesteraerosolchamberfacility |