Regulated adsorption sites using atomically single cluster over biochar for efficient elemental mercury uptake
Highlights A facile chelated coupled pyrolysis strategy was reported to prepare Mn single-cluster Hg0 adsorbent. The nitrogen-containing group in biomass determined the size of atomically dispersed manganese. The presence of oxygen and small size Mn clusters in biochar promoted Hg0 adsorption.
| Main Authors: | , , , , , , , , , |
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| Format: | Article |
| Language: | English |
| Published: |
Springer
2023-03-01
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| Series: | Biochar |
| Subjects: | |
| Online Access: | https://doi.org/10.1007/s42773-022-00200-y |
| _version_ | 1797863951244984320 |
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| author | Jiaxing Li Hongli Li Haomiao Xu Qinyuan Hong Leipeng Ji Zhisong Liu Yixiang Qiu Wenjun Huang Naiqiang Yan Zan Qu |
| author_facet | Jiaxing Li Hongli Li Haomiao Xu Qinyuan Hong Leipeng Ji Zhisong Liu Yixiang Qiu Wenjun Huang Naiqiang Yan Zan Qu |
| author_sort | Jiaxing Li |
| collection | DOAJ |
| description | Highlights A facile chelated coupled pyrolysis strategy was reported to prepare Mn single-cluster Hg0 adsorbent. The nitrogen-containing group in biomass determined the size of atomically dispersed manganese. The presence of oxygen and small size Mn clusters in biochar promoted Hg0 adsorption. |
| first_indexed | 2024-04-09T22:43:51Z |
| format | Article |
| id | doaj.art-7a1509f2f7ca448eb2d9d483cba39e85 |
| institution | Directory Open Access Journal |
| issn | 2524-7867 |
| language | English |
| last_indexed | 2024-04-09T22:43:51Z |
| publishDate | 2023-03-01 |
| publisher | Springer |
| record_format | Article |
| series | Biochar |
| spelling | doaj.art-7a1509f2f7ca448eb2d9d483cba39e852023-03-22T11:59:08ZengSpringerBiochar2524-78672023-03-015111510.1007/s42773-022-00200-yRegulated adsorption sites using atomically single cluster over biochar for efficient elemental mercury uptakeJiaxing Li0Hongli Li1Haomiao Xu2Qinyuan Hong3Leipeng Ji4Zhisong Liu5Yixiang Qiu6Wenjun Huang7Naiqiang Yan8Zan Qu9School of Environmental Science and Engineering, Shanghai Jiao Tong UniversityKey Laboratory of Magnetism and Magnetic Materials of the Ministry of Education, School of Physical Science and Technology and Electron, Microscopy Centre of Lanzhou University, Lanzhou UniversitySchool of Environmental Science and Engineering, Shanghai Jiao Tong UniversitySchool of Environmental Science and Engineering, Shanghai Jiao Tong UniversitySchool of Environmental Science and Engineering, Shanghai Jiao Tong UniversitySchool of Environmental Science and Engineering, Shanghai Jiao Tong UniversitySchool of Chemistry and Chemical Engineering, Shanghai Jiao Tong UniversitySchool of Environmental Science and Engineering, Shanghai Jiao Tong UniversitySchool of Environmental Science and Engineering, Shanghai Jiao Tong UniversitySchool of Environmental Science and Engineering, Shanghai Jiao Tong UniversityHighlights A facile chelated coupled pyrolysis strategy was reported to prepare Mn single-cluster Hg0 adsorbent. The nitrogen-containing group in biomass determined the size of atomically dispersed manganese. The presence of oxygen and small size Mn clusters in biochar promoted Hg0 adsorption.https://doi.org/10.1007/s42773-022-00200-yBiomassHeteroatomsManganese clustersElemental mercuryWaste recycling |
| spellingShingle | Jiaxing Li Hongli Li Haomiao Xu Qinyuan Hong Leipeng Ji Zhisong Liu Yixiang Qiu Wenjun Huang Naiqiang Yan Zan Qu Regulated adsorption sites using atomically single cluster over biochar for efficient elemental mercury uptake Biochar Biomass Heteroatoms Manganese clusters Elemental mercury Waste recycling |
| title | Regulated adsorption sites using atomically single cluster over biochar for efficient elemental mercury uptake |
| title_full | Regulated adsorption sites using atomically single cluster over biochar for efficient elemental mercury uptake |
| title_fullStr | Regulated adsorption sites using atomically single cluster over biochar for efficient elemental mercury uptake |
| title_full_unstemmed | Regulated adsorption sites using atomically single cluster over biochar for efficient elemental mercury uptake |
| title_short | Regulated adsorption sites using atomically single cluster over biochar for efficient elemental mercury uptake |
| title_sort | regulated adsorption sites using atomically single cluster over biochar for efficient elemental mercury uptake |
| topic | Biomass Heteroatoms Manganese clusters Elemental mercury Waste recycling |
| url | https://doi.org/10.1007/s42773-022-00200-y |
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