No circular birefringence exists in a chiral medium: an analysis of single-mode refraction

Optical activity is one of the most fundamental phenomena in nature. The existing theoretical description of optical activity is the circular birefringence, proposed in 1825 by Fresnel. It states that the right-handed circularly polarized (RCP) and left-handed circularly polarized (LCP) waves in a c...

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Main Authors: Zhi-Juan Hu, Chun-Fang Li
Format: Article
Language:English
Published: IOP Publishing 2023-01-01
Series:New Journal of Physics
Subjects:
Online Access:https://doi.org/10.1088/1367-2630/acb6e9
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author Zhi-Juan Hu
Chun-Fang Li
author_facet Zhi-Juan Hu
Chun-Fang Li
author_sort Zhi-Juan Hu
collection DOAJ
description Optical activity is one of the most fundamental phenomena in nature. The existing theoretical description of optical activity is the circular birefringence, proposed in 1825 by Fresnel. It states that the right-handed circularly polarized (RCP) and left-handed circularly polarized (LCP) waves in a chiral medium propagate at different velocities. Here we show that this is not the case. After obtaining the refraction and reflection coefficients of any elliptically polarized wave at the surface of an isotropic chiral medium, we derive the conditions for single-mode refraction. By means of the process of single-mode refraction, we demonstrate that both the refracted RCP and the refracted LCP waves at normal incidence can be expressed as a coherent superposition of a pair of orthogonal linearly polarized waves that are rotated simultaneously. As a result, they must propagate at the same velocity as the linearly polarized waves. A physical interpretation is also given in detail. In particular, we show that the state of polarization of any elliptically polarized wave in a chiral medium is rotated with propagation. Such a rotation amounts to the rotation of polarization bases without involving the change of the Jones vector. The rotation of the RCP and LCP waves, as special cases of elliptically polarized waves, results in two opposite phases as if they propagated at different phase velocities with their polarization states transmitted unchanged. These results demonstrate that the conventional characterization of optical polarization is incomplete. A further investigation into its new features is of great significance.
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spelling doaj.art-7a8ecf028c98421c9a8fbdfcccec93c22023-08-09T14:11:44ZengIOP PublishingNew Journal of Physics1367-26302023-01-0125202300710.1088/1367-2630/acb6e9No circular birefringence exists in a chiral medium: an analysis of single-mode refractionZhi-Juan Hu0https://orcid.org/0000-0003-4989-0326Chun-Fang Li1https://orcid.org/0000-0001-6897-8097Department of Physics, Shanghai Normal University , 100 Guilin Road, 200233 Shanghai, People’s Republic of ChinaDepartment of Physics, Shanghai University , 99 Shangda Road, 200444 Shanghai, People’s Republic of ChinaOptical activity is one of the most fundamental phenomena in nature. The existing theoretical description of optical activity is the circular birefringence, proposed in 1825 by Fresnel. It states that the right-handed circularly polarized (RCP) and left-handed circularly polarized (LCP) waves in a chiral medium propagate at different velocities. Here we show that this is not the case. After obtaining the refraction and reflection coefficients of any elliptically polarized wave at the surface of an isotropic chiral medium, we derive the conditions for single-mode refraction. By means of the process of single-mode refraction, we demonstrate that both the refracted RCP and the refracted LCP waves at normal incidence can be expressed as a coherent superposition of a pair of orthogonal linearly polarized waves that are rotated simultaneously. As a result, they must propagate at the same velocity as the linearly polarized waves. A physical interpretation is also given in detail. In particular, we show that the state of polarization of any elliptically polarized wave in a chiral medium is rotated with propagation. Such a rotation amounts to the rotation of polarization bases without involving the change of the Jones vector. The rotation of the RCP and LCP waves, as special cases of elliptically polarized waves, results in two opposite phases as if they propagated at different phase velocities with their polarization states transmitted unchanged. These results demonstrate that the conventional characterization of optical polarization is incomplete. A further investigation into its new features is of great significance.https://doi.org/10.1088/1367-2630/acb6e9polarization of lightcircular birefringenceoptical activityFresnel’s coefficientscircular double refractionsingle-mode refraction
spellingShingle Zhi-Juan Hu
Chun-Fang Li
No circular birefringence exists in a chiral medium: an analysis of single-mode refraction
New Journal of Physics
polarization of light
circular birefringence
optical activity
Fresnel’s coefficients
circular double refraction
single-mode refraction
title No circular birefringence exists in a chiral medium: an analysis of single-mode refraction
title_full No circular birefringence exists in a chiral medium: an analysis of single-mode refraction
title_fullStr No circular birefringence exists in a chiral medium: an analysis of single-mode refraction
title_full_unstemmed No circular birefringence exists in a chiral medium: an analysis of single-mode refraction
title_short No circular birefringence exists in a chiral medium: an analysis of single-mode refraction
title_sort no circular birefringence exists in a chiral medium an analysis of single mode refraction
topic polarization of light
circular birefringence
optical activity
Fresnel’s coefficients
circular double refraction
single-mode refraction
url https://doi.org/10.1088/1367-2630/acb6e9
work_keys_str_mv AT zhijuanhu nocircularbirefringenceexistsinachiralmediumananalysisofsinglemoderefraction
AT chunfangli nocircularbirefringenceexistsinachiralmediumananalysisofsinglemoderefraction