The Importance of Fiber/Matrix Adhesion and Annealing Process in Water Uptake of PLA/PMMA Matrix Composites Reinforced with Sisal Fibers: The Effect of Coupling Agent Addition
With the aim to open new applications possibilities to novel biocomposites based on PLA/PMMA matrix and reinforced with sisal fibers, it was studied the effect of water immersion aging on biocomposite tensile properties. In the current study it was evidenced the importance of the annealing process a...
Main Authors: | , , , , |
---|---|
Format: | Article |
Language: | English |
Published: |
Taylor & Francis Group
2022-11-01
|
Series: | Journal of Natural Fibers |
Subjects: | |
Online Access: | http://dx.doi.org/10.1080/15440478.2022.2028211 |
_version_ | 1797679963412889600 |
---|---|
author | Ander Orue Jon Anakabe Ane Miren Zaldua-Huici Arantxa Eceiza Aitor Arbelaiz |
author_facet | Ander Orue Jon Anakabe Ane Miren Zaldua-Huici Arantxa Eceiza Aitor Arbelaiz |
author_sort | Ander Orue |
collection | DOAJ |
description | With the aim to open new applications possibilities to novel biocomposites based on PLA/PMMA matrix and reinforced with sisal fibers, it was studied the effect of water immersion aging on biocomposite tensile properties. In the current study it was evidenced the importance of the annealing process and fiber/matrix adhesion on the mechanical performance of composites after immersing in water for around 7 months. The presence of the copolymer and the annealing process led to the minor extent of damage of mechanical properties of prepared biocomposites. Results obtained in the current study suggested that although the amount of copolymer incorporated in composites was low, the presence of copolymer is crucial to improve fiber/matrix adhesion and consequently the mechanical performance of composites after immersing in water. It was observed that even though the water uptake damaged the interfacial adhesion, leading to the tensile strength reduction; however, annealed composite with 30 wt% of fiber and modified with the copolymer showed a strength value of around 53.5 MPa. It must highlighted that even though water aged for 7 months, the annealed composite with copolymer showed yet a higher strength value than dried commercial mineral-filled PP composites reported in the literature. |
first_indexed | 2024-03-11T23:22:43Z |
format | Article |
id | doaj.art-7b2420e484be4fe998d4da2316f81dc4 |
institution | Directory Open Access Journal |
issn | 1544-0478 1544-046X |
language | English |
last_indexed | 2024-03-11T23:22:43Z |
publishDate | 2022-11-01 |
publisher | Taylor & Francis Group |
record_format | Article |
series | Journal of Natural Fibers |
spelling | doaj.art-7b2420e484be4fe998d4da2316f81dc42023-09-20T13:25:59ZengTaylor & Francis GroupJournal of Natural Fibers1544-04781544-046X2022-11-011915115241153510.1080/15440478.2022.20282112028211The Importance of Fiber/Matrix Adhesion and Annealing Process in Water Uptake of PLA/PMMA Matrix Composites Reinforced with Sisal Fibers: The Effect of Coupling Agent AdditionAnder Orue0Jon Anakabe1Ane Miren Zaldua-Huici2Arantxa Eceiza3Aitor Arbelaiz4Gipuzkoa, University of the Basque Country UPV/EHULeartiker S. CoopLeartiker S. CoopGipuzkoa, University of the Basque Country UPV/EHUGipuzkoa, University of the Basque Country UPV/EHUWith the aim to open new applications possibilities to novel biocomposites based on PLA/PMMA matrix and reinforced with sisal fibers, it was studied the effect of water immersion aging on biocomposite tensile properties. In the current study it was evidenced the importance of the annealing process and fiber/matrix adhesion on the mechanical performance of composites after immersing in water for around 7 months. The presence of the copolymer and the annealing process led to the minor extent of damage of mechanical properties of prepared biocomposites. Results obtained in the current study suggested that although the amount of copolymer incorporated in composites was low, the presence of copolymer is crucial to improve fiber/matrix adhesion and consequently the mechanical performance of composites after immersing in water. It was observed that even though the water uptake damaged the interfacial adhesion, leading to the tensile strength reduction; however, annealed composite with 30 wt% of fiber and modified with the copolymer showed a strength value of around 53.5 MPa. It must highlighted that even though water aged for 7 months, the annealed composite with copolymer showed yet a higher strength value than dried commercial mineral-filled PP composites reported in the literature.http://dx.doi.org/10.1080/15440478.2022.2028211sisal fiberspolymer-matrix compositeswater uptakemechanical propertiespoly(lactic acid)poly(methyl methacrylate) |
spellingShingle | Ander Orue Jon Anakabe Ane Miren Zaldua-Huici Arantxa Eceiza Aitor Arbelaiz The Importance of Fiber/Matrix Adhesion and Annealing Process in Water Uptake of PLA/PMMA Matrix Composites Reinforced with Sisal Fibers: The Effect of Coupling Agent Addition Journal of Natural Fibers sisal fibers polymer-matrix composites water uptake mechanical properties poly(lactic acid) poly(methyl methacrylate) |
title | The Importance of Fiber/Matrix Adhesion and Annealing Process in Water Uptake of PLA/PMMA Matrix Composites Reinforced with Sisal Fibers: The Effect of Coupling Agent Addition |
title_full | The Importance of Fiber/Matrix Adhesion and Annealing Process in Water Uptake of PLA/PMMA Matrix Composites Reinforced with Sisal Fibers: The Effect of Coupling Agent Addition |
title_fullStr | The Importance of Fiber/Matrix Adhesion and Annealing Process in Water Uptake of PLA/PMMA Matrix Composites Reinforced with Sisal Fibers: The Effect of Coupling Agent Addition |
title_full_unstemmed | The Importance of Fiber/Matrix Adhesion and Annealing Process in Water Uptake of PLA/PMMA Matrix Composites Reinforced with Sisal Fibers: The Effect of Coupling Agent Addition |
title_short | The Importance of Fiber/Matrix Adhesion and Annealing Process in Water Uptake of PLA/PMMA Matrix Composites Reinforced with Sisal Fibers: The Effect of Coupling Agent Addition |
title_sort | importance of fiber matrix adhesion and annealing process in water uptake of pla pmma matrix composites reinforced with sisal fibers the effect of coupling agent addition |
topic | sisal fibers polymer-matrix composites water uptake mechanical properties poly(lactic acid) poly(methyl methacrylate) |
url | http://dx.doi.org/10.1080/15440478.2022.2028211 |
work_keys_str_mv | AT anderorue theimportanceoffibermatrixadhesionandannealingprocessinwateruptakeofplapmmamatrixcompositesreinforcedwithsisalfiberstheeffectofcouplingagentaddition AT jonanakabe theimportanceoffibermatrixadhesionandannealingprocessinwateruptakeofplapmmamatrixcompositesreinforcedwithsisalfiberstheeffectofcouplingagentaddition AT anemirenzalduahuici theimportanceoffibermatrixadhesionandannealingprocessinwateruptakeofplapmmamatrixcompositesreinforcedwithsisalfiberstheeffectofcouplingagentaddition AT arantxaeceiza theimportanceoffibermatrixadhesionandannealingprocessinwateruptakeofplapmmamatrixcompositesreinforcedwithsisalfiberstheeffectofcouplingagentaddition AT aitorarbelaiz theimportanceoffibermatrixadhesionandannealingprocessinwateruptakeofplapmmamatrixcompositesreinforcedwithsisalfiberstheeffectofcouplingagentaddition AT anderorue importanceoffibermatrixadhesionandannealingprocessinwateruptakeofplapmmamatrixcompositesreinforcedwithsisalfiberstheeffectofcouplingagentaddition AT jonanakabe importanceoffibermatrixadhesionandannealingprocessinwateruptakeofplapmmamatrixcompositesreinforcedwithsisalfiberstheeffectofcouplingagentaddition AT anemirenzalduahuici importanceoffibermatrixadhesionandannealingprocessinwateruptakeofplapmmamatrixcompositesreinforcedwithsisalfiberstheeffectofcouplingagentaddition AT arantxaeceiza importanceoffibermatrixadhesionandannealingprocessinwateruptakeofplapmmamatrixcompositesreinforcedwithsisalfiberstheeffectofcouplingagentaddition AT aitorarbelaiz importanceoffibermatrixadhesionandannealingprocessinwateruptakeofplapmmamatrixcompositesreinforcedwithsisalfiberstheeffectofcouplingagentaddition |