Fluid Flow Control in Cotton Threads with Mesoporous Silica Coatings

Abstract Microfluidic devices are important, e.g. in the field of point of care diagnostics. They are of special importance, if they are fabricated out of cheap and renewable materials. Tackling complex separation or sensing problems profits from modular three‐dimensional fluidic devices. Using cott...

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Main Authors: Joanna J. Mikolei, Mathias Stanzel, Raheleh Pardehkorram, Robert Lehn, Marcelo Ceolin, Annette Andrieu‐Brunsen
Format: Article
Language:English
Published: Wiley-VCH 2023-07-01
Series:Advanced Materials Interfaces
Subjects:
Online Access:https://doi.org/10.1002/admi.202300211
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author Joanna J. Mikolei
Mathias Stanzel
Raheleh Pardehkorram
Robert Lehn
Marcelo Ceolin
Annette Andrieu‐Brunsen
author_facet Joanna J. Mikolei
Mathias Stanzel
Raheleh Pardehkorram
Robert Lehn
Marcelo Ceolin
Annette Andrieu‐Brunsen
author_sort Joanna J. Mikolei
collection DOAJ
description Abstract Microfluidic devices are important, e.g. in the field of point of care diagnostics. They are of special importance, if they are fabricated out of cheap and renewable materials. Tackling complex separation or sensing problems profits from modular three‐dimensional fluidic devices. Using cotton threads as renewable material allows the modular design of three‐dimensional fluidic devices and networks. Here, fluidic threads with modular designed and tunable thread wettability are presented. The wettability is gradually adjusted from highly hydrophilic to hydrophobic. The thread wettability directly affects the fluid imbibition velocity as well as the distance, which the fluid imbibes into the thread. The wettability adjustment is based on a simple dense or mesoporous silica coating applied onto the cotton thread using sol‐gel chemistry and evaporation induced self‐assembly. In addition to wettability, the mesoporosity and the pore functionalization are used to tune the fluid velocity within the thread. Connecting different silica functionalized threads into one device by knotting them together, fluids can be guided through this network in a predicted manner, which allows a modular design of 3D microfluidic thread‐based devices.
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spelling doaj.art-7c942946e8a2497c89a5d0d5ff0393ef2023-07-27T06:27:26ZengWiley-VCHAdvanced Materials Interfaces2196-73502023-07-011021n/an/a10.1002/admi.202300211Fluid Flow Control in Cotton Threads with Mesoporous Silica CoatingsJoanna J. Mikolei0Mathias Stanzel1Raheleh Pardehkorram2Robert Lehn3Marcelo Ceolin4Annette Andrieu‐Brunsen5Ernst‐Berl Institut für Technische und Makromolekulare Chemie Technische Universität Darmstadt Peter‐Grünberg‐Straße 8 D‐64287 Darmstadt GermanyErnst‐Berl Institut für Technische und Makromolekulare Chemie Technische Universität Darmstadt Peter‐Grünberg‐Straße 8 D‐64287 Darmstadt GermanyErnst‐Berl Institut für Technische und Makromolekulare Chemie Technische Universität Darmstadt Peter‐Grünberg‐Straße 8 D‐64287 Darmstadt GermanyErnst‐Berl Institut für Technische und Makromolekulare Chemie Technische Universität Darmstadt Peter‐Grünberg‐Straße 8 D‐64287 Darmstadt GermanyInstituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas Universidad Nacional de La Plata and CONICET. Diag. 113 y 64 La Plata (1900) ArgentinaErnst‐Berl Institut für Technische und Makromolekulare Chemie Technische Universität Darmstadt Peter‐Grünberg‐Straße 8 D‐64287 Darmstadt GermanyAbstract Microfluidic devices are important, e.g. in the field of point of care diagnostics. They are of special importance, if they are fabricated out of cheap and renewable materials. Tackling complex separation or sensing problems profits from modular three‐dimensional fluidic devices. Using cotton threads as renewable material allows the modular design of three‐dimensional fluidic devices and networks. Here, fluidic threads with modular designed and tunable thread wettability are presented. The wettability is gradually adjusted from highly hydrophilic to hydrophobic. The thread wettability directly affects the fluid imbibition velocity as well as the distance, which the fluid imbibes into the thread. The wettability adjustment is based on a simple dense or mesoporous silica coating applied onto the cotton thread using sol‐gel chemistry and evaporation induced self‐assembly. In addition to wettability, the mesoporosity and the pore functionalization are used to tune the fluid velocity within the thread. Connecting different silica functionalized threads into one device by knotting them together, fluids can be guided through this network in a predicted manner, which allows a modular design of 3D microfluidic thread‐based devices.https://doi.org/10.1002/admi.202300211microfluidic in threadsnanopore functionalizationnanoporessilica coatingssol‐gel‐chemistrysurface modification
spellingShingle Joanna J. Mikolei
Mathias Stanzel
Raheleh Pardehkorram
Robert Lehn
Marcelo Ceolin
Annette Andrieu‐Brunsen
Fluid Flow Control in Cotton Threads with Mesoporous Silica Coatings
Advanced Materials Interfaces
microfluidic in threads
nanopore functionalization
nanopores
silica coatings
sol‐gel‐chemistry
surface modification
title Fluid Flow Control in Cotton Threads with Mesoporous Silica Coatings
title_full Fluid Flow Control in Cotton Threads with Mesoporous Silica Coatings
title_fullStr Fluid Flow Control in Cotton Threads with Mesoporous Silica Coatings
title_full_unstemmed Fluid Flow Control in Cotton Threads with Mesoporous Silica Coatings
title_short Fluid Flow Control in Cotton Threads with Mesoporous Silica Coatings
title_sort fluid flow control in cotton threads with mesoporous silica coatings
topic microfluidic in threads
nanopore functionalization
nanopores
silica coatings
sol‐gel‐chemistry
surface modification
url https://doi.org/10.1002/admi.202300211
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AT robertlehn fluidflowcontrolincottonthreadswithmesoporoussilicacoatings
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