Revisiting Sampson's theory for hydrodynamic transport in ultrathin nanopores
Sampson's theory for hydrodynamic resistance across a zero-length orifice was developed over a century ago. Although a powerful theory for entrance/exit resistance in nanopores, it lacks accuracy for relatively small-radius pores since it does not account for the molecular interface chemistry....
Main Authors: | , , |
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Format: | Article |
Language: | English |
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American Physical Society
2020-10-01
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Series: | Physical Review Research |
Online Access: | http://doi.org/10.1103/PhysRevResearch.2.043153 |
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author | Mohammad Heiranian Amir Taqieddin Narayana R. Aluru |
author_facet | Mohammad Heiranian Amir Taqieddin Narayana R. Aluru |
author_sort | Mohammad Heiranian |
collection | DOAJ |
description | Sampson's theory for hydrodynamic resistance across a zero-length orifice was developed over a century ago. Although a powerful theory for entrance/exit resistance in nanopores, it lacks accuracy for relatively small-radius pores since it does not account for the molecular interface chemistry. Here, Sampson's theory is revisited for the finite slippage and interfacial viscosity variation near the pore wall. The corrected Sampson's theory can accurately predict the hydrodynamic resistance from molecular dynamics simulations of ultrathin nanopores. |
first_indexed | 2024-04-24T10:22:55Z |
format | Article |
id | doaj.art-7ca82d146df749059833a0ea0b191d9f |
institution | Directory Open Access Journal |
issn | 2643-1564 |
language | English |
last_indexed | 2024-04-24T10:22:55Z |
publishDate | 2020-10-01 |
publisher | American Physical Society |
record_format | Article |
series | Physical Review Research |
spelling | doaj.art-7ca82d146df749059833a0ea0b191d9f2024-04-12T17:03:10ZengAmerican Physical SocietyPhysical Review Research2643-15642020-10-012404315310.1103/PhysRevResearch.2.043153Revisiting Sampson's theory for hydrodynamic transport in ultrathin nanoporesMohammad HeiranianAmir TaqieddinNarayana R. AluruSampson's theory for hydrodynamic resistance across a zero-length orifice was developed over a century ago. Although a powerful theory for entrance/exit resistance in nanopores, it lacks accuracy for relatively small-radius pores since it does not account for the molecular interface chemistry. Here, Sampson's theory is revisited for the finite slippage and interfacial viscosity variation near the pore wall. The corrected Sampson's theory can accurately predict the hydrodynamic resistance from molecular dynamics simulations of ultrathin nanopores.http://doi.org/10.1103/PhysRevResearch.2.043153 |
spellingShingle | Mohammad Heiranian Amir Taqieddin Narayana R. Aluru Revisiting Sampson's theory for hydrodynamic transport in ultrathin nanopores Physical Review Research |
title | Revisiting Sampson's theory for hydrodynamic transport in ultrathin nanopores |
title_full | Revisiting Sampson's theory for hydrodynamic transport in ultrathin nanopores |
title_fullStr | Revisiting Sampson's theory for hydrodynamic transport in ultrathin nanopores |
title_full_unstemmed | Revisiting Sampson's theory for hydrodynamic transport in ultrathin nanopores |
title_short | Revisiting Sampson's theory for hydrodynamic transport in ultrathin nanopores |
title_sort | revisiting sampson s theory for hydrodynamic transport in ultrathin nanopores |
url | http://doi.org/10.1103/PhysRevResearch.2.043153 |
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