Dependence of column ozone on future ODSs and GHGs in the variability of 500-ensemble members

Abstract State-of-the-art chemistry–climate models (CCMs) have indicated that a future decrease in ozone-depleting substances (ODSs) combined with an increase in greenhouse gases (GHGs) would increase the column ozone amount in most regions except the tropics and Antarctic. However, large Arctic ozo...

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Main Authors: Hideharu Akiyoshi, Masanao Kadowaki, Yousuke Yamashita, Toshiharu Nagatomo
Format: Article
Language:English
Published: Nature Portfolio 2023-01-01
Series:Scientific Reports
Online Access:https://doi.org/10.1038/s41598-023-27635-y
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author Hideharu Akiyoshi
Masanao Kadowaki
Yousuke Yamashita
Toshiharu Nagatomo
author_facet Hideharu Akiyoshi
Masanao Kadowaki
Yousuke Yamashita
Toshiharu Nagatomo
author_sort Hideharu Akiyoshi
collection DOAJ
description Abstract State-of-the-art chemistry–climate models (CCMs) have indicated that a future decrease in ozone-depleting substances (ODSs) combined with an increase in greenhouse gases (GHGs) would increase the column ozone amount in most regions except the tropics and Antarctic. However, large Arctic ozone losses have occurred at a frequency of approximately once per decade since the 1990s (1997, 2011 and 2020), despite the ODS concentration peaking in the mid-1990s. To understand this, CCMs were used to conduct 24 experiments with ODS and GHG concentrations set based on predicted values for future years; each experiment consisted of 500-member ensembles. The 50 ensemble members with the lowest column ozone in the mid- and high latitudes of the Northern Hemisphere showed a clear ODS dependence associated with low temperatures and a strong westerly zonal mean zonal wind. Even with high GHG concentrations, several ensemble members showed extremely low spring column ozone in the Arctic when ODS concentration remained above the 1980–1985 level. Hence, ODS concentrations should be reduced to avoid large ozone losses in the presence of a stable Arctic polar vortex. The average of the lowest 50 members indicates that GHG increase towards the end of the twenty-first century will not cause worse Arctic ozone depletion.
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spelling doaj.art-7d4aaa412ec14b60bb6a80c0402074422023-01-08T12:10:27ZengNature PortfolioScientific Reports2045-23222023-01-0113111210.1038/s41598-023-27635-yDependence of column ozone on future ODSs and GHGs in the variability of 500-ensemble membersHideharu Akiyoshi0Masanao Kadowaki1Yousuke Yamashita2Toshiharu Nagatomo3Earth System Division, National Institute for Environmental StudiesNuclear Science and Engineering Center, Japan Atomic Energy AgencyEarth System Division, National Institute for Environmental StudiesEarth System Division, National Institute for Environmental StudiesAbstract State-of-the-art chemistry–climate models (CCMs) have indicated that a future decrease in ozone-depleting substances (ODSs) combined with an increase in greenhouse gases (GHGs) would increase the column ozone amount in most regions except the tropics and Antarctic. However, large Arctic ozone losses have occurred at a frequency of approximately once per decade since the 1990s (1997, 2011 and 2020), despite the ODS concentration peaking in the mid-1990s. To understand this, CCMs were used to conduct 24 experiments with ODS and GHG concentrations set based on predicted values for future years; each experiment consisted of 500-member ensembles. The 50 ensemble members with the lowest column ozone in the mid- and high latitudes of the Northern Hemisphere showed a clear ODS dependence associated with low temperatures and a strong westerly zonal mean zonal wind. Even with high GHG concentrations, several ensemble members showed extremely low spring column ozone in the Arctic when ODS concentration remained above the 1980–1985 level. Hence, ODS concentrations should be reduced to avoid large ozone losses in the presence of a stable Arctic polar vortex. The average of the lowest 50 members indicates that GHG increase towards the end of the twenty-first century will not cause worse Arctic ozone depletion.https://doi.org/10.1038/s41598-023-27635-y
spellingShingle Hideharu Akiyoshi
Masanao Kadowaki
Yousuke Yamashita
Toshiharu Nagatomo
Dependence of column ozone on future ODSs and GHGs in the variability of 500-ensemble members
Scientific Reports
title Dependence of column ozone on future ODSs and GHGs in the variability of 500-ensemble members
title_full Dependence of column ozone on future ODSs and GHGs in the variability of 500-ensemble members
title_fullStr Dependence of column ozone on future ODSs and GHGs in the variability of 500-ensemble members
title_full_unstemmed Dependence of column ozone on future ODSs and GHGs in the variability of 500-ensemble members
title_short Dependence of column ozone on future ODSs and GHGs in the variability of 500-ensemble members
title_sort dependence of column ozone on future odss and ghgs in the variability of 500 ensemble members
url https://doi.org/10.1038/s41598-023-27635-y
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