RECYCLING PROCESS OF U3O8 POWDER IN MnO-Al2O3 DOPED LARGE GRAIN UO2 PELLETS

The effect of various process variables on the powder properties of recycled U3O8 from MnO-Al2O3 doped large grain UO2 pellets and the effect of those recycled U3O8 powders on the sintered density and grain size of MnO-Al2O3 doped large grain UO2 pellets have been investigated. The evolution of morp...

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Main Authors: JANG SOO OH, DONG-JOO KIM, JAE HO YANG, KEON SIK KIM, YOUNG WOO RHEE, YANG-HYUN KOO
Format: Article
Language:English
Published: Elsevier 2014-02-01
Series:Nuclear Engineering and Technology
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S1738573315300978
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author JANG SOO OH
DONG-JOO KIM
JAE HO YANG
KEON SIK KIM
YOUNG WOO RHEE
YANG-HYUN KOO
author_facet JANG SOO OH
DONG-JOO KIM
JAE HO YANG
KEON SIK KIM
YOUNG WOO RHEE
YANG-HYUN KOO
author_sort JANG SOO OH
collection DOAJ
description The effect of various process variables on the powder properties of recycled U3O8 from MnO-Al2O3 doped large grain UO2 pellets and the effect of those recycled U3O8 powders on the sintered density and grain size of MnO-Al2O3 doped large grain UO2 pellets have been investigated. The evolution of morphology, size, and BET surface area of the recycled U3O8 powders according to the respective variation of the thermo-mechanical treatment variables of oxidation temperature, powder milling, and sequential cyclic heat treatment of oxidation and then reduction was examined. The correlation between the BET surface area of recycled U3O8 powder and the sintered pellet properties of MnO-Al2O3 doped pellets showed that the pellet density and grain size of doped pellets were increased and then saturated by increasing the BET surface area of the recycled U3O8 powder. The density and grain size of the pellets were maximized when the BET surface area of the recycled U3O8 powder was in the vicinity of 3m2/g. Among the process variables applied in this study, the cyclic heat treatment followed by low temperature oxidation was a potential process combination to obtain the sinter-active U3O8 powder.
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spelling doaj.art-7db69ead90704c7ebe59791abfb9aa892022-12-21T22:24:45ZengElsevierNuclear Engineering and Technology1738-57332014-02-0146111712410.5516/NET.07.2013.043RECYCLING PROCESS OF U3O8 POWDER IN MnO-Al2O3 DOPED LARGE GRAIN UO2 PELLETSJANG SOO OHDONG-JOO KIMJAE HO YANGKEON SIK KIMYOUNG WOO RHEEYANG-HYUN KOOThe effect of various process variables on the powder properties of recycled U3O8 from MnO-Al2O3 doped large grain UO2 pellets and the effect of those recycled U3O8 powders on the sintered density and grain size of MnO-Al2O3 doped large grain UO2 pellets have been investigated. The evolution of morphology, size, and BET surface area of the recycled U3O8 powders according to the respective variation of the thermo-mechanical treatment variables of oxidation temperature, powder milling, and sequential cyclic heat treatment of oxidation and then reduction was examined. The correlation between the BET surface area of recycled U3O8 powder and the sintered pellet properties of MnO-Al2O3 doped pellets showed that the pellet density and grain size of doped pellets were increased and then saturated by increasing the BET surface area of the recycled U3O8 powder. The density and grain size of the pellets were maximized when the BET surface area of the recycled U3O8 powder was in the vicinity of 3m2/g. Among the process variables applied in this study, the cyclic heat treatment followed by low temperature oxidation was a potential process combination to obtain the sinter-active U3O8 powder.http://www.sciencedirect.com/science/article/pii/S1738573315300978Doped Large Grain PelletRecycling ProcessMnO-Al2O3U3O8 Powder
spellingShingle JANG SOO OH
DONG-JOO KIM
JAE HO YANG
KEON SIK KIM
YOUNG WOO RHEE
YANG-HYUN KOO
RECYCLING PROCESS OF U3O8 POWDER IN MnO-Al2O3 DOPED LARGE GRAIN UO2 PELLETS
Nuclear Engineering and Technology
Doped Large Grain Pellet
Recycling Process
MnO-Al2O3
U3O8 Powder
title RECYCLING PROCESS OF U3O8 POWDER IN MnO-Al2O3 DOPED LARGE GRAIN UO2 PELLETS
title_full RECYCLING PROCESS OF U3O8 POWDER IN MnO-Al2O3 DOPED LARGE GRAIN UO2 PELLETS
title_fullStr RECYCLING PROCESS OF U3O8 POWDER IN MnO-Al2O3 DOPED LARGE GRAIN UO2 PELLETS
title_full_unstemmed RECYCLING PROCESS OF U3O8 POWDER IN MnO-Al2O3 DOPED LARGE GRAIN UO2 PELLETS
title_short RECYCLING PROCESS OF U3O8 POWDER IN MnO-Al2O3 DOPED LARGE GRAIN UO2 PELLETS
title_sort recycling process of u3o8 powder in mno al2o3 doped large grain uo2 pellets
topic Doped Large Grain Pellet
Recycling Process
MnO-Al2O3
U3O8 Powder
url http://www.sciencedirect.com/science/article/pii/S1738573315300978
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