Fröhlich interaction dominated by a single phonon mode in CsPbBr3

Electron-phonon interaction is essential for understanding electronic and optical properties of lead halide perovskites. Here, using multiphonon Raman scattering and THz time-domain spectroscopy, the authors characterize the full phonon spectrum of CsPbBr3 and identify a single phonon mode that domi...

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Main Authors: Claudiu M. Iaru, Annalisa Brodu, Niels J. J. van Hoof, Stan E. T. ter Huurne, Jonathan Buhot, Federico Montanarella, Sophia Buhbut, Peter C. M. Christianen, Daniël Vanmaekelbergh, Celso de Mello Donega, Jaime Gòmez Rivas, Paul M. Koenraad, Andrei Yu. Silov
Format: Article
Language:English
Published: Nature Portfolio 2021-10-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-021-26192-0
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author Claudiu M. Iaru
Annalisa Brodu
Niels J. J. van Hoof
Stan E. T. ter Huurne
Jonathan Buhot
Federico Montanarella
Sophia Buhbut
Peter C. M. Christianen
Daniël Vanmaekelbergh
Celso de Mello Donega
Jaime Gòmez Rivas
Paul M. Koenraad
Andrei Yu. Silov
author_facet Claudiu M. Iaru
Annalisa Brodu
Niels J. J. van Hoof
Stan E. T. ter Huurne
Jonathan Buhot
Federico Montanarella
Sophia Buhbut
Peter C. M. Christianen
Daniël Vanmaekelbergh
Celso de Mello Donega
Jaime Gòmez Rivas
Paul M. Koenraad
Andrei Yu. Silov
author_sort Claudiu M. Iaru
collection DOAJ
description Electron-phonon interaction is essential for understanding electronic and optical properties of lead halide perovskites. Here, using multiphonon Raman scattering and THz time-domain spectroscopy, the authors characterize the full phonon spectrum of CsPbBr3 and identify a single phonon mode that dominates electron-phonon scattering.
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spelling doaj.art-7e5ca449a580406c9d802d83e6a700c32022-12-21T23:12:07ZengNature PortfolioNature Communications2041-17232021-10-011211810.1038/s41467-021-26192-0Fröhlich interaction dominated by a single phonon mode in CsPbBr3Claudiu M. Iaru0Annalisa Brodu1Niels J. J. van Hoof2Stan E. T. ter Huurne3Jonathan Buhot4Federico Montanarella5Sophia Buhbut6Peter C. M. Christianen7Daniël Vanmaekelbergh8Celso de Mello Donega9Jaime Gòmez Rivas10Paul M. Koenraad11Andrei Yu. Silov12Department of Applied Physics and Institute for Photonic Integration, Eindhoven University of TechnologyCondensed Matter and Interfaces, Debye Institute for Nanomaterials Science, Utrecht UniversityDepartment of Applied Physics and Institute for Photonic Integration, Eindhoven University of TechnologyDepartment of Applied Physics and Institute for Photonic Integration, Eindhoven University of TechnologyHH Wills Laboratory, University of BristolCondensed Matter and Interfaces, Debye Institute for Nanomaterials Science, Utrecht UniversityCondensed Matter and Interfaces, Debye Institute for Nanomaterials Science, Utrecht UniversityHigh Field Magnet Laboratory (HFML - EMFL), Radboud UniversityCondensed Matter and Interfaces, Debye Institute for Nanomaterials Science, Utrecht UniversityCondensed Matter and Interfaces, Debye Institute for Nanomaterials Science, Utrecht UniversityDepartment of Applied Physics and Institute for Photonic Integration, Eindhoven University of TechnologyDepartment of Applied Physics and Institute for Photonic Integration, Eindhoven University of TechnologyDepartment of Applied Physics and Institute for Photonic Integration, Eindhoven University of TechnologyElectron-phonon interaction is essential for understanding electronic and optical properties of lead halide perovskites. Here, using multiphonon Raman scattering and THz time-domain spectroscopy, the authors characterize the full phonon spectrum of CsPbBr3 and identify a single phonon mode that dominates electron-phonon scattering.https://doi.org/10.1038/s41467-021-26192-0
spellingShingle Claudiu M. Iaru
Annalisa Brodu
Niels J. J. van Hoof
Stan E. T. ter Huurne
Jonathan Buhot
Federico Montanarella
Sophia Buhbut
Peter C. M. Christianen
Daniël Vanmaekelbergh
Celso de Mello Donega
Jaime Gòmez Rivas
Paul M. Koenraad
Andrei Yu. Silov
Fröhlich interaction dominated by a single phonon mode in CsPbBr3
Nature Communications
title Fröhlich interaction dominated by a single phonon mode in CsPbBr3
title_full Fröhlich interaction dominated by a single phonon mode in CsPbBr3
title_fullStr Fröhlich interaction dominated by a single phonon mode in CsPbBr3
title_full_unstemmed Fröhlich interaction dominated by a single phonon mode in CsPbBr3
title_short Fröhlich interaction dominated by a single phonon mode in CsPbBr3
title_sort frohlich interaction dominated by a single phonon mode in cspbbr3
url https://doi.org/10.1038/s41467-021-26192-0
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