Retrieval of Aerosol Optical Depth and FMF over East Asia from Directional Intensity and Polarization Measurements of PARASOL

The advantages of performing aerosol retrieval with multi-angle, multi-spectral photopolarimetric measurements over intensity-only measurements come from this technique’s sensitivity to aerosols’ microphysical properties, such as their particle size, shape, and complex refraction index. In this stud...

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Main Authors: Shupeng Wang, Li Fang, Weishu Gong, Weihe Wang, Shihao Tang
Format: Article
Language:English
Published: MDPI AG 2023-12-01
Series:Atmosphere
Subjects:
Online Access:https://www.mdpi.com/2073-4433/15/1/6
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author Shupeng Wang
Li Fang
Weishu Gong
Weihe Wang
Shihao Tang
author_facet Shupeng Wang
Li Fang
Weishu Gong
Weihe Wang
Shihao Tang
author_sort Shupeng Wang
collection DOAJ
description The advantages of performing aerosol retrieval with multi-angle, multi-spectral photopolarimetric measurements over intensity-only measurements come from this technique’s sensitivity to aerosols’ microphysical properties, such as their particle size, shape, and complex refraction index. In this study, an extended LUT (Look Up Table) algorithm inherited from a previous work based on the assumption of surface reflectance spectral shape invariance is proposed and applied to PARASOL (Polarization and Anisotropy of Reflectances for Atmospheric Science coupled with Observations from a Lidar) measurements to retrieve aerosols’ optical properties including aerosol optical depth (AOD) and aerosol fine-mode fraction (FMF). Case studies conducted over East China for different aerosol scenes are investigated. A comparison between the retrieved AOD regional distribution and the corresponding MODIS (Moderate-resolution Imaging Spectroradiometer) C6 AOD products shows similar spatial distributions in the Jing-Jin-Ji (Beijing–Tianjin–Hebei, China’s mega city cluster) region. The PARASOL AOD retrievals were compared against the AOD measurements of seven AERONET (Aerosol Robotic Network) stations in China to evaluate the performance of the retrieval algorithm. In the fine-particle-dominated regions, lower RMSEs were found at Beijing and Hefei urban stations (0.16 and 0.18, respectively) compared to those at other fine-particle-dominated AERONET stations, which can be attributed to the assumption of surface reflectance spectral shape invariance that has significant advantages in separating the contribution of surface and aerosol scattering in urban areas. For the FMF validation, an RMSE of 0.23, a correlation of 0.57, and a bias of −0.01 were found. These results show that the algorithm performs reasonably in distinguishing the contribution of fine and coarse particles.
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spelling doaj.art-7f35a902ab8344f589807ed60556eaf22024-01-26T15:00:39ZengMDPI AGAtmosphere2073-44332023-12-01151610.3390/atmos15010006Retrieval of Aerosol Optical Depth and FMF over East Asia from Directional Intensity and Polarization Measurements of PARASOLShupeng Wang0Li Fang1Weishu Gong2Weihe Wang3Shihao Tang4Key Laboratory of Radiometric Calibration and Validation for Environmental Satellites, China Meteorological Administration, Beijing 100081, ChinaChina Siwei Surveying and Mapping Technology Co., Ltd., Beijing 100094, ChinaDepartment of Geographical Sciences, University of Maryland, 2181 Samuel J. LeFrak Hall, 7251 Preinkert Drive, College Park, MD 20742, USAKey Laboratory of Radiometric Calibration and Validation for Environmental Satellites, China Meteorological Administration, Beijing 100081, ChinaKey Laboratory of Radiometric Calibration and Validation for Environmental Satellites, China Meteorological Administration, Beijing 100081, ChinaThe advantages of performing aerosol retrieval with multi-angle, multi-spectral photopolarimetric measurements over intensity-only measurements come from this technique’s sensitivity to aerosols’ microphysical properties, such as their particle size, shape, and complex refraction index. In this study, an extended LUT (Look Up Table) algorithm inherited from a previous work based on the assumption of surface reflectance spectral shape invariance is proposed and applied to PARASOL (Polarization and Anisotropy of Reflectances for Atmospheric Science coupled with Observations from a Lidar) measurements to retrieve aerosols’ optical properties including aerosol optical depth (AOD) and aerosol fine-mode fraction (FMF). Case studies conducted over East China for different aerosol scenes are investigated. A comparison between the retrieved AOD regional distribution and the corresponding MODIS (Moderate-resolution Imaging Spectroradiometer) C6 AOD products shows similar spatial distributions in the Jing-Jin-Ji (Beijing–Tianjin–Hebei, China’s mega city cluster) region. The PARASOL AOD retrievals were compared against the AOD measurements of seven AERONET (Aerosol Robotic Network) stations in China to evaluate the performance of the retrieval algorithm. In the fine-particle-dominated regions, lower RMSEs were found at Beijing and Hefei urban stations (0.16 and 0.18, respectively) compared to those at other fine-particle-dominated AERONET stations, which can be attributed to the assumption of surface reflectance spectral shape invariance that has significant advantages in separating the contribution of surface and aerosol scattering in urban areas. For the FMF validation, an RMSE of 0.23, a correlation of 0.57, and a bias of −0.01 were found. These results show that the algorithm performs reasonably in distinguishing the contribution of fine and coarse particles.https://www.mdpi.com/2073-4433/15/1/6polarizationAODFMFaerosol retrievalPOLDER
spellingShingle Shupeng Wang
Li Fang
Weishu Gong
Weihe Wang
Shihao Tang
Retrieval of Aerosol Optical Depth and FMF over East Asia from Directional Intensity and Polarization Measurements of PARASOL
Atmosphere
polarization
AOD
FMF
aerosol retrieval
POLDER
title Retrieval of Aerosol Optical Depth and FMF over East Asia from Directional Intensity and Polarization Measurements of PARASOL
title_full Retrieval of Aerosol Optical Depth and FMF over East Asia from Directional Intensity and Polarization Measurements of PARASOL
title_fullStr Retrieval of Aerosol Optical Depth and FMF over East Asia from Directional Intensity and Polarization Measurements of PARASOL
title_full_unstemmed Retrieval of Aerosol Optical Depth and FMF over East Asia from Directional Intensity and Polarization Measurements of PARASOL
title_short Retrieval of Aerosol Optical Depth and FMF over East Asia from Directional Intensity and Polarization Measurements of PARASOL
title_sort retrieval of aerosol optical depth and fmf over east asia from directional intensity and polarization measurements of parasol
topic polarization
AOD
FMF
aerosol retrieval
POLDER
url https://www.mdpi.com/2073-4433/15/1/6
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