Climate response to off-equatorial stratospheric sulfur injections in three Earth system models – Part 1: Experimental protocols and surface changes

<p>There is now substantial literature on climate model studies of equatorial or tropical stratospheric SO<span class="inline-formula"><sub>2</sub></span> injections that aim to counteract the surface warming produced by rising concentrations of greenhouse gas...

Full description

Bibliographic Details
Main Authors: D. Visioni, E. M. Bednarz, W. R. Lee, B. Kravitz, A. Jones, J. M. Haywood, D. G. MacMartin
Format: Article
Language:English
Published: Copernicus Publications 2023-01-01
Series:Atmospheric Chemistry and Physics
Online Access:https://acp.copernicus.org/articles/23/663/2023/acp-23-663-2023.pdf
_version_ 1797951870700879872
author D. Visioni
E. M. Bednarz
W. R. Lee
B. Kravitz
B. Kravitz
A. Jones
J. M. Haywood
J. M. Haywood
D. G. MacMartin
author_facet D. Visioni
E. M. Bednarz
W. R. Lee
B. Kravitz
B. Kravitz
A. Jones
J. M. Haywood
J. M. Haywood
D. G. MacMartin
author_sort D. Visioni
collection DOAJ
description <p>There is now substantial literature on climate model studies of equatorial or tropical stratospheric SO<span class="inline-formula"><sub>2</sub></span> injections that aim to counteract the surface warming produced by rising concentrations of greenhouse gases. Here we present the results from the first systematic intercomparison of climate responses in three Earth system models wherein the injection of SO<span class="inline-formula"><sub>2</sub></span> occurs at different latitudes in the lower stratosphere: CESM2-WACCM6, UKESM1.0 and GISS-E2.1-G. The first two use a modal aerosol microphysics scheme, while two versions of GISS-E2.1-G use a bulk aerosol (One-Moment Aerosol, OMA) and a two-moment (Multiconfiguration Aerosol TRacker of mIXing state, MATRIX) microphysics approach, respectively. Our aim in this work is to determine commonalities and differences between the climate model responses in terms of the distribution of the optically reflective sulfate aerosols produced from the oxidation of SO<span class="inline-formula"><sub>2</sub></span> and in terms of the surface response to the resulting reduction in solar radiation. A focus on understanding the contribution of characteristics of models transport alongside their microphysical and chemical schemes, and on evaluating the resulting stratospheric responses in different models, is given in the companion paper <span class="cit" id="xref_paren.1">(<a href="#bib1.bibx6">Bednarz et al.</a>, <a href="#bib1.bibx6">2023</a>)</span>. The goal of this exercise is not to evaluate these single-point injection simulations as stand-alone proposed strategies to counteract global warming; instead we determine sources and areas of agreement and uncertainty in the simulated responses and, ultimately, the possibility of designing a comprehensive intervention strategy capable of managing multiple simultaneous climate goals through the combination of different injection locations.</p> <p>We find large disagreements between GISS-E2.1-G and the CESM2-WACCM6 and UKESM1.0 models regarding the magnitude of cooling per unit of aerosol optical depth (AOD) produced, which varies from 4.7 K per unit of AOD in CESM2-WACCM6 to 16.7 K in the GISS-E2.1-G version with two-moment aerosol microphysics. By normalizing the results with the global mean response in each of the models and thus assuming that the amount of SO<span class="inline-formula"><sub>2</sub></span> injected is a free parameter that can be managed independently, we highlight some commonalities in the overall distributions of the aerosols, in the inter-hemispheric surface temperature response and in shifts to the Intertropical Convergence Zone, as well as some areas of disagreement, such as the extent of the aerosol confinement in the equatorial region and the efficiency of the transport to polar latitudes. In conclusion, we demonstrate that it is possible to use these simulations to produce more comprehensive injection strategies in multiple climate models. However, large differences in the injection magnitudes can be expected, potentially increasing inter-model spreads in some stratospheric quantities (such as aerosol distribution) while reducing the spread in the surface response in terms of temperature and precipitation; furthermore, the selection of the injection locations may be dependent on the models' specific stratospheric transport.</p>
first_indexed 2024-04-10T22:37:26Z
format Article
id doaj.art-7f4ac84dfc414fdfa3b186b66ae6ac17
institution Directory Open Access Journal
issn 1680-7316
1680-7324
language English
last_indexed 2024-04-10T22:37:26Z
publishDate 2023-01-01
publisher Copernicus Publications
record_format Article
series Atmospheric Chemistry and Physics
spelling doaj.art-7f4ac84dfc414fdfa3b186b66ae6ac172023-01-16T10:40:15ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242023-01-012366368510.5194/acp-23-663-2023Climate response to off-equatorial stratospheric sulfur injections in three Earth system models – Part 1: Experimental protocols and surface changesD. Visioni0E. M. Bednarz1W. R. Lee2B. Kravitz3B. Kravitz4A. Jones5J. M. Haywood6J. M. Haywood7D. G. MacMartin8Sibley School of Mechanical and Aerospace Engineering, Cornell University, Ithaca, NY, USASibley School of Mechanical and Aerospace Engineering, Cornell University, Ithaca, NY, USASibley School of Mechanical and Aerospace Engineering, Cornell University, Ithaca, NY, USADepartment of Earth and Atmospheric Science, Indiana University, Bloomington, IN, USAAtmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, WA, USAMet Office Hadley Centre, Exeter, UKMet Office Hadley Centre, Exeter, UKCollege of Engineering, Mathematics and Physical Sciences, University of Exeter, Exeter, UKSibley School of Mechanical and Aerospace Engineering, Cornell University, Ithaca, NY, USA<p>There is now substantial literature on climate model studies of equatorial or tropical stratospheric SO<span class="inline-formula"><sub>2</sub></span> injections that aim to counteract the surface warming produced by rising concentrations of greenhouse gases. Here we present the results from the first systematic intercomparison of climate responses in three Earth system models wherein the injection of SO<span class="inline-formula"><sub>2</sub></span> occurs at different latitudes in the lower stratosphere: CESM2-WACCM6, UKESM1.0 and GISS-E2.1-G. The first two use a modal aerosol microphysics scheme, while two versions of GISS-E2.1-G use a bulk aerosol (One-Moment Aerosol, OMA) and a two-moment (Multiconfiguration Aerosol TRacker of mIXing state, MATRIX) microphysics approach, respectively. Our aim in this work is to determine commonalities and differences between the climate model responses in terms of the distribution of the optically reflective sulfate aerosols produced from the oxidation of SO<span class="inline-formula"><sub>2</sub></span> and in terms of the surface response to the resulting reduction in solar radiation. A focus on understanding the contribution of characteristics of models transport alongside their microphysical and chemical schemes, and on evaluating the resulting stratospheric responses in different models, is given in the companion paper <span class="cit" id="xref_paren.1">(<a href="#bib1.bibx6">Bednarz et al.</a>, <a href="#bib1.bibx6">2023</a>)</span>. The goal of this exercise is not to evaluate these single-point injection simulations as stand-alone proposed strategies to counteract global warming; instead we determine sources and areas of agreement and uncertainty in the simulated responses and, ultimately, the possibility of designing a comprehensive intervention strategy capable of managing multiple simultaneous climate goals through the combination of different injection locations.</p> <p>We find large disagreements between GISS-E2.1-G and the CESM2-WACCM6 and UKESM1.0 models regarding the magnitude of cooling per unit of aerosol optical depth (AOD) produced, which varies from 4.7 K per unit of AOD in CESM2-WACCM6 to 16.7 K in the GISS-E2.1-G version with two-moment aerosol microphysics. By normalizing the results with the global mean response in each of the models and thus assuming that the amount of SO<span class="inline-formula"><sub>2</sub></span> injected is a free parameter that can be managed independently, we highlight some commonalities in the overall distributions of the aerosols, in the inter-hemispheric surface temperature response and in shifts to the Intertropical Convergence Zone, as well as some areas of disagreement, such as the extent of the aerosol confinement in the equatorial region and the efficiency of the transport to polar latitudes. In conclusion, we demonstrate that it is possible to use these simulations to produce more comprehensive injection strategies in multiple climate models. However, large differences in the injection magnitudes can be expected, potentially increasing inter-model spreads in some stratospheric quantities (such as aerosol distribution) while reducing the spread in the surface response in terms of temperature and precipitation; furthermore, the selection of the injection locations may be dependent on the models' specific stratospheric transport.</p>https://acp.copernicus.org/articles/23/663/2023/acp-23-663-2023.pdf
spellingShingle D. Visioni
E. M. Bednarz
W. R. Lee
B. Kravitz
B. Kravitz
A. Jones
J. M. Haywood
J. M. Haywood
D. G. MacMartin
Climate response to off-equatorial stratospheric sulfur injections in three Earth system models – Part 1: Experimental protocols and surface changes
Atmospheric Chemistry and Physics
title Climate response to off-equatorial stratospheric sulfur injections in three Earth system models – Part 1: Experimental protocols and surface changes
title_full Climate response to off-equatorial stratospheric sulfur injections in three Earth system models – Part 1: Experimental protocols and surface changes
title_fullStr Climate response to off-equatorial stratospheric sulfur injections in three Earth system models – Part 1: Experimental protocols and surface changes
title_full_unstemmed Climate response to off-equatorial stratospheric sulfur injections in three Earth system models – Part 1: Experimental protocols and surface changes
title_short Climate response to off-equatorial stratospheric sulfur injections in three Earth system models – Part 1: Experimental protocols and surface changes
title_sort climate response to off equatorial stratospheric sulfur injections in three earth system models part 1 experimental protocols and surface changes
url https://acp.copernicus.org/articles/23/663/2023/acp-23-663-2023.pdf
work_keys_str_mv AT dvisioni climateresponsetooffequatorialstratosphericsulfurinjectionsinthreeearthsystemmodelspart1experimentalprotocolsandsurfacechanges
AT embednarz climateresponsetooffequatorialstratosphericsulfurinjectionsinthreeearthsystemmodelspart1experimentalprotocolsandsurfacechanges
AT wrlee climateresponsetooffequatorialstratosphericsulfurinjectionsinthreeearthsystemmodelspart1experimentalprotocolsandsurfacechanges
AT bkravitz climateresponsetooffequatorialstratosphericsulfurinjectionsinthreeearthsystemmodelspart1experimentalprotocolsandsurfacechanges
AT bkravitz climateresponsetooffequatorialstratosphericsulfurinjectionsinthreeearthsystemmodelspart1experimentalprotocolsandsurfacechanges
AT ajones climateresponsetooffequatorialstratosphericsulfurinjectionsinthreeearthsystemmodelspart1experimentalprotocolsandsurfacechanges
AT jmhaywood climateresponsetooffequatorialstratosphericsulfurinjectionsinthreeearthsystemmodelspart1experimentalprotocolsandsurfacechanges
AT jmhaywood climateresponsetooffequatorialstratosphericsulfurinjectionsinthreeearthsystemmodelspart1experimentalprotocolsandsurfacechanges
AT dgmacmartin climateresponsetooffequatorialstratosphericsulfurinjectionsinthreeearthsystemmodelspart1experimentalprotocolsandsurfacechanges