Light scattering at small angles by atmospheric irregular particles: modelling and laboratory measurements

We have investigated the behaviour of light scattering by particulates of various sizes (0.1 μm to 100 μm) at a small scattering angle (below 20°). It has been previously shown that, for a small angle, the scattered intensities are weakly dependent upon the particulates' composition (Renard et...

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Main Authors: T. Lurton, J.-B. Renard, D. Vignelles, M. Jeannot, R. Akiki, J.-L. Mineau, T. Tonnelier
Format: Article
Language:English
Published: Copernicus Publications 2014-04-01
Series:Atmospheric Measurement Techniques
Online Access:http://www.atmos-meas-tech.net/7/931/2014/amt-7-931-2014.pdf
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author T. Lurton
J.-B. Renard
D. Vignelles
M. Jeannot
R. Akiki
J.-L. Mineau
T. Tonnelier
author_facet T. Lurton
J.-B. Renard
D. Vignelles
M. Jeannot
R. Akiki
J.-L. Mineau
T. Tonnelier
author_sort T. Lurton
collection DOAJ
description We have investigated the behaviour of light scattering by particulates of various sizes (0.1 μm to 100 μm) at a small scattering angle (below 20°). It has been previously shown that, for a small angle, the scattered intensities are weakly dependent upon the particulates' composition (Renard et al., 2010). Particles found in the atmosphere exhibit roughness that leads to large discrepancies with the classical Mie solution in terms of scattered intensities in the low angular set-up. This article focuses on building an effective theoretical tool to predict the behaviour of light scattering by real particulates at a small scattering angle. <br><br> We present both the classical Mie theory and its adaptation to the case of rough particulates with a fairly simple roughness parameterisation. An experimental device was built, corresponding to the angular set-up of interest (low scattering angle and therefore low angular aperture). Measurements are presented that confirm the theoretical results with good agreement. It was found that differences between the classical Mie solution and actual measurements – especially for large particulates – can be attributed to the particulate roughness. <br><br> It was also found that, in this low angular set-up, saturation of the scattered intensities occurs for relatively small values of the roughness parameter. This confirms the low variability in the scattered intensities observed for atmospheric particulates of different kinds. A direct interest of this study is a broadening of the dynamic range of optical counters: using a small angle of aperture for measurements allows greater dynamics in terms of particle size. Thus it allows a single device to observe a broad range of particle sizes whilst utilising the same electronics.
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spelling doaj.art-7fb68cc0e2d1493893b2a398128cc1292022-12-21T17:32:08ZengCopernicus PublicationsAtmospheric Measurement Techniques1867-13811867-85482014-04-017493193910.5194/amt-7-931-2014Light scattering at small angles by atmospheric irregular particles: modelling and laboratory measurementsT. Lurton0J.-B. Renard1D. Vignelles2M. Jeannot3R. Akiki4J.-L. Mineau5T. Tonnelier6Laboratoire de Physique et Chimie de l'Environnement et de l'Espace, CNRS UMR7328, 3A, avenue de la Recherche Scientifique, 45071 Orléans, FranceLaboratoire de Physique et Chimie de l'Environnement et de l'Espace, CNRS UMR7328, 3A, avenue de la Recherche Scientifique, 45071 Orléans, FranceLaboratoire de Physique et Chimie de l'Environnement et de l'Espace, CNRS UMR7328, 3A, avenue de la Recherche Scientifique, 45071 Orléans, FranceLaboratoire de Physique et Chimie de l'Environnement et de l'Espace, CNRS UMR7328, 3A, avenue de la Recherche Scientifique, 45071 Orléans, FranceEnvironnement S. A., 111, boulevard Maximilien-Robespierre, 78300 Poissy, FranceEnvironnement S. A., 111, boulevard Maximilien-Robespierre, 78300 Poissy, FranceEnvironnement S. A., 111, boulevard Maximilien-Robespierre, 78300 Poissy, FranceWe have investigated the behaviour of light scattering by particulates of various sizes (0.1 μm to 100 μm) at a small scattering angle (below 20°). It has been previously shown that, for a small angle, the scattered intensities are weakly dependent upon the particulates' composition (Renard et al., 2010). Particles found in the atmosphere exhibit roughness that leads to large discrepancies with the classical Mie solution in terms of scattered intensities in the low angular set-up. This article focuses on building an effective theoretical tool to predict the behaviour of light scattering by real particulates at a small scattering angle. <br><br> We present both the classical Mie theory and its adaptation to the case of rough particulates with a fairly simple roughness parameterisation. An experimental device was built, corresponding to the angular set-up of interest (low scattering angle and therefore low angular aperture). Measurements are presented that confirm the theoretical results with good agreement. It was found that differences between the classical Mie solution and actual measurements – especially for large particulates – can be attributed to the particulate roughness. <br><br> It was also found that, in this low angular set-up, saturation of the scattered intensities occurs for relatively small values of the roughness parameter. This confirms the low variability in the scattered intensities observed for atmospheric particulates of different kinds. A direct interest of this study is a broadening of the dynamic range of optical counters: using a small angle of aperture for measurements allows greater dynamics in terms of particle size. Thus it allows a single device to observe a broad range of particle sizes whilst utilising the same electronics.http://www.atmos-meas-tech.net/7/931/2014/amt-7-931-2014.pdf
spellingShingle T. Lurton
J.-B. Renard
D. Vignelles
M. Jeannot
R. Akiki
J.-L. Mineau
T. Tonnelier
Light scattering at small angles by atmospheric irregular particles: modelling and laboratory measurements
Atmospheric Measurement Techniques
title Light scattering at small angles by atmospheric irregular particles: modelling and laboratory measurements
title_full Light scattering at small angles by atmospheric irregular particles: modelling and laboratory measurements
title_fullStr Light scattering at small angles by atmospheric irregular particles: modelling and laboratory measurements
title_full_unstemmed Light scattering at small angles by atmospheric irregular particles: modelling and laboratory measurements
title_short Light scattering at small angles by atmospheric irregular particles: modelling and laboratory measurements
title_sort light scattering at small angles by atmospheric irregular particles modelling and laboratory measurements
url http://www.atmos-meas-tech.net/7/931/2014/amt-7-931-2014.pdf
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