Radiative heat exchange driven by acoustic modes between two solids at the atomic scale

In the near field (for separation distances smaller than the thermal wavelength, of the order of some microns at ambient temperature), the radiative heat flow between two solids at different temperatures can exceed the blackbody limit by several orders of magnitude. Furthermore, at the atomic scale,...

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Main Authors: Gómez Viloria Mauricio, Guo Yangyu, Merabia Samy, Messina Riccardo, Ben-Abdallah Philippe
Format: Article
Language:English
Published: EDP Sciences 2023-01-01
Series:EPJ Web of Conferences
Online Access:https://www.epj-conferences.org/articles/epjconf/pdf/2023/13/epjconf_eosam2023_04012.pdf
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author Gómez Viloria Mauricio
Guo Yangyu
Merabia Samy
Messina Riccardo
Ben-Abdallah Philippe
author_facet Gómez Viloria Mauricio
Guo Yangyu
Merabia Samy
Messina Riccardo
Ben-Abdallah Philippe
author_sort Gómez Viloria Mauricio
collection DOAJ
description In the near field (for separation distances smaller than the thermal wavelength, of the order of some microns at ambient temperature), the radiative heat flow between two solids at different temperatures can exceed the blackbody limit by several orders of magnitude. Furthermore, at the atomic scale, close to contact, the vibrational modes of the crystal lattice are expected to play an important role in the heat exchange. While the contribution of acoustic phonons tunnel-ing due to Van der Waals forces and electrostatic interactions near the surface has been investigated [1–5], the radiative contribution of the acoustic modes has been neglected so far. Under the local assumption (wavevector k ≈ 0), optical modes are independent from the acoustic modes, and are the sole responsible for the thermal radiation for distances larger than a few nanometers. However at subnanometer distances, the electromagnetic response of solids is nonlocal (k ≠ 0) and both acoustic and optical modes are coupled, contributing together to the radiative heat exchange. In order to demonstrate the role of this contribu-tion, we calculate [6] the nonlocal dielectric permittivity of magnesium oxide (MgO) using molecular dynamics. In conjunction with fluctuational electrody-namics calculations, we are able to highlight the role of radiation between two polar crystals produced by acoustic modes compared to the expected results from the local theory. We show that this additional contribution can become the dominant channel for radiative heat exchanges at atomic scale in the cryo-genic regime (below 100 K). Since the acoustic vibration modes can be excited with the help of piezoelectric transducers, our work opens the possibility to the control of radiative heat exchanges at atomic scale using external mechanical actuation.
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spelling doaj.art-81abd92844bb4fe8a33cb128bcf79a222023-11-07T10:20:47ZengEDP SciencesEPJ Web of Conferences2100-014X2023-01-012870401210.1051/epjconf/202328704012epjconf_eosam2023_04012Radiative heat exchange driven by acoustic modes between two solids at the atomic scaleGómez Viloria Mauricio0Guo Yangyu1Merabia Samy2Messina Riccardo3Ben-Abdallah Philippe4Laboratoire Charles Fabry, UMR 8501, Institut d’Optique, CNRS, Université Paris-SaclayInstitut Lumière Matière, Université Claude Bernard Lyon 1, CNRS, Université de LyonInstitut Lumière Matière, Université Claude Bernard Lyon 1, CNRS, Université de LyonLaboratoire Charles Fabry, UMR 8501, Institut d’Optique, CNRS, Université Paris-SaclayLaboratoire Charles Fabry, UMR 8501, Institut d’Optique, CNRS, Université Paris-SaclayIn the near field (for separation distances smaller than the thermal wavelength, of the order of some microns at ambient temperature), the radiative heat flow between two solids at different temperatures can exceed the blackbody limit by several orders of magnitude. Furthermore, at the atomic scale, close to contact, the vibrational modes of the crystal lattice are expected to play an important role in the heat exchange. While the contribution of acoustic phonons tunnel-ing due to Van der Waals forces and electrostatic interactions near the surface has been investigated [1–5], the radiative contribution of the acoustic modes has been neglected so far. Under the local assumption (wavevector k ≈ 0), optical modes are independent from the acoustic modes, and are the sole responsible for the thermal radiation for distances larger than a few nanometers. However at subnanometer distances, the electromagnetic response of solids is nonlocal (k ≠ 0) and both acoustic and optical modes are coupled, contributing together to the radiative heat exchange. In order to demonstrate the role of this contribu-tion, we calculate [6] the nonlocal dielectric permittivity of magnesium oxide (MgO) using molecular dynamics. In conjunction with fluctuational electrody-namics calculations, we are able to highlight the role of radiation between two polar crystals produced by acoustic modes compared to the expected results from the local theory. We show that this additional contribution can become the dominant channel for radiative heat exchanges at atomic scale in the cryo-genic regime (below 100 K). Since the acoustic vibration modes can be excited with the help of piezoelectric transducers, our work opens the possibility to the control of radiative heat exchanges at atomic scale using external mechanical actuation.https://www.epj-conferences.org/articles/epjconf/pdf/2023/13/epjconf_eosam2023_04012.pdf
spellingShingle Gómez Viloria Mauricio
Guo Yangyu
Merabia Samy
Messina Riccardo
Ben-Abdallah Philippe
Radiative heat exchange driven by acoustic modes between two solids at the atomic scale
EPJ Web of Conferences
title Radiative heat exchange driven by acoustic modes between two solids at the atomic scale
title_full Radiative heat exchange driven by acoustic modes between two solids at the atomic scale
title_fullStr Radiative heat exchange driven by acoustic modes between two solids at the atomic scale
title_full_unstemmed Radiative heat exchange driven by acoustic modes between two solids at the atomic scale
title_short Radiative heat exchange driven by acoustic modes between two solids at the atomic scale
title_sort radiative heat exchange driven by acoustic modes between two solids at the atomic scale
url https://www.epj-conferences.org/articles/epjconf/pdf/2023/13/epjconf_eosam2023_04012.pdf
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