Catalytic-Dielectric Barrier Discharge Plasma Reactor For Methane and Carbon Dioxide Conversion

A catalytic - DBD plasma reactor was designed and developed for co-generation of synthesis gas and C2+ hydrocarbons from methane. A hybrid Artificial Neural Network - Genetic Algorithm (ANN-GA) was developed to model, simulate and optimize the reactor. Effects of CH4/CO2 feed ratio, total feed flow...

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Main Authors: Istadi Istadi, N. A. S. Amin
Format: Article
Language:English
Published: Masyarakat Katalis Indonesia - Indonesian Catalyst Society (MKICS) 2007-10-01
Series:Bulletin of Chemical Reaction Engineering & Catalysis
Subjects:
Online Access:https://journal.bcrec.id/index.php/bcrec/article/view/19717
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author Istadi Istadi
N. A. S. Amin
author_facet Istadi Istadi
N. A. S. Amin
author_sort Istadi Istadi
collection DOAJ
description A catalytic - DBD plasma reactor was designed and developed for co-generation of synthesis gas and C2+ hydrocarbons from methane. A hybrid Artificial Neural Network - Genetic Algorithm (ANN-GA) was developed to model, simulate and optimize the reactor. Effects of CH4/CO2 feed ratio, total feed flow rate, discharge voltage and reactor wall temperature on the performance of catalytic DBD plasma reactor was explored. The Pareto optimal solutions and corresponding optimal operating parameters ranges based on multi-objectives can be suggested for catalytic DBD plasma reactor owing to two cases, i.e. simultaneous maximization of CH4 conversion and C2+ selectivity, and H2 selectivity and H2/CO ratio. It can be concluded that the hybrid catalytic DBD plasma reactor is potential for co-generation of synthesis gas and higher hydrocarbons from methane and carbon dioxide and showed better than the conventional fixed bed reactor with respect to CH4 conversion, C2+ yield and H2 selectivity for CO2 OCM process. © 2007 by Authors, Published by BCREC Group. This is an open access article under the CC BY-SA License (https://creativecommons.org/licenses/by-sa/4.0)
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spelling doaj.art-81b1fd9e44f94a41a811052d01ee56e22023-09-22T04:12:09ZengMasyarakat Katalis Indonesia - Indonesian Catalyst Society (MKICS)Bulletin of Chemical Reaction Engineering & Catalysis1978-29932007-10-0122-3374410.9767/bcrec.2.2-3.8.37-448312Catalytic-Dielectric Barrier Discharge Plasma Reactor For Methane and Carbon Dioxide ConversionIstadi Istadi0N. A. S. Amin1Department of Chemical Engineering, Diponegoro University, Jl. Prof. Sudarto, Kampus Undip Tembalang, Semarang, IndonesiaFaculty of Chemical & Natural Resources Engineering, Universiti Teknologi Malaysia, Johor Bahru, MalaysiaA catalytic - DBD plasma reactor was designed and developed for co-generation of synthesis gas and C2+ hydrocarbons from methane. A hybrid Artificial Neural Network - Genetic Algorithm (ANN-GA) was developed to model, simulate and optimize the reactor. Effects of CH4/CO2 feed ratio, total feed flow rate, discharge voltage and reactor wall temperature on the performance of catalytic DBD plasma reactor was explored. The Pareto optimal solutions and corresponding optimal operating parameters ranges based on multi-objectives can be suggested for catalytic DBD plasma reactor owing to two cases, i.e. simultaneous maximization of CH4 conversion and C2+ selectivity, and H2 selectivity and H2/CO ratio. It can be concluded that the hybrid catalytic DBD plasma reactor is potential for co-generation of synthesis gas and higher hydrocarbons from methane and carbon dioxide and showed better than the conventional fixed bed reactor with respect to CH4 conversion, C2+ yield and H2 selectivity for CO2 OCM process. © 2007 by Authors, Published by BCREC Group. This is an open access article under the CC BY-SA License (https://creativecommons.org/licenses/by-sa/4.0)https://journal.bcrec.id/index.php/bcrec/article/view/19717plasma chemical reactorsoptimizationhybrid ann-gadielectric-barrier dischargepareto optimal solution
spellingShingle Istadi Istadi
N. A. S. Amin
Catalytic-Dielectric Barrier Discharge Plasma Reactor For Methane and Carbon Dioxide Conversion
Bulletin of Chemical Reaction Engineering & Catalysis
plasma chemical reactors
optimization
hybrid ann-ga
dielectric-barrier discharge
pareto optimal solution
title Catalytic-Dielectric Barrier Discharge Plasma Reactor For Methane and Carbon Dioxide Conversion
title_full Catalytic-Dielectric Barrier Discharge Plasma Reactor For Methane and Carbon Dioxide Conversion
title_fullStr Catalytic-Dielectric Barrier Discharge Plasma Reactor For Methane and Carbon Dioxide Conversion
title_full_unstemmed Catalytic-Dielectric Barrier Discharge Plasma Reactor For Methane and Carbon Dioxide Conversion
title_short Catalytic-Dielectric Barrier Discharge Plasma Reactor For Methane and Carbon Dioxide Conversion
title_sort catalytic dielectric barrier discharge plasma reactor for methane and carbon dioxide conversion
topic plasma chemical reactors
optimization
hybrid ann-ga
dielectric-barrier discharge
pareto optimal solution
url https://journal.bcrec.id/index.php/bcrec/article/view/19717
work_keys_str_mv AT istadiistadi catalyticdielectricbarrierdischargeplasmareactorformethaneandcarbondioxideconversion
AT nasamin catalyticdielectricbarrierdischargeplasmareactorformethaneandcarbondioxideconversion