Evaluation of the Simulated Atmospheric Particulate Matter Chemical Composition in Athens: Organic Aerosols Formation Sensitivity Tests

Air quality simulations were performed for the Greater Athens Area in very high spatial resolution using the modeling system WRF-CAMx. Sensitivity runs were performed using the SOAP and VBS schemes for organic gas–aerosol partitioning and oxidation. In January 2019, OA-VBS decreased compared to OA-S...

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Main Authors: Anastasia Poupkou, Serafim Kontos, Natalia Liora, Dimitrios Tsiaousidis, Ioannis Kapsomenakis, Stavros Solomos, Eleni Liakakou, Eleni Athanasopoulou, Georgios Grivas, Evangelia Diapouli, Vasiliki Vasilatou, Stefanos Papagiannis, Athena Progiou, Pavlos Kalabokas, Dimitrios Melas, Evangelos Gerasopoulos, Konstantinos Eleftheriadis, Christos Zerefos
Format: Article
Language:English
Published: MDPI AG 2023-08-01
Series:Environmental Sciences Proceedings
Subjects:
Online Access:https://www.mdpi.com/2673-4931/26/1/32
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author Anastasia Poupkou
Serafim Kontos
Natalia Liora
Dimitrios Tsiaousidis
Ioannis Kapsomenakis
Stavros Solomos
Eleni Liakakou
Eleni Athanasopoulou
Georgios Grivas
Evangelia Diapouli
Vasiliki Vasilatou
Stefanos Papagiannis
Athena Progiou
Pavlos Kalabokas
Dimitrios Melas
Evangelos Gerasopoulos
Konstantinos Eleftheriadis
Christos Zerefos
author_facet Anastasia Poupkou
Serafim Kontos
Natalia Liora
Dimitrios Tsiaousidis
Ioannis Kapsomenakis
Stavros Solomos
Eleni Liakakou
Eleni Athanasopoulou
Georgios Grivas
Evangelia Diapouli
Vasiliki Vasilatou
Stefanos Papagiannis
Athena Progiou
Pavlos Kalabokas
Dimitrios Melas
Evangelos Gerasopoulos
Konstantinos Eleftheriadis
Christos Zerefos
author_sort Anastasia Poupkou
collection DOAJ
description Air quality simulations were performed for the Greater Athens Area in very high spatial resolution using the modeling system WRF-CAMx. Sensitivity runs were performed using the SOAP and VBS schemes for organic gas–aerosol partitioning and oxidation. In January 2019, OA-VBS decreased compared to OA-SOAP because of POA reduction. In July 2019, the OA-VBS increased with respect to OA-SOAP as a result of the increase in SOA levels exceeding the decrease in POA ones. The comparison of the WRF-CAMx results against PM<sub>10</sub>, PM<sub>2.5,</sub> and OC surface measurements provides the first indications for improved CAMx performance with the VBS scheme.
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spelling doaj.art-82478a66f6f84866a862d7bd18889adc2024-03-27T13:37:11ZengMDPI AGEnvironmental Sciences Proceedings2673-49312023-08-012613210.3390/environsciproc2023026032Evaluation of the Simulated Atmospheric Particulate Matter Chemical Composition in Athens: Organic Aerosols Formation Sensitivity TestsAnastasia Poupkou0Serafim Kontos1Natalia Liora2Dimitrios Tsiaousidis3Ioannis Kapsomenakis4Stavros Solomos5Eleni Liakakou6Eleni Athanasopoulou7Georgios Grivas8Evangelia Diapouli9Vasiliki Vasilatou10Stefanos Papagiannis11Athena Progiou12Pavlos Kalabokas13Dimitrios Melas14Evangelos Gerasopoulos15Konstantinos Eleftheriadis16Christos Zerefos17Research Centre for Atmospheric Physics and Climatology, Academy of Athens, 10680 Athens, GreeceLaboratory of Atmospheric Physics, Aristotle University of Thessaloniki, 54124 Thessaloniki, GreeceLaboratory of Atmospheric Physics, Aristotle University of Thessaloniki, 54124 Thessaloniki, GreeceLaboratory of Atmospheric Physics, Aristotle University of Thessaloniki, 54124 Thessaloniki, GreeceResearch Centre for Atmospheric Physics and Climatology, Academy of Athens, 10680 Athens, GreeceResearch Centre for Atmospheric Physics and Climatology, Academy of Athens, 10680 Athens, GreeceInstitute for Environmental Research and Sustainable Development, National Observatory of Athens, 15236 Athens, GreeceInstitute for Environmental Research and Sustainable Development, National Observatory of Athens, 15236 Athens, GreeceInstitute for Environmental Research and Sustainable Development, National Observatory of Athens, 15236 Athens, GreeceEnvironmental Radioactivity & Aerosol Technology for Atmospheric and Climate Impact Laboratory, Institute of Nuclear & Radiological Sciences & Technology, Energy & Safety, N.C.S.R. “Demokritos”, 15310 Athens, GreeceEnvironmental Radioactivity & Aerosol Technology for Atmospheric and Climate Impact Laboratory, Institute of Nuclear & Radiological Sciences & Technology, Energy & Safety, N.C.S.R. “Demokritos”, 15310 Athens, GreeceEnvironmental Radioactivity & Aerosol Technology for Atmospheric and Climate Impact Laboratory, Institute of Nuclear & Radiological Sciences & Technology, Energy & Safety, N.C.S.R. “Demokritos”, 15310 Athens, GreeceAXON Enviro-Group Ltd., 11257 Athens, GreeceResearch Centre for Atmospheric Physics and Climatology, Academy of Athens, 10680 Athens, GreeceLaboratory of Atmospheric Physics, Aristotle University of Thessaloniki, 54124 Thessaloniki, GreeceInstitute for Environmental Research and Sustainable Development, National Observatory of Athens, 15236 Athens, GreeceEnvironmental Radioactivity & Aerosol Technology for Atmospheric and Climate Impact Laboratory, Institute of Nuclear & Radiological Sciences & Technology, Energy & Safety, N.C.S.R. “Demokritos”, 15310 Athens, GreeceResearch Centre for Atmospheric Physics and Climatology, Academy of Athens, 10680 Athens, GreeceAir quality simulations were performed for the Greater Athens Area in very high spatial resolution using the modeling system WRF-CAMx. Sensitivity runs were performed using the SOAP and VBS schemes for organic gas–aerosol partitioning and oxidation. In January 2019, OA-VBS decreased compared to OA-SOAP because of POA reduction. In July 2019, the OA-VBS increased with respect to OA-SOAP as a result of the increase in SOA levels exceeding the decrease in POA ones. The comparison of the WRF-CAMx results against PM<sub>10</sub>, PM<sub>2.5,</sub> and OC surface measurements provides the first indications for improved CAMx performance with the VBS scheme.https://www.mdpi.com/2673-4931/26/1/32PM atmospheric modelingorganic aerosolsCAMxSOAPVBS
spellingShingle Anastasia Poupkou
Serafim Kontos
Natalia Liora
Dimitrios Tsiaousidis
Ioannis Kapsomenakis
Stavros Solomos
Eleni Liakakou
Eleni Athanasopoulou
Georgios Grivas
Evangelia Diapouli
Vasiliki Vasilatou
Stefanos Papagiannis
Athena Progiou
Pavlos Kalabokas
Dimitrios Melas
Evangelos Gerasopoulos
Konstantinos Eleftheriadis
Christos Zerefos
Evaluation of the Simulated Atmospheric Particulate Matter Chemical Composition in Athens: Organic Aerosols Formation Sensitivity Tests
Environmental Sciences Proceedings
PM atmospheric modeling
organic aerosols
CAMx
SOAP
VBS
title Evaluation of the Simulated Atmospheric Particulate Matter Chemical Composition in Athens: Organic Aerosols Formation Sensitivity Tests
title_full Evaluation of the Simulated Atmospheric Particulate Matter Chemical Composition in Athens: Organic Aerosols Formation Sensitivity Tests
title_fullStr Evaluation of the Simulated Atmospheric Particulate Matter Chemical Composition in Athens: Organic Aerosols Formation Sensitivity Tests
title_full_unstemmed Evaluation of the Simulated Atmospheric Particulate Matter Chemical Composition in Athens: Organic Aerosols Formation Sensitivity Tests
title_short Evaluation of the Simulated Atmospheric Particulate Matter Chemical Composition in Athens: Organic Aerosols Formation Sensitivity Tests
title_sort evaluation of the simulated atmospheric particulate matter chemical composition in athens organic aerosols formation sensitivity tests
topic PM atmospheric modeling
organic aerosols
CAMx
SOAP
VBS
url https://www.mdpi.com/2673-4931/26/1/32
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