Construction of Ni3S2-NixPy/NF@NiFe LDH with heterogeneous interface to accelerate catalytic kinetics of overall water splitting

Reasonable design of a kind of non-noble metal catalyst with high catalytic performance, good stability and low cost is of great significance to realize the overall water splitting. Herein, a bottom-up method is proposed to synthesize NiFe layered double hydroxides (NiFe LDHs) coated sulfide/phosphi...

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Main Authors: Chengdong Han, Zhengtong Ji, Yongfu Zhu, Xue Yao, Peng Chen, Manying Guo, Lijun Zhao, Xingyou Lang, Qing Jiang
Format: Article
Language:English
Published: Taylor & Francis Group 2022-11-01
Series:Materials Research Letters
Subjects:
Online Access:https://www.tandfonline.com/doi/10.1080/21663831.2022.2094206
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author Chengdong Han
Zhengtong Ji
Yongfu Zhu
Xue Yao
Peng Chen
Manying Guo
Lijun Zhao
Xingyou Lang
Qing Jiang
author_facet Chengdong Han
Zhengtong Ji
Yongfu Zhu
Xue Yao
Peng Chen
Manying Guo
Lijun Zhao
Xingyou Lang
Qing Jiang
author_sort Chengdong Han
collection DOAJ
description Reasonable design of a kind of non-noble metal catalyst with high catalytic performance, good stability and low cost is of great significance to realize the overall water splitting. Herein, a bottom-up method is proposed to synthesize NiFe layered double hydroxides (NiFe LDHs) coated sulfide/phosphide heterostructure on the nickel foam (Ni3S2-NixPy/NF@NiFe LDH) through hydrothermal method combined with electrodeposition. Low overpotentials of only 248 and 298 mV are required to achieve the current densities of 50 and 100 mA cm−2 for OER. Meanwhile, the HER performance only needs 137 mV at a current density of 10 mA cm−2.
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spelling doaj.art-83aad7acc51c48ae9fd0710d3be0ca022022-12-22T03:40:04ZengTaylor & Francis GroupMaterials Research Letters2166-38312022-11-01101176277010.1080/21663831.2022.2094206Construction of Ni3S2-NixPy/NF@NiFe LDH with heterogeneous interface to accelerate catalytic kinetics of overall water splittingChengdong Han0Zhengtong Ji1Yongfu Zhu2Xue Yao3Peng Chen4Manying Guo5Lijun Zhao6Xingyou Lang7Qing Jiang8Key Laboratory of Automobile Materials, Ministry of Education and School of Materials Science and Engineering, Jilin University, Changchun, People’s Republic of ChinaKey Laboratory of Automobile Materials, Ministry of Education and School of Materials Science and Engineering, Jilin University, Changchun, People’s Republic of ChinaKey Laboratory of Automobile Materials, Ministry of Education and School of Materials Science and Engineering, Jilin University, Changchun, People’s Republic of ChinaKey Laboratory of Automobile Materials, Ministry of Education and School of Materials Science and Engineering, Jilin University, Changchun, People’s Republic of ChinaKey Laboratory of Automobile Materials, Ministry of Education and School of Materials Science and Engineering, Jilin University, Changchun, People’s Republic of ChinaKey Laboratory of Automobile Materials, Ministry of Education and School of Materials Science and Engineering, Jilin University, Changchun, People’s Republic of ChinaKey Laboratory of Automobile Materials, Ministry of Education and School of Materials Science and Engineering, Jilin University, Changchun, People’s Republic of ChinaKey Laboratory of Automobile Materials, Ministry of Education and School of Materials Science and Engineering, Jilin University, Changchun, People’s Republic of ChinaKey Laboratory of Automobile Materials, Ministry of Education and School of Materials Science and Engineering, Jilin University, Changchun, People’s Republic of ChinaReasonable design of a kind of non-noble metal catalyst with high catalytic performance, good stability and low cost is of great significance to realize the overall water splitting. Herein, a bottom-up method is proposed to synthesize NiFe layered double hydroxides (NiFe LDHs) coated sulfide/phosphide heterostructure on the nickel foam (Ni3S2-NixPy/NF@NiFe LDH) through hydrothermal method combined with electrodeposition. Low overpotentials of only 248 and 298 mV are required to achieve the current densities of 50 and 100 mA cm−2 for OER. Meanwhile, the HER performance only needs 137 mV at a current density of 10 mA cm−2.https://www.tandfonline.com/doi/10.1080/21663831.2022.2094206Electrocatalystheterogeneous interfacewater splitting
spellingShingle Chengdong Han
Zhengtong Ji
Yongfu Zhu
Xue Yao
Peng Chen
Manying Guo
Lijun Zhao
Xingyou Lang
Qing Jiang
Construction of Ni3S2-NixPy/NF@NiFe LDH with heterogeneous interface to accelerate catalytic kinetics of overall water splitting
Materials Research Letters
Electrocatalyst
heterogeneous interface
water splitting
title Construction of Ni3S2-NixPy/NF@NiFe LDH with heterogeneous interface to accelerate catalytic kinetics of overall water splitting
title_full Construction of Ni3S2-NixPy/NF@NiFe LDH with heterogeneous interface to accelerate catalytic kinetics of overall water splitting
title_fullStr Construction of Ni3S2-NixPy/NF@NiFe LDH with heterogeneous interface to accelerate catalytic kinetics of overall water splitting
title_full_unstemmed Construction of Ni3S2-NixPy/NF@NiFe LDH with heterogeneous interface to accelerate catalytic kinetics of overall water splitting
title_short Construction of Ni3S2-NixPy/NF@NiFe LDH with heterogeneous interface to accelerate catalytic kinetics of overall water splitting
title_sort construction of ni3s2 nixpy nf nife ldh with heterogeneous interface to accelerate catalytic kinetics of overall water splitting
topic Electrocatalyst
heterogeneous interface
water splitting
url https://www.tandfonline.com/doi/10.1080/21663831.2022.2094206
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