Enhanced Performance of GaN-based Ultraviolet Light Emitting Diodes by Photon Recycling Using Graphene Quantum Dots

Abstract Graphene quantum dots (GQDs) with an average diameter of 3.5 nm were prepared via pulsed laser ablation. The synthesized GQDs can improve the optical and electrical properties of InGaN/InAlGaN UV light emitting diodes (LEDs) remarkably. An enhancement of electroluminescence and a decrease o...

Full description

Bibliographic Details
Main Authors: Tzu-Neng Lin, Svette Reina Merden Santiago, Chi-Tsu Yuan, Kuo-Pin Chiu, Ji-Lin Shen, Ting-Chun Wang, Hao-Chung Kuo, Ching-Hsueh Chiu, Yung-Chi Yao, Ya-Ju Lee
Format: Article
Language:English
Published: Nature Portfolio 2017-08-01
Series:Scientific Reports
Online Access:https://doi.org/10.1038/s41598-017-07483-3
_version_ 1818423176036614144
author Tzu-Neng Lin
Svette Reina Merden Santiago
Chi-Tsu Yuan
Kuo-Pin Chiu
Ji-Lin Shen
Ting-Chun Wang
Hao-Chung Kuo
Ching-Hsueh Chiu
Yung-Chi Yao
Ya-Ju Lee
author_facet Tzu-Neng Lin
Svette Reina Merden Santiago
Chi-Tsu Yuan
Kuo-Pin Chiu
Ji-Lin Shen
Ting-Chun Wang
Hao-Chung Kuo
Ching-Hsueh Chiu
Yung-Chi Yao
Ya-Ju Lee
author_sort Tzu-Neng Lin
collection DOAJ
description Abstract Graphene quantum dots (GQDs) with an average diameter of 3.5 nm were prepared via pulsed laser ablation. The synthesized GQDs can improve the optical and electrical properties of InGaN/InAlGaN UV light emitting diodes (LEDs) remarkably. An enhancement of electroluminescence and a decrease of series resistance of LEDs were observed after incorporation of GQDs on the LED surface. As the GQD concentration is increased, the emitted light (series resistance) in the LED increases (decreases) accordingly. The light output power achieved a maximum increase as high as 71% after introducing GQDs with the concentration of 0.9 mg/ml. The improved performance of LEDs after the introduction of GQDs is explained by the photon recycling through the light extraction from the waveguide mode and the carrier transfer from GQDs to the active layer.
first_indexed 2024-12-14T13:37:59Z
format Article
id doaj.art-84637e9ed34047bf8788a2fa47890714
institution Directory Open Access Journal
issn 2045-2322
language English
last_indexed 2024-12-14T13:37:59Z
publishDate 2017-08-01
publisher Nature Portfolio
record_format Article
series Scientific Reports
spelling doaj.art-84637e9ed34047bf8788a2fa478907142022-12-21T22:59:31ZengNature PortfolioScientific Reports2045-23222017-08-01711910.1038/s41598-017-07483-3Enhanced Performance of GaN-based Ultraviolet Light Emitting Diodes by Photon Recycling Using Graphene Quantum DotsTzu-Neng Lin0Svette Reina Merden Santiago1Chi-Tsu Yuan2Kuo-Pin Chiu3Ji-Lin Shen4Ting-Chun Wang5Hao-Chung Kuo6Ching-Hsueh Chiu7Yung-Chi Yao8Ya-Ju Lee9Department of Physics and Center for Nanotechnology, Chung Yuan Christian UniversityDepartment of Physics and Center for Nanotechnology, Chung Yuan Christian UniversityDepartment of Physics and Center for Nanotechnology, Chung Yuan Christian UniversityDepartment of Physics and Center for Nanotechnology, Chung Yuan Christian UniversityDepartment of Physics and Center for Nanotechnology, Chung Yuan Christian UniversityDepartment of Photonics, Research Center Energy Technology and Strategy, National Cheng Kung UniversityDepartment of Photonics, National Chiao Tung UniversityDepartment of Electronic Engineering, Chung Yuan Christian UniversityInstitute of Electro-Optical Science and Technology, National Taiwan Normal UniversityInstitute of Electro-Optical Science and Technology, National Taiwan Normal UniversityAbstract Graphene quantum dots (GQDs) with an average diameter of 3.5 nm were prepared via pulsed laser ablation. The synthesized GQDs can improve the optical and electrical properties of InGaN/InAlGaN UV light emitting diodes (LEDs) remarkably. An enhancement of electroluminescence and a decrease of series resistance of LEDs were observed after incorporation of GQDs on the LED surface. As the GQD concentration is increased, the emitted light (series resistance) in the LED increases (decreases) accordingly. The light output power achieved a maximum increase as high as 71% after introducing GQDs with the concentration of 0.9 mg/ml. The improved performance of LEDs after the introduction of GQDs is explained by the photon recycling through the light extraction from the waveguide mode and the carrier transfer from GQDs to the active layer.https://doi.org/10.1038/s41598-017-07483-3
spellingShingle Tzu-Neng Lin
Svette Reina Merden Santiago
Chi-Tsu Yuan
Kuo-Pin Chiu
Ji-Lin Shen
Ting-Chun Wang
Hao-Chung Kuo
Ching-Hsueh Chiu
Yung-Chi Yao
Ya-Ju Lee
Enhanced Performance of GaN-based Ultraviolet Light Emitting Diodes by Photon Recycling Using Graphene Quantum Dots
Scientific Reports
title Enhanced Performance of GaN-based Ultraviolet Light Emitting Diodes by Photon Recycling Using Graphene Quantum Dots
title_full Enhanced Performance of GaN-based Ultraviolet Light Emitting Diodes by Photon Recycling Using Graphene Quantum Dots
title_fullStr Enhanced Performance of GaN-based Ultraviolet Light Emitting Diodes by Photon Recycling Using Graphene Quantum Dots
title_full_unstemmed Enhanced Performance of GaN-based Ultraviolet Light Emitting Diodes by Photon Recycling Using Graphene Quantum Dots
title_short Enhanced Performance of GaN-based Ultraviolet Light Emitting Diodes by Photon Recycling Using Graphene Quantum Dots
title_sort enhanced performance of gan based ultraviolet light emitting diodes by photon recycling using graphene quantum dots
url https://doi.org/10.1038/s41598-017-07483-3
work_keys_str_mv AT tzunenglin enhancedperformanceofganbasedultravioletlightemittingdiodesbyphotonrecyclingusinggraphenequantumdots
AT svettereinamerdensantiago enhancedperformanceofganbasedultravioletlightemittingdiodesbyphotonrecyclingusinggraphenequantumdots
AT chitsuyuan enhancedperformanceofganbasedultravioletlightemittingdiodesbyphotonrecyclingusinggraphenequantumdots
AT kuopinchiu enhancedperformanceofganbasedultravioletlightemittingdiodesbyphotonrecyclingusinggraphenequantumdots
AT jilinshen enhancedperformanceofganbasedultravioletlightemittingdiodesbyphotonrecyclingusinggraphenequantumdots
AT tingchunwang enhancedperformanceofganbasedultravioletlightemittingdiodesbyphotonrecyclingusinggraphenequantumdots
AT haochungkuo enhancedperformanceofganbasedultravioletlightemittingdiodesbyphotonrecyclingusinggraphenequantumdots
AT chinghsuehchiu enhancedperformanceofganbasedultravioletlightemittingdiodesbyphotonrecyclingusinggraphenequantumdots
AT yungchiyao enhancedperformanceofganbasedultravioletlightemittingdiodesbyphotonrecyclingusinggraphenequantumdots
AT yajulee enhancedperformanceofganbasedultravioletlightemittingdiodesbyphotonrecyclingusinggraphenequantumdots