Angular momentum of doubly magic 132Sn fission product: Experimental and theoretical aspects

Despite the numerous theoretical and experimental works published very recently, the way in which fission fragments acquire their angular momentum is still an open question. This angular momentum generation mechanism is important not only for improving our understanding of the fission process, but a...

Full description

Bibliographic Details
Main Authors: Serot Olivier, Chebboubi Abdelhazize, Nicholson Jehaan, Kessedjian Grégoire, Litaize Olivier, Sage Christophe, Meplan Olivier, Ramdhane Mourad, Köster Ulli, Kim Yung Hee
Format: Article
Language:English
Published: EDP Sciences 2023-01-01
Series:EPJ Web of Conferences
Online Access:https://www.epj-conferences.org/articles/epjconf/pdf/2023/10/epjconf_nd2023_04022.pdf
_version_ 1797807655285161984
author Serot Olivier
Chebboubi Abdelhazize
Nicholson Jehaan
Kessedjian Grégoire
Litaize Olivier
Sage Christophe
Meplan Olivier
Ramdhane Mourad
Köster Ulli
Kim Yung Hee
author_facet Serot Olivier
Chebboubi Abdelhazize
Nicholson Jehaan
Kessedjian Grégoire
Litaize Olivier
Sage Christophe
Meplan Olivier
Ramdhane Mourad
Köster Ulli
Kim Yung Hee
author_sort Serot Olivier
collection DOAJ
description Despite the numerous theoretical and experimental works published very recently, the way in which fission fragments acquire their angular momentum is still an open question. This angular momentum generation mechanism is important not only for improving our understanding of the fission process, but also for nuclear energy applications, since the angular momentum of fission fragments strongly impact the prompt gamma spectra and consequently the decay heat in a reactor. In this context, within the framework of a collaboration between the ‘Laboratoire de Physique Subatomique et Corpusculaire’ (LPSC, France), the ‘Institut Laue Langevin’ (ILL, France) and the CEA-Cadarache (France), an experimental program was developed on the LO-HENGRIN mass-spectrometer with the aim of measuring isomeric ratio of some fission products for different thermal-neutron-induced fission reactions. This paper will be focused on the results obtained for the spherical nucleus 132Sn following thermal-neutron-induced fission of both 235U and 241Pu targets. To further challenge the angular momentum generation models, 132Sn isomeric ratio (IR) was measured as a function of 132Sn fission product kinetic energy (KE). The angular momentum was determined by combining our experimental data with the calculations performed with the FIFRELIN Monte Carlo code. A clear angular momentum decrease with KE was observed for both reactions. Lastly, we investigate the dependence of the 132Sn angular momentum with the incident neutron energy, from thermal region up to 5 MeV (below the second-chance fission). For that, the four free available parameters in FIFRELIN are selected in order to reproduce the average prompt neutron multiplicity. In this way, the angular momentum is deduced for each neutron energy. These results are discussed in terms of the impact of the available intrinsic excitation energy at scission on the spin generation mechanism.
first_indexed 2024-03-13T06:25:53Z
format Article
id doaj.art-855eea31ddcd4d1eb45a7ec404cdf4bb
institution Directory Open Access Journal
issn 2100-014X
language English
last_indexed 2024-03-13T06:25:53Z
publishDate 2023-01-01
publisher EDP Sciences
record_format Article
series EPJ Web of Conferences
spelling doaj.art-855eea31ddcd4d1eb45a7ec404cdf4bb2023-06-09T09:18:02ZengEDP SciencesEPJ Web of Conferences2100-014X2023-01-012840402210.1051/epjconf/202328404022epjconf_nd2023_04022Angular momentum of doubly magic 132Sn fission product: Experimental and theoretical aspectsSerot Olivier0Chebboubi Abdelhazize1Nicholson Jehaan2Kessedjian Grégoire3Litaize Olivier4Sage Christophe5Meplan Olivier6Ramdhane Mourad7Köster Ulli8Kim Yung Hee9CEA, DES, IRESNE, DER, SPRC, CadaracheCEA, DES, IRESNE, DER, SPRC, CadaracheCEA, DES, IRESNE, DER, SPRC, CadaracheCEA, DES, IRESNE, DER, SPRC, CadaracheCEA, DES, IRESNE, DER, SPRC, CadaracheLPSC, Université Grenoble Alpes, CNRS/IN2P3LPSC, Université Grenoble Alpes, CNRS/IN2P3LPSC, Université Grenoble Alpes, CNRS/IN2P3Institut Laue LangevinInstitut Laue LangevinDespite the numerous theoretical and experimental works published very recently, the way in which fission fragments acquire their angular momentum is still an open question. This angular momentum generation mechanism is important not only for improving our understanding of the fission process, but also for nuclear energy applications, since the angular momentum of fission fragments strongly impact the prompt gamma spectra and consequently the decay heat in a reactor. In this context, within the framework of a collaboration between the ‘Laboratoire de Physique Subatomique et Corpusculaire’ (LPSC, France), the ‘Institut Laue Langevin’ (ILL, France) and the CEA-Cadarache (France), an experimental program was developed on the LO-HENGRIN mass-spectrometer with the aim of measuring isomeric ratio of some fission products for different thermal-neutron-induced fission reactions. This paper will be focused on the results obtained for the spherical nucleus 132Sn following thermal-neutron-induced fission of both 235U and 241Pu targets. To further challenge the angular momentum generation models, 132Sn isomeric ratio (IR) was measured as a function of 132Sn fission product kinetic energy (KE). The angular momentum was determined by combining our experimental data with the calculations performed with the FIFRELIN Monte Carlo code. A clear angular momentum decrease with KE was observed for both reactions. Lastly, we investigate the dependence of the 132Sn angular momentum with the incident neutron energy, from thermal region up to 5 MeV (below the second-chance fission). For that, the four free available parameters in FIFRELIN are selected in order to reproduce the average prompt neutron multiplicity. In this way, the angular momentum is deduced for each neutron energy. These results are discussed in terms of the impact of the available intrinsic excitation energy at scission on the spin generation mechanism.https://www.epj-conferences.org/articles/epjconf/pdf/2023/10/epjconf_nd2023_04022.pdf
spellingShingle Serot Olivier
Chebboubi Abdelhazize
Nicholson Jehaan
Kessedjian Grégoire
Litaize Olivier
Sage Christophe
Meplan Olivier
Ramdhane Mourad
Köster Ulli
Kim Yung Hee
Angular momentum of doubly magic 132Sn fission product: Experimental and theoretical aspects
EPJ Web of Conferences
title Angular momentum of doubly magic 132Sn fission product: Experimental and theoretical aspects
title_full Angular momentum of doubly magic 132Sn fission product: Experimental and theoretical aspects
title_fullStr Angular momentum of doubly magic 132Sn fission product: Experimental and theoretical aspects
title_full_unstemmed Angular momentum of doubly magic 132Sn fission product: Experimental and theoretical aspects
title_short Angular momentum of doubly magic 132Sn fission product: Experimental and theoretical aspects
title_sort angular momentum of doubly magic 132sn fission product experimental and theoretical aspects
url https://www.epj-conferences.org/articles/epjconf/pdf/2023/10/epjconf_nd2023_04022.pdf
work_keys_str_mv AT serotolivier angularmomentumofdoublymagic132snfissionproductexperimentalandtheoreticalaspects
AT chebboubiabdelhazize angularmomentumofdoublymagic132snfissionproductexperimentalandtheoreticalaspects
AT nicholsonjehaan angularmomentumofdoublymagic132snfissionproductexperimentalandtheoreticalaspects
AT kessedjiangregoire angularmomentumofdoublymagic132snfissionproductexperimentalandtheoreticalaspects
AT litaizeolivier angularmomentumofdoublymagic132snfissionproductexperimentalandtheoreticalaspects
AT sagechristophe angularmomentumofdoublymagic132snfissionproductexperimentalandtheoreticalaspects
AT meplanolivier angularmomentumofdoublymagic132snfissionproductexperimentalandtheoreticalaspects
AT ramdhanemourad angularmomentumofdoublymagic132snfissionproductexperimentalandtheoreticalaspects
AT kosterulli angularmomentumofdoublymagic132snfissionproductexperimentalandtheoreticalaspects
AT kimyunghee angularmomentumofdoublymagic132snfissionproductexperimentalandtheoreticalaspects