Roller Nanoimprinted Honeycomb Texture as an Efficient Antireflective Coating for Perovskite Solar Cells

Abstract The properly chosen light management strategy in perovskite solar cell devices is indispensable in achieving high power conversion efficiency. To diminish the reflection losses, texturization of the front surface, similar to what is used in established solar cell technologies, shall be take...

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Main Authors: Maciej Krajewski, Adrian Callies, Minasadat Heydarian, Maryamsadat Heydarian, Mario Hanser, Patricia S. C. Schulze, Benedikt Bläsi, Oliver Höhn
Format: Article
Language:English
Published: Wiley-VCH 2023-09-01
Series:Advanced Materials Interfaces
Subjects:
Online Access:https://doi.org/10.1002/admi.202300134
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author Maciej Krajewski
Adrian Callies
Minasadat Heydarian
Maryamsadat Heydarian
Mario Hanser
Patricia S. C. Schulze
Benedikt Bläsi
Oliver Höhn
author_facet Maciej Krajewski
Adrian Callies
Minasadat Heydarian
Maryamsadat Heydarian
Mario Hanser
Patricia S. C. Schulze
Benedikt Bläsi
Oliver Höhn
author_sort Maciej Krajewski
collection DOAJ
description Abstract The properly chosen light management strategy in perovskite solar cell devices is indispensable in achieving high power conversion efficiency. To diminish the reflection losses, texturization of the front surface, similar to what is used in established solar cell technologies, shall be taken into consideration. Within this paper, a honeycomb‐like textured SU‐8 photoresist layer is applied using a roller nanoimprint technique onto a planar perovskite solar cell to minimize reflection losses. The results show that the applied honeycomb pattern reduces the solar‐weighted reflectance from 13.6% to 2.7%, which enhances the current density of the unmodified cell by 2.1 mA cm−2, outperforming the commonly used planar MgF2 antireflective coating by 0.5 mA cm−2. The experimental results are combined with optical modeling to find optimized structures and predict the optical behavior within a solar module. The process used within this work can be transferred to perovskite‐silicon tandem solar cells, providing a promising pathway for the reflection reduction in future devices.
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spelling doaj.art-8590197ee95d4dd8bfa75f0867b62c6d2023-09-13T07:27:03ZengWiley-VCHAdvanced Materials Interfaces2196-73502023-09-011026n/an/a10.1002/admi.202300134Roller Nanoimprinted Honeycomb Texture as an Efficient Antireflective Coating for Perovskite Solar CellsMaciej Krajewski0Adrian Callies1Minasadat Heydarian2Maryamsadat Heydarian3Mario Hanser4Patricia S. C. Schulze5Benedikt Bläsi6Oliver Höhn7University of Warsaw Faculty of Physics Warsaw 02‐093 PolandFraunhofer Institute for Solar Energy Systems ISE im Breisgau 79110 Freiburg GermanyFraunhofer Institute for Solar Energy Systems ISE im Breisgau 79110 Freiburg GermanyFraunhofer Institute for Solar Energy Systems ISE im Breisgau 79110 Freiburg GermanyFraunhofer Institute for Solar Energy Systems ISE im Breisgau 79110 Freiburg GermanyFraunhofer Institute for Solar Energy Systems ISE im Breisgau 79110 Freiburg GermanyFraunhofer Institute for Solar Energy Systems ISE im Breisgau 79110 Freiburg GermanyFraunhofer Institute for Solar Energy Systems ISE im Breisgau 79110 Freiburg GermanyAbstract The properly chosen light management strategy in perovskite solar cell devices is indispensable in achieving high power conversion efficiency. To diminish the reflection losses, texturization of the front surface, similar to what is used in established solar cell technologies, shall be taken into consideration. Within this paper, a honeycomb‐like textured SU‐8 photoresist layer is applied using a roller nanoimprint technique onto a planar perovskite solar cell to minimize reflection losses. The results show that the applied honeycomb pattern reduces the solar‐weighted reflectance from 13.6% to 2.7%, which enhances the current density of the unmodified cell by 2.1 mA cm−2, outperforming the commonly used planar MgF2 antireflective coating by 0.5 mA cm−2. The experimental results are combined with optical modeling to find optimized structures and predict the optical behavior within a solar module. The process used within this work can be transferred to perovskite‐silicon tandem solar cells, providing a promising pathway for the reflection reduction in future devices.https://doi.org/10.1002/admi.202300134antireflective coatingsclean energy technologylight managementnanoimprint lithographyperovskite solar cellsRCWA simulations
spellingShingle Maciej Krajewski
Adrian Callies
Minasadat Heydarian
Maryamsadat Heydarian
Mario Hanser
Patricia S. C. Schulze
Benedikt Bläsi
Oliver Höhn
Roller Nanoimprinted Honeycomb Texture as an Efficient Antireflective Coating for Perovskite Solar Cells
Advanced Materials Interfaces
antireflective coatings
clean energy technology
light management
nanoimprint lithography
perovskite solar cells
RCWA simulations
title Roller Nanoimprinted Honeycomb Texture as an Efficient Antireflective Coating for Perovskite Solar Cells
title_full Roller Nanoimprinted Honeycomb Texture as an Efficient Antireflective Coating for Perovskite Solar Cells
title_fullStr Roller Nanoimprinted Honeycomb Texture as an Efficient Antireflective Coating for Perovskite Solar Cells
title_full_unstemmed Roller Nanoimprinted Honeycomb Texture as an Efficient Antireflective Coating for Perovskite Solar Cells
title_short Roller Nanoimprinted Honeycomb Texture as an Efficient Antireflective Coating for Perovskite Solar Cells
title_sort roller nanoimprinted honeycomb texture as an efficient antireflective coating for perovskite solar cells
topic antireflective coatings
clean energy technology
light management
nanoimprint lithography
perovskite solar cells
RCWA simulations
url https://doi.org/10.1002/admi.202300134
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