Programmable hierarchical plasmonic–photonic arrays via laser-induced film dewetting

Hierarchical and periodic nanostructures of dielectrics or metals are highly demanded for wide applications in optical, electrical, biological, and quantum devices. In this work, programmable plasmonic–photonic hierarchical nanostructures are fabricated using a facile and effective method with high...

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Main Authors: Zheng Zeyu, Miao Yu, Yao Jiyuan, Chen Jiamei, Wen Jialin, Chen Xiaodan, Lu Yanxin, Jiang Xiaofang, Shui Lingling
Format: Article
Language:English
Published: De Gruyter 2022-07-01
Series:Nanophotonics
Subjects:
Online Access:https://doi.org/10.1515/nanoph-2022-0272
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author Zheng Zeyu
Miao Yu
Yao Jiyuan
Chen Jiamei
Wen Jialin
Chen Xiaodan
Lu Yanxin
Jiang Xiaofang
Shui Lingling
author_facet Zheng Zeyu
Miao Yu
Yao Jiyuan
Chen Jiamei
Wen Jialin
Chen Xiaodan
Lu Yanxin
Jiang Xiaofang
Shui Lingling
author_sort Zheng Zeyu
collection DOAJ
description Hierarchical and periodic nanostructures of dielectrics or metals are highly demanded for wide applications in optical, electrical, biological, and quantum devices. In this work, programmable plasmonic–photonic hierarchical nanostructures are fabricated using a facile and effective method with high controllability and stable reproducibility. The fabrication involves colloidal self-assembly, metal film deposition, and pulsed laser-induced dewetting in sequence for controllably pairing metal nanostructures on dielectric nanospheres in either large area or a local precision. Au nanostructures including Au nanocrown (AuNC), large Au nanosphere (AuNS), and multiple small Au nanoparticles (AuNPs) have been paired one-on-one on assembled SiO2 nanosphere (SiO2NS) arrays, with size and shape controlled by correlating the laser fluence and irradiation time, and the Au film thickness. The fabricated hierarchical nanostructures demonstrate synergistic effect of the photonic effects from the monolayer SiO2NS arrays and the surface plasma resonance effect from the Au nanostructures. The dewetting induced metal film reshaping has been modeled theoretically corresponding to observed experimental results. We can directly “write” the plasmonic Au nanostructures on the photonic crystal array using a focused laser beam to form encode patterns, showing angle-dependent structural colors for anti-counterfeiting information storage and display in rigid/flexible and opaque/transparent devices. It provides a promising path to actively construct on-demand pixelated plasmonic–photonic arrays for optical multiplexing technology in sensing, information encryption, and display.
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spelling doaj.art-85bf9af39a6142669bbb6a6b98d0901a2023-01-19T12:47:01ZengDe GruyterNanophotonics2192-86142022-07-0111163641365110.1515/nanoph-2022-0272Programmable hierarchical plasmonic–photonic arrays via laser-induced film dewettingZheng Zeyu0Miao Yu1Yao Jiyuan2Chen Jiamei3Wen Jialin4Chen Xiaodan5Lu Yanxin6Jiang Xiaofang7Shui Lingling8Guangdong Provincial Key Laboratory of Nanophotonic Functional Materials and Devices, School of Information and Optoelectronic Science and Engineering, South China Normal University, Guangzhou510006, P. R. ChinaLaboratory of Quantum Engineering and Quantum Material, School of Physics and Telecommunication Engineering, South China Normal University, Guangzhou510006, ChinaGuangdong Provincial Key Laboratory of Nanophotonic Functional Materials and Devices, School of Information and Optoelectronic Science and Engineering, South China Normal University, Guangzhou510006, P. R. ChinaGuangdong Provincial Key Laboratory of Nanophotonic Functional Materials and Devices, School of Information and Optoelectronic Science and Engineering, South China Normal University, Guangzhou510006, P. R. ChinaGuangdong Provincial Key Laboratory of Nanophotonic Functional Materials and Devices, School of Information and Optoelectronic Science and Engineering, South China Normal University, Guangzhou510006, P. R. ChinaGuangdong Provincial Key Laboratory of Nanophotonic Functional Materials and Devices, School of Information and Optoelectronic Science and Engineering, South China Normal University, Guangzhou510006, P. R. ChinaLaboratory of Quantum Engineering and Quantum Material, School of Physics and Telecommunication Engineering, South China Normal University, Guangzhou510006, ChinaGuangdong Provincial Key Laboratory of Nanophotonic Functional Materials and Devices, School of Information and Optoelectronic Science and Engineering, South China Normal University, Guangzhou510006, P. R. ChinaGuangdong Provincial Key Laboratory of Nanophotonic Functional Materials and Devices, School of Information and Optoelectronic Science and Engineering, South China Normal University, Guangzhou510006, P. R. ChinaHierarchical and periodic nanostructures of dielectrics or metals are highly demanded for wide applications in optical, electrical, biological, and quantum devices. In this work, programmable plasmonic–photonic hierarchical nanostructures are fabricated using a facile and effective method with high controllability and stable reproducibility. The fabrication involves colloidal self-assembly, metal film deposition, and pulsed laser-induced dewetting in sequence for controllably pairing metal nanostructures on dielectric nanospheres in either large area or a local precision. Au nanostructures including Au nanocrown (AuNC), large Au nanosphere (AuNS), and multiple small Au nanoparticles (AuNPs) have been paired one-on-one on assembled SiO2 nanosphere (SiO2NS) arrays, with size and shape controlled by correlating the laser fluence and irradiation time, and the Au film thickness. The fabricated hierarchical nanostructures demonstrate synergistic effect of the photonic effects from the monolayer SiO2NS arrays and the surface plasma resonance effect from the Au nanostructures. The dewetting induced metal film reshaping has been modeled theoretically corresponding to observed experimental results. We can directly “write” the plasmonic Au nanostructures on the photonic crystal array using a focused laser beam to form encode patterns, showing angle-dependent structural colors for anti-counterfeiting information storage and display in rigid/flexible and opaque/transparent devices. It provides a promising path to actively construct on-demand pixelated plasmonic–photonic arrays for optical multiplexing technology in sensing, information encryption, and display.https://doi.org/10.1515/nanoph-2022-0272displayhierarchical nanostructureinformation storagelaser-induced dewettingphotonic crystalself-assembly
spellingShingle Zheng Zeyu
Miao Yu
Yao Jiyuan
Chen Jiamei
Wen Jialin
Chen Xiaodan
Lu Yanxin
Jiang Xiaofang
Shui Lingling
Programmable hierarchical plasmonic–photonic arrays via laser-induced film dewetting
Nanophotonics
display
hierarchical nanostructure
information storage
laser-induced dewetting
photonic crystal
self-assembly
title Programmable hierarchical plasmonic–photonic arrays via laser-induced film dewetting
title_full Programmable hierarchical plasmonic–photonic arrays via laser-induced film dewetting
title_fullStr Programmable hierarchical plasmonic–photonic arrays via laser-induced film dewetting
title_full_unstemmed Programmable hierarchical plasmonic–photonic arrays via laser-induced film dewetting
title_short Programmable hierarchical plasmonic–photonic arrays via laser-induced film dewetting
title_sort programmable hierarchical plasmonic photonic arrays via laser induced film dewetting
topic display
hierarchical nanostructure
information storage
laser-induced dewetting
photonic crystal
self-assembly
url https://doi.org/10.1515/nanoph-2022-0272
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