Trends and Variability of Ozone Pollution over the Mountain-Basin Areas in Sichuan Province during 2013–2020: Synoptic Impacts and Formation Regimes

Sichuan Province, the most industrialized and populated region in southwestern China, has been experiencing severe ozone pollution in the boreal warm season (April–September). With a surface ozone monitoring network and reanalysis dataset, we find that nearly all cities in Sichuan Province showed po...

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Bibliographic Details
Main Authors: Youfan Chen, Han Han, Murong Zhang, Yuanhong Zhao, Yipeng Huang, Mi Zhou, Cong Wang, Guangyan He, Ran Huang, Bin Luo, Yongtao Hu
Format: Article
Language:English
Published: MDPI AG 2021-11-01
Series:Atmosphere
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Online Access:https://www.mdpi.com/2073-4433/12/12/1557
Description
Summary:Sichuan Province, the most industrialized and populated region in southwestern China, has been experiencing severe ozone pollution in the boreal warm season (April–September). With a surface ozone monitoring network and reanalysis dataset, we find that nearly all cities in Sichuan Province showed positive increasing trends in the warm-season ozone levels. The warm-season daily maximum 8-h average (MDA8) ozone levels increased by 2.0 ppb (4.8%) year<sup>−1</sup> as a whole, with slightly larger trends in some sites such as a site in Zigong (5.2 ppb year<sup>−1</sup>). Seasonally, the monthly ozone level in Sichuan peaks from May to August (varies with year). The predominant warm-season synoptic patterns were objectively identified based on concurrent hourly meteorological fields from ERA5. High-pressure systems promote ozone production and result in high ozone concentrations, due to strong solar radiation as well as hot and dry atmospheric conditions. The increased occurrence of high-pressure patterns probably drives the ozone increase in Sichuan. When ozone pollution is relatively weak (with MDA8 ozone around 170 μg m<sup>−3</sup>), the air quality standard could be achieved in the short term by a 25% reduction of NO<sub>x</sub> and VOCs emissions. Strengthened emission control is needed when ozone pollution is more severe. Our study provides implications for effective emission control of ozone pollution in Sichuan.
ISSN:2073-4433