High-Resolution X-Ray Computed Tomography of Liquid CO2 Permeation in Water-Saturated Sandstone

Geological sequestration of carbon dioxide (CO2) is an effective method to achieve a substantial reduction in CO2 emissions to the atmosphere at a relatively low cost; however, the migration process of CO2 in deep saline aquifers has not been clarified. In order to evaluate the storage site and asse...

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Main Authors: Suguru UEMURA, Ryoto KATAOKA, Shohji TSUSHIMA, Shuichiro HIRAI
Format: Article
Language:English
Published: The Japan Society of Mechanical Engineers 2013-04-01
Series:Journal of Thermal Science and Technology
Subjects:
Online Access:https://www.jstage.jst.go.jp/article/jtst/8/1/8_152/_pdf/-char/en
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author Suguru UEMURA
Ryoto KATAOKA
Shohji TSUSHIMA
Shuichiro HIRAI
author_facet Suguru UEMURA
Ryoto KATAOKA
Shohji TSUSHIMA
Shuichiro HIRAI
author_sort Suguru UEMURA
collection DOAJ
description Geological sequestration of carbon dioxide (CO2) is an effective method to achieve a substantial reduction in CO2 emissions to the atmosphere at a relatively low cost; however, the migration process of CO2 in deep saline aquifers has not been clarified. In order to evaluate the storage site and assess the CO2 leakage risks and storage costs, fundamental visualization and study of immiscible two-phase flow in sandstone are required. This study observed the behavior of liquid CO2 injected into water-saturated Berea sandstone by using microfocus X-ray computed tomography with high spatial resolution. The three-dimensional CO2 distribution in the sample was clearly reconstructed. The bedding structure of the rock strongly determined the CO2 permeation process, and a strong correlation was seen between the local porosity of the sample and the CO2 saturation. The real time CO2 permeation process was also observed in the transparent images that showed the CO2 gradually permeating the rock in the axial direction with increased saturation in the higher porosity beddings. The effects of the sandstone micro-heterogeneity on the behavior of the injected liquid CO2 are discussed.
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spelling doaj.art-8787803ffb024d6886d2acef73769ee72022-12-22T02:41:00ZengThe Japan Society of Mechanical EngineersJournal of Thermal Science and Technology1880-55662013-04-018115216410.1299/jtst.8.152jtstHigh-Resolution X-Ray Computed Tomography of Liquid CO2 Permeation in Water-Saturated SandstoneSuguru UEMURA0Ryoto KATAOKA1Shohji TSUSHIMA2Shuichiro HIRAI3Tokyo Institute of TechnologyTokyo Institute of TechnologyTokyo Institute of TechnologyTokyo Institute of TechnologyGeological sequestration of carbon dioxide (CO2) is an effective method to achieve a substantial reduction in CO2 emissions to the atmosphere at a relatively low cost; however, the migration process of CO2 in deep saline aquifers has not been clarified. In order to evaluate the storage site and assess the CO2 leakage risks and storage costs, fundamental visualization and study of immiscible two-phase flow in sandstone are required. This study observed the behavior of liquid CO2 injected into water-saturated Berea sandstone by using microfocus X-ray computed tomography with high spatial resolution. The three-dimensional CO2 distribution in the sample was clearly reconstructed. The bedding structure of the rock strongly determined the CO2 permeation process, and a strong correlation was seen between the local porosity of the sample and the CO2 saturation. The real time CO2 permeation process was also observed in the transparent images that showed the CO2 gradually permeating the rock in the axial direction with increased saturation in the higher porosity beddings. The effects of the sandstone micro-heterogeneity on the behavior of the injected liquid CO2 are discussed.https://www.jstage.jst.go.jp/article/jtst/8/1/8_152/_pdf/-char/enco2 geological sequestrationliquid co2porous mediatwo-phase flowx-ray computed tomography
spellingShingle Suguru UEMURA
Ryoto KATAOKA
Shohji TSUSHIMA
Shuichiro HIRAI
High-Resolution X-Ray Computed Tomography of Liquid CO2 Permeation in Water-Saturated Sandstone
Journal of Thermal Science and Technology
co2 geological sequestration
liquid co2
porous media
two-phase flow
x-ray computed tomography
title High-Resolution X-Ray Computed Tomography of Liquid CO2 Permeation in Water-Saturated Sandstone
title_full High-Resolution X-Ray Computed Tomography of Liquid CO2 Permeation in Water-Saturated Sandstone
title_fullStr High-Resolution X-Ray Computed Tomography of Liquid CO2 Permeation in Water-Saturated Sandstone
title_full_unstemmed High-Resolution X-Ray Computed Tomography of Liquid CO2 Permeation in Water-Saturated Sandstone
title_short High-Resolution X-Ray Computed Tomography of Liquid CO2 Permeation in Water-Saturated Sandstone
title_sort high resolution x ray computed tomography of liquid co2 permeation in water saturated sandstone
topic co2 geological sequestration
liquid co2
porous media
two-phase flow
x-ray computed tomography
url https://www.jstage.jst.go.jp/article/jtst/8/1/8_152/_pdf/-char/en
work_keys_str_mv AT suguruuemura highresolutionxraycomputedtomographyofliquidco2permeationinwatersaturatedsandstone
AT ryotokataoka highresolutionxraycomputedtomographyofliquidco2permeationinwatersaturatedsandstone
AT shohjitsushima highresolutionxraycomputedtomographyofliquidco2permeationinwatersaturatedsandstone
AT shuichirohirai highresolutionxraycomputedtomographyofliquidco2permeationinwatersaturatedsandstone