Purcell-enhanced dipolar interactions in nanostructures

Strong light-induced interactions between atoms are known to cause nonlinearities at a few-photon level, which are crucial for applications in quantum information processing. Compared to free space, the scattering and the light-induced dipolar interaction of atoms can be enhanced by a dielectric env...

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Main Authors: A. Skljarow, H. Kübler, C. S. Adams, T. Pfau, R. Löw, H. Alaeian
Format: Article
Language:English
Published: American Physical Society 2022-04-01
Series:Physical Review Research
Online Access:http://doi.org/10.1103/PhysRevResearch.4.023073
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author A. Skljarow
H. Kübler
C. S. Adams
T. Pfau
R. Löw
H. Alaeian
author_facet A. Skljarow
H. Kübler
C. S. Adams
T. Pfau
R. Löw
H. Alaeian
author_sort A. Skljarow
collection DOAJ
description Strong light-induced interactions between atoms are known to cause nonlinearities at a few-photon level, which are crucial for applications in quantum information processing. Compared to free space, the scattering and the light-induced dipolar interaction of atoms can be enhanced by a dielectric environment. For this Purcell effect, either a cavity or a waveguide can be used. Here, we combine the high densities achievable in thermal atomic vapors with an efficient coupling to a slot waveguide. In contrast to free-space interactions, atoms aligned within the slot exhibit repulsive interactions that are further enhanced by a factor of 8 due to the Purcell effect. The corresponding blueshift of the transition frequency of atoms arranged in the essentially one-dimensional geometry vanishes above the saturation, providing a controllable nonlinearity at the few-photon level. The experimental results are in good agreement with Monte Carlo simulations that include the dielectric environment, dipolar interactions, and motional effects. The results pave the way towards a robust scalable platform for quantum nonlinear optics and all-optical quantum information processing at room temperature.
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spelling doaj.art-87b0c7151f5f4e1580cc084a4ab04f3e2024-04-12T17:20:18ZengAmerican Physical SocietyPhysical Review Research2643-15642022-04-014202307310.1103/PhysRevResearch.4.023073Purcell-enhanced dipolar interactions in nanostructuresA. SkljarowH. KüblerC. S. AdamsT. PfauR. LöwH. AlaeianStrong light-induced interactions between atoms are known to cause nonlinearities at a few-photon level, which are crucial for applications in quantum information processing. Compared to free space, the scattering and the light-induced dipolar interaction of atoms can be enhanced by a dielectric environment. For this Purcell effect, either a cavity or a waveguide can be used. Here, we combine the high densities achievable in thermal atomic vapors with an efficient coupling to a slot waveguide. In contrast to free-space interactions, atoms aligned within the slot exhibit repulsive interactions that are further enhanced by a factor of 8 due to the Purcell effect. The corresponding blueshift of the transition frequency of atoms arranged in the essentially one-dimensional geometry vanishes above the saturation, providing a controllable nonlinearity at the few-photon level. The experimental results are in good agreement with Monte Carlo simulations that include the dielectric environment, dipolar interactions, and motional effects. The results pave the way towards a robust scalable platform for quantum nonlinear optics and all-optical quantum information processing at room temperature.http://doi.org/10.1103/PhysRevResearch.4.023073
spellingShingle A. Skljarow
H. Kübler
C. S. Adams
T. Pfau
R. Löw
H. Alaeian
Purcell-enhanced dipolar interactions in nanostructures
Physical Review Research
title Purcell-enhanced dipolar interactions in nanostructures
title_full Purcell-enhanced dipolar interactions in nanostructures
title_fullStr Purcell-enhanced dipolar interactions in nanostructures
title_full_unstemmed Purcell-enhanced dipolar interactions in nanostructures
title_short Purcell-enhanced dipolar interactions in nanostructures
title_sort purcell enhanced dipolar interactions in nanostructures
url http://doi.org/10.1103/PhysRevResearch.4.023073
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