The Different Impacts of Emissions and Meteorology on PM<sub>2.5</sub> Changes in Various Regions in China: A Case Study

Emissions and meteorology are significant factors affecting aerosol pollution, but it is not sufficient to understand their relative contributions to aerosol pollution changes. In this study, the observational data and the chemical model (GRAPES_CUACE) are combined to estimate the drivers of PM<s...

Full description

Bibliographic Details
Main Authors: Wenjie Zhang, Hong Wang, Xiaoye Zhang, Yue Peng, Zhaodong Liu, Junting Zhong, Yaqiang Wang, Huizheng Che, Yifan Zhao
Format: Article
Language:English
Published: MDPI AG 2022-01-01
Series:Atmosphere
Subjects:
Online Access:https://www.mdpi.com/2073-4433/13/2/222
_version_ 1797482875952562176
author Wenjie Zhang
Hong Wang
Xiaoye Zhang
Yue Peng
Zhaodong Liu
Junting Zhong
Yaqiang Wang
Huizheng Che
Yifan Zhao
author_facet Wenjie Zhang
Hong Wang
Xiaoye Zhang
Yue Peng
Zhaodong Liu
Junting Zhong
Yaqiang Wang
Huizheng Che
Yifan Zhao
author_sort Wenjie Zhang
collection DOAJ
description Emissions and meteorology are significant factors affecting aerosol pollution, but it is not sufficient to understand their relative contributions to aerosol pollution changes. In this study, the observational data and the chemical model (GRAPES_CUACE) are combined to estimate the drivers of PM<sub>2.5</sub> changes in various regions (the Beijing–Tianjin–Hebei (BTH), the Central China (CC), the Yangtze River Delta (YRD), and the Pearl River Delta (PRD)) between the first month after COVID-19 (FMC_2020) (i.e., from 23 January to 23 February 2020) and the corresponding period in 2019 (FMC_2019). The results show that PM<sub>2.5</sub> mass concentration increased by 26% (from 61 to 77 µg m<sup>−3</sup>) in the BTH, while it decreased by 26% (from 94 to 70 µg m<sup>−3</sup>) in the CC, 29% (from 52 to 37 µg m<sup>−3</sup>) in the YRD, and 32% (from 34 to 23 µg m<sup>−3</sup>) in the PRD in FMC_2020 comparing with FMC_2019, respectively. In the BTH, although emissions reductions partly improved PM<sub>2.5</sub> pollution (−5%, i.e., PM<sub>2.5</sub> mass concentration decreased by 5% due to emissions) in FMC_2020 compared with that of FMC_2019, the total increase in PM<sub>2.5</sub> mass concentration was dominated by more unfavorable meteorological conditions (+31%, i.e., PM<sub>2.5</sub> mass concentration increased by 31% due to meteorology). In the CC and the YRD, emissions reductions (−33 and −36%) played a dominating role in the total decrease in PM<sub>2.5</sub> in FMC_2020, while the changed meteorological conditions partly worsened PM<sub>2.5</sub> pollution (+7 and +7%). In the PRD, emissions reductions (−23%) and more favorable meteorological conditions (−9%) led to a total decrease in PM<sub>2.5</sub> mass concentration. This study reminds us that the uncertainties of relative contributions of meteorological conditions and emissions on PM<sub>2.5</sub> changes in various regions are large, which is conducive to policymaking scientifically in China.
first_indexed 2024-03-09T22:38:49Z
format Article
id doaj.art-897b20a754aa4b8c9c9ac5355b2a94bb
institution Directory Open Access Journal
issn 2073-4433
language English
last_indexed 2024-03-09T22:38:49Z
publishDate 2022-01-01
publisher MDPI AG
record_format Article
series Atmosphere
spelling doaj.art-897b20a754aa4b8c9c9ac5355b2a94bb2023-11-23T18:44:09ZengMDPI AGAtmosphere2073-44332022-01-0113222210.3390/atmos13020222The Different Impacts of Emissions and Meteorology on PM<sub>2.5</sub> Changes in Various Regions in China: A Case StudyWenjie Zhang0Hong Wang1Xiaoye Zhang2Yue Peng3Zhaodong Liu4Junting Zhong5Yaqiang Wang6Huizheng Che7Yifan Zhao8Department of Atmospheric and Oceanic Sciences and Institute of Atmospheric Sciences, Fudan University, Shanghai 200433, ChinaState Key Laboratory of Severe Weather and Key Laboratory of Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, ChinaState Key Laboratory of Severe Weather and Key Laboratory of Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, ChinaState Key Laboratory of Severe Weather and Key Laboratory of Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, ChinaState Key Laboratory of Severe Weather and Key Laboratory of Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, ChinaState Key Laboratory of Severe Weather and Key Laboratory of Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, ChinaState Key Laboratory of Severe Weather and Key Laboratory of Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, ChinaState Key Laboratory of Severe Weather and Key Laboratory of Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, ChinaState Key Laboratory of Severe Weather and Key Laboratory of Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, ChinaEmissions and meteorology are significant factors affecting aerosol pollution, but it is not sufficient to understand their relative contributions to aerosol pollution changes. In this study, the observational data and the chemical model (GRAPES_CUACE) are combined to estimate the drivers of PM<sub>2.5</sub> changes in various regions (the Beijing–Tianjin–Hebei (BTH), the Central China (CC), the Yangtze River Delta (YRD), and the Pearl River Delta (PRD)) between the first month after COVID-19 (FMC_2020) (i.e., from 23 January to 23 February 2020) and the corresponding period in 2019 (FMC_2019). The results show that PM<sub>2.5</sub> mass concentration increased by 26% (from 61 to 77 µg m<sup>−3</sup>) in the BTH, while it decreased by 26% (from 94 to 70 µg m<sup>−3</sup>) in the CC, 29% (from 52 to 37 µg m<sup>−3</sup>) in the YRD, and 32% (from 34 to 23 µg m<sup>−3</sup>) in the PRD in FMC_2020 comparing with FMC_2019, respectively. In the BTH, although emissions reductions partly improved PM<sub>2.5</sub> pollution (−5%, i.e., PM<sub>2.5</sub> mass concentration decreased by 5% due to emissions) in FMC_2020 compared with that of FMC_2019, the total increase in PM<sub>2.5</sub> mass concentration was dominated by more unfavorable meteorological conditions (+31%, i.e., PM<sub>2.5</sub> mass concentration increased by 31% due to meteorology). In the CC and the YRD, emissions reductions (−33 and −36%) played a dominating role in the total decrease in PM<sub>2.5</sub> in FMC_2020, while the changed meteorological conditions partly worsened PM<sub>2.5</sub> pollution (+7 and +7%). In the PRD, emissions reductions (−23%) and more favorable meteorological conditions (−9%) led to a total decrease in PM<sub>2.5</sub> mass concentration. This study reminds us that the uncertainties of relative contributions of meteorological conditions and emissions on PM<sub>2.5</sub> changes in various regions are large, which is conducive to policymaking scientifically in China.https://www.mdpi.com/2073-4433/13/2/222PM<sub>2.5</sub>meteorological conditionsemissions reductionsdifferent regions in China
spellingShingle Wenjie Zhang
Hong Wang
Xiaoye Zhang
Yue Peng
Zhaodong Liu
Junting Zhong
Yaqiang Wang
Huizheng Che
Yifan Zhao
The Different Impacts of Emissions and Meteorology on PM<sub>2.5</sub> Changes in Various Regions in China: A Case Study
Atmosphere
PM<sub>2.5</sub>
meteorological conditions
emissions reductions
different regions in China
title The Different Impacts of Emissions and Meteorology on PM<sub>2.5</sub> Changes in Various Regions in China: A Case Study
title_full The Different Impacts of Emissions and Meteorology on PM<sub>2.5</sub> Changes in Various Regions in China: A Case Study
title_fullStr The Different Impacts of Emissions and Meteorology on PM<sub>2.5</sub> Changes in Various Regions in China: A Case Study
title_full_unstemmed The Different Impacts of Emissions and Meteorology on PM<sub>2.5</sub> Changes in Various Regions in China: A Case Study
title_short The Different Impacts of Emissions and Meteorology on PM<sub>2.5</sub> Changes in Various Regions in China: A Case Study
title_sort different impacts of emissions and meteorology on pm sub 2 5 sub changes in various regions in china a case study
topic PM<sub>2.5</sub>
meteorological conditions
emissions reductions
different regions in China
url https://www.mdpi.com/2073-4433/13/2/222
work_keys_str_mv AT wenjiezhang thedifferentimpactsofemissionsandmeteorologyonpmsub25subchangesinvariousregionsinchinaacasestudy
AT hongwang thedifferentimpactsofemissionsandmeteorologyonpmsub25subchangesinvariousregionsinchinaacasestudy
AT xiaoyezhang thedifferentimpactsofemissionsandmeteorologyonpmsub25subchangesinvariousregionsinchinaacasestudy
AT yuepeng thedifferentimpactsofemissionsandmeteorologyonpmsub25subchangesinvariousregionsinchinaacasestudy
AT zhaodongliu thedifferentimpactsofemissionsandmeteorologyonpmsub25subchangesinvariousregionsinchinaacasestudy
AT juntingzhong thedifferentimpactsofemissionsandmeteorologyonpmsub25subchangesinvariousregionsinchinaacasestudy
AT yaqiangwang thedifferentimpactsofemissionsandmeteorologyonpmsub25subchangesinvariousregionsinchinaacasestudy
AT huizhengche thedifferentimpactsofemissionsandmeteorologyonpmsub25subchangesinvariousregionsinchinaacasestudy
AT yifanzhao thedifferentimpactsofemissionsandmeteorologyonpmsub25subchangesinvariousregionsinchinaacasestudy
AT wenjiezhang differentimpactsofemissionsandmeteorologyonpmsub25subchangesinvariousregionsinchinaacasestudy
AT hongwang differentimpactsofemissionsandmeteorologyonpmsub25subchangesinvariousregionsinchinaacasestudy
AT xiaoyezhang differentimpactsofemissionsandmeteorologyonpmsub25subchangesinvariousregionsinchinaacasestudy
AT yuepeng differentimpactsofemissionsandmeteorologyonpmsub25subchangesinvariousregionsinchinaacasestudy
AT zhaodongliu differentimpactsofemissionsandmeteorologyonpmsub25subchangesinvariousregionsinchinaacasestudy
AT juntingzhong differentimpactsofemissionsandmeteorologyonpmsub25subchangesinvariousregionsinchinaacasestudy
AT yaqiangwang differentimpactsofemissionsandmeteorologyonpmsub25subchangesinvariousregionsinchinaacasestudy
AT huizhengche differentimpactsofemissionsandmeteorologyonpmsub25subchangesinvariousregionsinchinaacasestudy
AT yifanzhao differentimpactsofemissionsandmeteorologyonpmsub25subchangesinvariousregionsinchinaacasestudy